{"title":"高性能(Zn0.5Mg0.5)TiO3陶瓷基复合薄膜为多模式平移单元和人体运动监测供电","authors":"Bochao Xie*, Yihuang Xie, Yingying Ma, Nianzu Luo, Tianyi Xiang, Chinglai Chin, Daiwei Wang, Feiyang Wang, Borui Li, Guowu Jiang* and Xiange Li*, ","doi":"10.1021/acsaelm.4c0164810.1021/acsaelm.4c01648","DOIUrl":null,"url":null,"abstract":"<p >The high operating temperature of the multimode translation unit presents persistent challenges in ensuring rapid power supply during emergency situations. To tackle this challenge, (Zn<sub>0.5</sub>Mg<sub>0.5</sub>)TiO<sub>3</sub> (ZMT) ceramic powder, known for its exceptional dielectric properties and high dielectric constant, was selected. It was combined with P(VDF-TrFE) to develop composite films exhibiting stable performance across varying temperatures. Leveraging the triboelectric mechanism, ZMT/P(VDF-TrFE) composite films were employed as the triboelectric layer to develop high-performance and temperature-stable self-powered devices. A remarkable open-circuit voltage of 451.63 V and a short-circuit current of 9.41 μA were observed in the ZMT-based triboelectric nanogenerator (ZMT-TENG), highlighting its potential for high-performance applications. It achieved a 21.1 times increase compared to traditional ceramic-based P(VDF-TrFE) TENGs, representing the highest electronic performance documented in the literature to date. Remarkably, <i>V</i><sub>OC</sub> and <i>I</i><sub>SC</sub> variations remained within 20% over a wide temperature range from −10 to 180 °C. This study not only advances TENG performance through material innovation but also enhances temperature stability, improving its effectiveness for both multimode translation units and high-precision human motion monitoring.</p>","PeriodicalId":3,"journal":{"name":"ACS Applied Electronic Materials","volume":"7 1","pages":"185–192 185–192"},"PeriodicalIF":4.7000,"publicationDate":"2024-12-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"High-Performance (Zn0.5Mg0.5)TiO3 Ceramics Based Composite Films for Powering a Multimode Translation Unit and Human Motion Monitoring\",\"authors\":\"Bochao Xie*, Yihuang Xie, Yingying Ma, Nianzu Luo, Tianyi Xiang, Chinglai Chin, Daiwei Wang, Feiyang Wang, Borui Li, Guowu Jiang* and Xiange Li*, \",\"doi\":\"10.1021/acsaelm.4c0164810.1021/acsaelm.4c01648\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >The high operating temperature of the multimode translation unit presents persistent challenges in ensuring rapid power supply during emergency situations. To tackle this challenge, (Zn<sub>0.5</sub>Mg<sub>0.5</sub>)TiO<sub>3</sub> (ZMT) ceramic powder, known for its exceptional dielectric properties and high dielectric constant, was selected. It was combined with P(VDF-TrFE) to develop composite films exhibiting stable performance across varying temperatures. Leveraging the triboelectric mechanism, ZMT/P(VDF-TrFE) composite films were employed as the triboelectric layer to develop high-performance and temperature-stable self-powered devices. A remarkable open-circuit voltage of 451.63 V and a short-circuit current of 9.41 μA were observed in the ZMT-based triboelectric nanogenerator (ZMT-TENG), highlighting its potential for high-performance applications. It achieved a 21.1 times increase compared to traditional ceramic-based P(VDF-TrFE) TENGs, representing the highest electronic performance documented in the literature to date. Remarkably, <i>V</i><sub>OC</sub> and <i>I</i><sub>SC</sub> variations remained within 20% over a wide temperature range from −10 to 180 °C. This study not only advances TENG performance through material innovation but also enhances temperature stability, improving its effectiveness for both multimode translation units and high-precision human motion monitoring.</p>\",\"PeriodicalId\":3,\"journal\":{\"name\":\"ACS Applied Electronic Materials\",\"volume\":\"7 1\",\"pages\":\"185–192 185–192\"},\"PeriodicalIF\":4.7000,\"publicationDate\":\"2024-12-19\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Applied Electronic Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acsaelm.4c01648\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, ELECTRICAL & ELECTRONIC\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Electronic Materials","FirstCategoryId":"88","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsaelm.4c01648","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, ELECTRICAL & ELECTRONIC","Score":null,"Total":0}
High-Performance (Zn0.5Mg0.5)TiO3 Ceramics Based Composite Films for Powering a Multimode Translation Unit and Human Motion Monitoring
The high operating temperature of the multimode translation unit presents persistent challenges in ensuring rapid power supply during emergency situations. To tackle this challenge, (Zn0.5Mg0.5)TiO3 (ZMT) ceramic powder, known for its exceptional dielectric properties and high dielectric constant, was selected. It was combined with P(VDF-TrFE) to develop composite films exhibiting stable performance across varying temperatures. Leveraging the triboelectric mechanism, ZMT/P(VDF-TrFE) composite films were employed as the triboelectric layer to develop high-performance and temperature-stable self-powered devices. A remarkable open-circuit voltage of 451.63 V and a short-circuit current of 9.41 μA were observed in the ZMT-based triboelectric nanogenerator (ZMT-TENG), highlighting its potential for high-performance applications. It achieved a 21.1 times increase compared to traditional ceramic-based P(VDF-TrFE) TENGs, representing the highest electronic performance documented in the literature to date. Remarkably, VOC and ISC variations remained within 20% over a wide temperature range from −10 to 180 °C. This study not only advances TENG performance through material innovation but also enhances temperature stability, improving its effectiveness for both multimode translation units and high-precision human motion monitoring.
期刊介绍:
ACS Applied Electronic Materials is an interdisciplinary journal publishing original research covering all aspects of electronic materials. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials science, engineering, optics, physics, and chemistry into important applications of electronic materials. Sample research topics that span the journal's scope are inorganic, organic, ionic and polymeric materials with properties that include conducting, semiconducting, superconducting, insulating, dielectric, magnetic, optoelectronic, piezoelectric, ferroelectric and thermoelectric.
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