{"title":"通过调整共价有机框架中的腙键密度来增强光催化过氧化氢的生成","authors":"Avanti Chakraborty, Akhtar Alam, Uttam Pal, Archisman Sinha, Subhadip Das, Tanusri Saha-Dasgupta, Pradip Pachfule","doi":"10.1038/s41467-025-55894-y","DOIUrl":null,"url":null,"abstract":"<p>The conversion of solar energy into chemical energy or high-value chemicals has attracted considerable research interest in the context of the global energy crisis. Hydrogen peroxide (H<sub>2</sub>O<sub>2</sub>) is a versatile and powerful oxidizing agent widely used in chemical synthesis and medical disinfection. H<sub>2</sub>O<sub>2</sub> also serves as a clean energy source in fuel cells, generating electricity with zero-carbon emissions. Recently, the sustainable production of H<sub>2</sub>O<sub>2</sub> from water and oxygen using covalent organic frameworks (COFs) as photocatalysts has attracted considerable attention; however, systematic studies highlighting the role of linkages in determining photocatalytic performance are scarce. Under these circumstances, herein, we demonstrate that varying the imine and hydrazone linkages within the framework significantly influences photocatalytic H<sub>2</sub>O<sub>2</sub> production. COFs with high-density hydrazone linkages, providing optimal docking sites for water and oxygen, enhance H<sub>2</sub>O<sub>2</sub> generation activity (1588 μmol g<sup>−1</sup> h<sup>−1</sup> from pure water in the air), leading to highly efficient solar-to-chemical energy conversion.</p>","PeriodicalId":19066,"journal":{"name":"Nature Communications","volume":"6 1","pages":""},"PeriodicalIF":15.7000,"publicationDate":"2025-01-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Enhancing photocatalytic hydrogen peroxide generation by tuning hydrazone linkage density in covalent organic frameworks\",\"authors\":\"Avanti Chakraborty, Akhtar Alam, Uttam Pal, Archisman Sinha, Subhadip Das, Tanusri Saha-Dasgupta, Pradip Pachfule\",\"doi\":\"10.1038/s41467-025-55894-y\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>The conversion of solar energy into chemical energy or high-value chemicals has attracted considerable research interest in the context of the global energy crisis. Hydrogen peroxide (H<sub>2</sub>O<sub>2</sub>) is a versatile and powerful oxidizing agent widely used in chemical synthesis and medical disinfection. H<sub>2</sub>O<sub>2</sub> also serves as a clean energy source in fuel cells, generating electricity with zero-carbon emissions. Recently, the sustainable production of H<sub>2</sub>O<sub>2</sub> from water and oxygen using covalent organic frameworks (COFs) as photocatalysts has attracted considerable attention; however, systematic studies highlighting the role of linkages in determining photocatalytic performance are scarce. Under these circumstances, herein, we demonstrate that varying the imine and hydrazone linkages within the framework significantly influences photocatalytic H<sub>2</sub>O<sub>2</sub> production. COFs with high-density hydrazone linkages, providing optimal docking sites for water and oxygen, enhance H<sub>2</sub>O<sub>2</sub> generation activity (1588 μmol g<sup>−1</sup> h<sup>−1</sup> from pure water in the air), leading to highly efficient solar-to-chemical energy conversion.</p>\",\"PeriodicalId\":19066,\"journal\":{\"name\":\"Nature Communications\",\"volume\":\"6 1\",\"pages\":\"\"},\"PeriodicalIF\":15.7000,\"publicationDate\":\"2025-01-08\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nature Communications\",\"FirstCategoryId\":\"103\",\"ListUrlMain\":\"https://doi.org/10.1038/s41467-025-55894-y\",\"RegionNum\":1,\"RegionCategory\":\"综合性期刊\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MULTIDISCIPLINARY SCIENCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nature Communications","FirstCategoryId":"103","ListUrlMain":"https://doi.org/10.1038/s41467-025-55894-y","RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MULTIDISCIPLINARY SCIENCES","Score":null,"Total":0}
Enhancing photocatalytic hydrogen peroxide generation by tuning hydrazone linkage density in covalent organic frameworks
The conversion of solar energy into chemical energy or high-value chemicals has attracted considerable research interest in the context of the global energy crisis. Hydrogen peroxide (H2O2) is a versatile and powerful oxidizing agent widely used in chemical synthesis and medical disinfection. H2O2 also serves as a clean energy source in fuel cells, generating electricity with zero-carbon emissions. Recently, the sustainable production of H2O2 from water and oxygen using covalent organic frameworks (COFs) as photocatalysts has attracted considerable attention; however, systematic studies highlighting the role of linkages in determining photocatalytic performance are scarce. Under these circumstances, herein, we demonstrate that varying the imine and hydrazone linkages within the framework significantly influences photocatalytic H2O2 production. COFs with high-density hydrazone linkages, providing optimal docking sites for water and oxygen, enhance H2O2 generation activity (1588 μmol g−1 h−1 from pure water in the air), leading to highly efficient solar-to-chemical energy conversion.
期刊介绍:
Nature Communications, an open-access journal, publishes high-quality research spanning all areas of the natural sciences. Papers featured in the journal showcase significant advances relevant to specialists in each respective field. With a 2-year impact factor of 16.6 (2022) and a median time of 8 days from submission to the first editorial decision, Nature Communications is committed to rapid dissemination of research findings. As a multidisciplinary journal, it welcomes contributions from biological, health, physical, chemical, Earth, social, mathematical, applied, and engineering sciences, aiming to highlight important breakthroughs within each domain.