{"title":"更有效的乙醇电合成催化剂和微环境设计","authors":"","doi":"10.1038/s44160-024-00663-w","DOIUrl":null,"url":null,"abstract":"Simultaneously achieving high energy and carbon efficiency in ethanol electrosynthesis is challenging. Now, an interfacial cation matrix (ICM) is developed that modifies the catalyst microenvironment to increase these performance metrics towards multicarbon products in the acidic CO2 reduction reaction. Furthermore, combining a tailored Cu–Ag catalyst with the ICM facilitates selective ethanol electrosynthesis.","PeriodicalId":74251,"journal":{"name":"Nature synthesis","volume":"4 1","pages":"13-14"},"PeriodicalIF":0.0000,"publicationDate":"2024-10-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Catalyst and microenvironment design for more efficient ethanol electrosynthesis\",\"authors\":\"\",\"doi\":\"10.1038/s44160-024-00663-w\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Simultaneously achieving high energy and carbon efficiency in ethanol electrosynthesis is challenging. Now, an interfacial cation matrix (ICM) is developed that modifies the catalyst microenvironment to increase these performance metrics towards multicarbon products in the acidic CO2 reduction reaction. Furthermore, combining a tailored Cu–Ag catalyst with the ICM facilitates selective ethanol electrosynthesis.\",\"PeriodicalId\":74251,\"journal\":{\"name\":\"Nature synthesis\",\"volume\":\"4 1\",\"pages\":\"13-14\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2024-10-04\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nature synthesis\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://www.nature.com/articles/s44160-024-00663-w\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"0\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nature synthesis","FirstCategoryId":"1085","ListUrlMain":"https://www.nature.com/articles/s44160-024-00663-w","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"0","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Catalyst and microenvironment design for more efficient ethanol electrosynthesis
Simultaneously achieving high energy and carbon efficiency in ethanol electrosynthesis is challenging. Now, an interfacial cation matrix (ICM) is developed that modifies the catalyst microenvironment to increase these performance metrics towards multicarbon products in the acidic CO2 reduction reaction. Furthermore, combining a tailored Cu–Ag catalyst with the ICM facilitates selective ethanol electrosynthesis.