Ru@MnO2 core@shell纳米线作为高效太阳能驱动海水分解的双功能电催化剂。

IF 4.2 2区化学 Q2 CHEMISTRY, MULTIDISCIPLINARY

Chemical Communications Pub Date : 2025-01-02 DOI:10.1039/d4cc06144f

Na Li , Aitong Yang , Mengyuan Jin , Shun Wang , Ping Yu , Juan Wang , Huile Jin

{"title":"Ru@MnO2 core@shell纳米线作为高效太阳能驱动海水分解的双功能电催化剂。","authors":"Na Li , Aitong Yang , Mengyuan Jin , Shun Wang , Ping Yu , Juan Wang , Huile Jin","doi":"10.1039/d4cc06144f","DOIUrl":null,"url":null,"abstract":"<div><div>Seawater electrolysis technology for hydrogen production has attracted worldwide attention due to the abundant seawater resources. Herein, we proposed core–shell Ru@MnO<sub>2</sub> nanowires (NWs) with α/β-MnO<sub>2</sub> NWs as the core and amorphous Ru as the shell, in which the Ru@α-MnO<sub>2</sub> NWs exhibited lower overpotential and better stability. More importantly, they can operate stably as a bifunctional catalyst for more than 250 h and maintain excellent catalytic performance when driven by solar energy.</div></div>","PeriodicalId":67,"journal":{"name":"Chemical Communications","volume":"61 13","pages":"Pages 2762-2765"},"PeriodicalIF":4.2000,"publicationDate":"2025-01-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Ru@MnO2 core@shell nanowires as a bifunctional electrocatalyst for efficient solar-driven seawater splitting†\",\"authors\":\"Na Li , Aitong Yang , Mengyuan Jin , Shun Wang , Ping Yu , Juan Wang , Huile Jin\",\"doi\":\"10.1039/d4cc06144f\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Seawater electrolysis technology for hydrogen production has attracted worldwide attention due to the abundant seawater resources. Herein, we proposed core–shell Ru@MnO<sub>2</sub> nanowires (NWs) with α/β-MnO<sub>2</sub> NWs as the core and amorphous Ru as the shell, in which the Ru@α-MnO<sub>2</sub> NWs exhibited lower overpotential and better stability. More importantly, they can operate stably as a bifunctional catalyst for more than 250 h and maintain excellent catalytic performance when driven by solar energy.</div></div>\",\"PeriodicalId\":67,\"journal\":{\"name\":\"Chemical Communications\",\"volume\":\"61 13\",\"pages\":\"Pages 2762-2765\"},\"PeriodicalIF\":4.2000,\"publicationDate\":\"2025-01-02\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Chemical Communications\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://www.sciencedirect.com/org/science/article/pii/S1359734525000795\",\"RegionNum\":2,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Chemical Communications","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/org/science/article/pii/S1359734525000795","RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}

引用次数: 0

摘要

由于海水资源丰富，海水电解制氢技术受到了世界各国的广泛关注。在此，我们提出了以α/β-MnO2纳米线为核心，无定形Ru为外壳的核壳Ru@MnO2纳米线，其中Ru@α- mno2纳米线具有较低的过电位和较好的稳定性。更重要的是，它们可以作为双功能催化剂稳定运行250 h以上，并且在太阳能驱动下保持优异的催化性能。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

Ru@MnO2 core@shell nanowires as a bifunctional electrocatalyst for efficient solar-driven seawater splitting†

查看原文本刊更多论文

Ru@MnO2 core@shell nanowires as a bifunctional electrocatalyst for efficient solar-driven seawater splitting†

Seawater electrolysis technology for hydrogen production has attracted worldwide attention due to the abundant seawater resources. Herein, we proposed core–shell Ru@MnO₂ nanowires (NWs) with α/β-MnO₂ NWs as the core and amorphous Ru as the shell, in which the Ru@α-MnO₂ NWs exhibited lower overpotential and better stability. More importantly, they can operate stably as a bifunctional catalyst for more than 250 h and maintain excellent catalytic performance when driven by solar energy.

求助全文

通过发布文献求助，成功后即可免费获取论文全文。去求助

来源期刊

Chemical Communications 化学-化学综合

CiteScore

8.60

自引率

4.10%

发文量

2705

审稿时长

1.4 months

期刊介绍： ChemComm (Chemical Communications) is renowned as the fastest publisher of articles providing information on new avenues of research, drawn from all the world''s major areas of chemical research.