通过调整共价有机框架中的腙键密度来增强光催化过氧化氢的生成

IF 15.7 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES
Avanti Chakraborty, Akhtar Alam, Uttam Pal, Archisman Sinha, Subhadip Das, Tanusri Saha-Dasgupta, Pradip Pachfule
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引用次数: 0

摘要

在全球能源危机的背景下,将太阳能转化为化学能或高价值化学品引起了相当大的研究兴趣。过氧化氢(H2O2)是一种用途广泛的强氧化剂,广泛用于化学合成和医疗消毒。H2O2在燃料电池中也是一种清洁能源,可以产生零碳排放的电力。近年来,利用共价有机框架(COFs)作为光催化剂从水和氧中可持续生产H2O2引起了人们的广泛关注;然而,强调键在决定光催化性能中的作用的系统研究很少。在这种情况下,我们证明了在框架内改变亚胺和腙键会显著影响光催化H2O2的产生。COFs具有高密度的腙键,为水和氧提供了最佳的对接位置,提高了H2O2的生成活性(空气中纯水产生1588 μmol g−1 h−1),从而实现了高效的太阳能-化学能转换。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Enhancing photocatalytic hydrogen peroxide generation by tuning hydrazone linkage density in covalent organic frameworks

Enhancing photocatalytic hydrogen peroxide generation by tuning hydrazone linkage density in covalent organic frameworks

The conversion of solar energy into chemical energy or high-value chemicals has attracted considerable research interest in the context of the global energy crisis. Hydrogen peroxide (H2O2) is a versatile and powerful oxidizing agent widely used in chemical synthesis and medical disinfection. H2O2 also serves as a clean energy source in fuel cells, generating electricity with zero-carbon emissions. Recently, the sustainable production of H2O2 from water and oxygen using covalent organic frameworks (COFs) as photocatalysts has attracted considerable attention; however, systematic studies highlighting the role of linkages in determining photocatalytic performance are scarce. Under these circumstances, herein, we demonstrate that varying the imine and hydrazone linkages within the framework significantly influences photocatalytic H2O2 production. COFs with high-density hydrazone linkages, providing optimal docking sites for water and oxygen, enhance H2O2 generation activity (1588 μmol g−1 h−1 from pure water in the air), leading to highly efficient solar-to-chemical energy conversion.

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来源期刊
Nature Communications
Nature Communications Biological Science Disciplines-
CiteScore
24.90
自引率
2.40%
发文量
6928
审稿时长
3.7 months
期刊介绍: Nature Communications, an open-access journal, publishes high-quality research spanning all areas of the natural sciences. Papers featured in the journal showcase significant advances relevant to specialists in each respective field. With a 2-year impact factor of 16.6 (2022) and a median time of 8 days from submission to the first editorial decision, Nature Communications is committed to rapid dissemination of research findings. As a multidisciplinary journal, it welcomes contributions from biological, health, physical, chemical, Earth, social, mathematical, applied, and engineering sciences, aiming to highlight important breakthroughs within each domain.
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