Yuanrui Zhu, Gregory Ross, Olga Khaliukova, Selina A Roman-White, Fiji C George, Dorit Hammerling, Arvind P Ravikumar
{"title":"美国天然气液化终端温室气体排放的多尺度测量。","authors":"Yuanrui Zhu, Gregory Ross, Olga Khaliukova, Selina A Roman-White, Fiji C George, Dorit Hammerling, Arvind P Ravikumar","doi":"10.1021/acs.estlett.4c00713","DOIUrl":null,"url":null,"abstract":"<p><p>Addressing methane emissions across the liquefied natural gas (LNG) supply chain is key to reducing climate impacts of LNG. Actions to address methane emissions have emphasized the importance of the use of measurement-informed emissions inventories given the systematic underestimation in official greenhouse gas (GHG) emission inventories. Despite significant progress in field measurements of GHG emissions across the natural gas supply chain, no detailed measurements at US liquefaction terminals are publicly available. In this work, we conduct multiscale, periodic measurements of methane and carbon dioxide emissions at two US LNG terminals over a 16-month campaign. We find that methane emission intensity varied from 0.007% to 0.045%, normalized to methane in LNG production. Carbon dioxide emissions accounted for over 95% of total GHG emissions using 100-year global warming potential (GWP) for methane. Thus, contrary to observations across other natural gas supply chain segments, we find that reported GHG emissions intensity closely matches measurement informed GHG emissions intensity of 0.24-0.27 kg CO<sub>2</sub>e/kg CH<sub>4</sub>. In the context of developing LNG supply chain emissions intensity, we conclude that the use of the Greenhouse Gas Reporting Program emissions intensity provides reasonably accurate estimates of total GHG emissions at LNG terminals.</p>","PeriodicalId":37,"journal":{"name":"Environmental Science & Technology Letters Environ.","volume":"12 1","pages":"44-50"},"PeriodicalIF":8.9000,"publicationDate":"2024-12-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11736837/pdf/","citationCount":"0","resultStr":"{\"title\":\"Multiscale Measurements of Greenhouse Gas Emissions at U.S. Natural Gas Liquefaction Terminals.\",\"authors\":\"Yuanrui Zhu, Gregory Ross, Olga Khaliukova, Selina A Roman-White, Fiji C George, Dorit Hammerling, Arvind P Ravikumar\",\"doi\":\"10.1021/acs.estlett.4c00713\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>Addressing methane emissions across the liquefied natural gas (LNG) supply chain is key to reducing climate impacts of LNG. Actions to address methane emissions have emphasized the importance of the use of measurement-informed emissions inventories given the systematic underestimation in official greenhouse gas (GHG) emission inventories. Despite significant progress in field measurements of GHG emissions across the natural gas supply chain, no detailed measurements at US liquefaction terminals are publicly available. In this work, we conduct multiscale, periodic measurements of methane and carbon dioxide emissions at two US LNG terminals over a 16-month campaign. We find that methane emission intensity varied from 0.007% to 0.045%, normalized to methane in LNG production. Carbon dioxide emissions accounted for over 95% of total GHG emissions using 100-year global warming potential (GWP) for methane. Thus, contrary to observations across other natural gas supply chain segments, we find that reported GHG emissions intensity closely matches measurement informed GHG emissions intensity of 0.24-0.27 kg CO<sub>2</sub>e/kg CH<sub>4</sub>. In the context of developing LNG supply chain emissions intensity, we conclude that the use of the Greenhouse Gas Reporting Program emissions intensity provides reasonably accurate estimates of total GHG emissions at LNG terminals.</p>\",\"PeriodicalId\":37,\"journal\":{\"name\":\"Environmental Science & Technology Letters Environ.\",\"volume\":\"12 1\",\"pages\":\"44-50\"},\"PeriodicalIF\":8.9000,\"publicationDate\":\"2024-12-16\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11736837/pdf/\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Environmental Science & Technology Letters Environ.\",\"FirstCategoryId\":\"1\",\"ListUrlMain\":\"https://doi.org/10.1021/acs.estlett.4c00713\",\"RegionNum\":2,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"2025/1/14 0:00:00\",\"PubModel\":\"eCollection\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, ENVIRONMENTAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Environmental Science & Technology Letters Environ.","FirstCategoryId":"1","ListUrlMain":"https://doi.org/10.1021/acs.estlett.4c00713","RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2025/1/14 0:00:00","PubModel":"eCollection","JCR":"Q1","JCRName":"ENGINEERING, ENVIRONMENTAL","Score":null,"Total":0}
引用次数: 0
摘要
解决整个液化天然气(LNG)供应链的甲烷排放问题是减少液化天然气对气候影响的关键。鉴于官方温室气体(GHG)排放清单存在系统性低估,解决甲烷排放问题的行动强调了使用基于测量的排放清单的重要性。尽管在天然气供应链的温室气体排放现场测量方面取得了重大进展,但美国液化终端的详细测量数据尚未公开。在这项工作中,我们在为期16个月的活动中对两个美国液化天然气接收站的甲烷和二氧化碳排放量进行了多尺度、定期测量。我们发现甲烷排放强度在0.007% ~ 0.045%之间变化,归一化到LNG生产中的甲烷。使用100年全球变暖潜能值(GWP)计算甲烷,二氧化碳排放量占温室气体总排放量的95%以上。因此,与其他天然气供应链环节的观察结果相反,我们发现报告的温室气体排放强度与测量结果的温室气体排放强度(0.24-0.27 kg CO2e/kg CH4)非常吻合。在开发LNG供应链排放强度的背景下,我们得出结论,使用温室气体报告计划排放强度可以合理准确地估计LNG终端的温室气体排放总量。
Multiscale Measurements of Greenhouse Gas Emissions at U.S. Natural Gas Liquefaction Terminals.
Addressing methane emissions across the liquefied natural gas (LNG) supply chain is key to reducing climate impacts of LNG. Actions to address methane emissions have emphasized the importance of the use of measurement-informed emissions inventories given the systematic underestimation in official greenhouse gas (GHG) emission inventories. Despite significant progress in field measurements of GHG emissions across the natural gas supply chain, no detailed measurements at US liquefaction terminals are publicly available. In this work, we conduct multiscale, periodic measurements of methane and carbon dioxide emissions at two US LNG terminals over a 16-month campaign. We find that methane emission intensity varied from 0.007% to 0.045%, normalized to methane in LNG production. Carbon dioxide emissions accounted for over 95% of total GHG emissions using 100-year global warming potential (GWP) for methane. Thus, contrary to observations across other natural gas supply chain segments, we find that reported GHG emissions intensity closely matches measurement informed GHG emissions intensity of 0.24-0.27 kg CO2e/kg CH4. In the context of developing LNG supply chain emissions intensity, we conclude that the use of the Greenhouse Gas Reporting Program emissions intensity provides reasonably accurate estimates of total GHG emissions at LNG terminals.
期刊介绍:
Environmental Science & Technology Letters serves as an international forum for brief communications on experimental or theoretical results of exceptional timeliness in all aspects of environmental science, both pure and applied. Published as soon as accepted, these communications are summarized in monthly issues. Additionally, the journal features short reviews on emerging topics in environmental science and technology.