沙箱实验为野外尺度二氧化碳储存模拟提供信息:小尺度异质性的影响

IF 4.6 3区 工程技术 Q2 ENERGY & FUELS
Jose Eduardo Ubillus , Sahar Bakhshian , Hailun Ni , David DiCarlo , Tip Meckel
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引用次数: 0

摘要

小规模的非均质性可以显著影响CO2羽流的命运和CO2迁移过程中的捕获。我们进行了地质碳储存场尺度模拟,以研究小尺度非均质性对烟柱动力学和捕获性能的影响。在浮力驱动的流动过程中,小规模的非均质性已被证明会增加被困二氧化碳的量。捕获的CO2饱和度通过以往在实际非均质区域浮力驱动流动中的沙盒实验工作进行验证,并通过临界CO2饱和度参数(即排水CO2相对渗透率曲线中的第一个非零值)实现。根据非均质性的类型和程度,出现了不同的临界co2饱和度值。此外,我们还研究了采用多个毛细管压力模型时小尺度非均质性的影响。研究表明,临界co2饱和度的增加降低了co2羽流的大小和横向范围,并伴有残余捕获的增加和溶解度捕获的减少。最后,我们表明,与毛细管压力模型无关,临界饱和度的增加导致co2羽流动力学分布和捕集性能相似。这些结果强调了量化小尺度非均质效应的重要性,因为它们影响co2羽流的大尺度行为。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Informing field-scale CO2storage simulations with sandbox experiments: The effect of small-scale heterogeneities
Small-scale heterogeneities can significantly affect the fate of the CO2 plume and trapping during CO2migration. We conducted geologic carbon storage field-scale simulations to investigate the impact of small-scale heterogeneities on plume dynamics and trapping performance. Small-scale heterogeneities have been shown to increase the amount of trapped CO2during buoyancy-driven flow. The trapped CO2 saturation is validated by previous sandbox experimental work during buoyancy-driven flow in realistic heterogeneous domains and is implemented through the critical CO2saturation parameter (i.e., the first non-zero value in the drainage CO2relative permeability curve). Depending on the type and degree of heterogeneity, various critical CO2saturation values are exhibited. Furthermore, we investigated the effect of small-scale heterogeneties when multiple capillary pressure models are employed. This study demonstrates that an increase in critical CO2saturation reduces the CO2plume size and lateral extent, accompanying an increase in residual trapping and a decrease in solubility trapping. Finally, we show that independent of the capillary pressure model used, an increase in critical saturation leads to similar CO2plume dynamics distribution and trapping performance. These results emphasize the importance of quantifying the effect of small-scale heterogeneity as they affect the large-scale behavior of the CO2plume.
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来源期刊
CiteScore
9.20
自引率
10.30%
发文量
199
审稿时长
4.8 months
期刊介绍: The International Journal of Greenhouse Gas Control is a peer reviewed journal focusing on scientific and engineering developments in greenhouse gas control through capture and storage at large stationary emitters in the power sector and in other major resource, manufacturing and production industries. The Journal covers all greenhouse gas emissions within the power and industrial sectors, and comprises both technical and non-technical related literature in one volume. Original research, review and comments papers are included.
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