Tayyab Sohail Aslam , Jinsong Chen , Umm Y. Umna , Kamran Muzaffar , Ateeq Ur Rehman , Syeda Andleeb Zahra Naqvi , Rahul Anil Borse , Yangyang Feng , Yaobing Wang
{"title":"Ag@g-C3N4/可见光下高效光催化析氧的MoS2异质结构。","authors":"Tayyab Sohail Aslam , Jinsong Chen , Umm Y. Umna , Kamran Muzaffar , Ateeq Ur Rehman , Syeda Andleeb Zahra Naqvi , Rahul Anil Borse , Yangyang Feng , Yaobing Wang","doi":"10.1039/d4cc05869k","DOIUrl":null,"url":null,"abstract":"<div><div>Herein, an Ag@g-C<sub>3</sub>N<sub>4</sub>/MoS<sub>2</sub> heterostructure is successfully synthesized for efficient solar-to-water oxidation. UV-vis DRS and steady-state PL analyses reveal the narrow band gap (2.10 eV) and efficient charge separation properties of the Ag nanoparticles and MoS<sub>2</sub>, respectively. The benefits include an excellent ∼3.2-fold increase in O<sub>2</sub> production rate (2727 μmol g<sup>−1</sup> h<sup>−1</sup>) compared to Ag@g-C<sub>3</sub>N<sub>4</sub>. A plausible Z-scheme mechanism is also proposed.</div></div>","PeriodicalId":67,"journal":{"name":"Chemical Communications","volume":"61 15","pages":"Pages 3207-3210"},"PeriodicalIF":4.2000,"publicationDate":"2025-01-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Ag@g-C3N4/MoS2 heterostructure for efficient photocatalytic oxygen evolution under visible light irradiation†\",\"authors\":\"Tayyab Sohail Aslam , Jinsong Chen , Umm Y. Umna , Kamran Muzaffar , Ateeq Ur Rehman , Syeda Andleeb Zahra Naqvi , Rahul Anil Borse , Yangyang Feng , Yaobing Wang\",\"doi\":\"10.1039/d4cc05869k\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Herein, an Ag@g-C<sub>3</sub>N<sub>4</sub>/MoS<sub>2</sub> heterostructure is successfully synthesized for efficient solar-to-water oxidation. UV-vis DRS and steady-state PL analyses reveal the narrow band gap (2.10 eV) and efficient charge separation properties of the Ag nanoparticles and MoS<sub>2</sub>, respectively. The benefits include an excellent ∼3.2-fold increase in O<sub>2</sub> production rate (2727 μmol g<sup>−1</sup> h<sup>−1</sup>) compared to Ag@g-C<sub>3</sub>N<sub>4</sub>. A plausible Z-scheme mechanism is also proposed.</div></div>\",\"PeriodicalId\":67,\"journal\":{\"name\":\"Chemical Communications\",\"volume\":\"61 15\",\"pages\":\"Pages 3207-3210\"},\"PeriodicalIF\":4.2000,\"publicationDate\":\"2025-01-24\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Chemical Communications\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://www.sciencedirect.com/org/science/article/pii/S1359734525001417\",\"RegionNum\":2,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Chemical Communications","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/org/science/article/pii/S1359734525001417","RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Ag@g-C3N4/MoS2 heterostructure for efficient photocatalytic oxygen evolution under visible light irradiation†
Herein, an Ag@g-C3N4/MoS2 heterostructure is successfully synthesized for efficient solar-to-water oxidation. UV-vis DRS and steady-state PL analyses reveal the narrow band gap (2.10 eV) and efficient charge separation properties of the Ag nanoparticles and MoS2, respectively. The benefits include an excellent ∼3.2-fold increase in O2 production rate (2727 μmol g−1 h−1) compared to Ag@g-C3N4. A plausible Z-scheme mechanism is also proposed.
期刊介绍:
ChemComm (Chemical Communications) is renowned as the fastest publisher of articles providing information on new avenues of research, drawn from all the world''s major areas of chemical research.