蛤蚌烯基可控自组装结晶三维超分子聚合物及其在光热转化中的应用

IF 8.2 2区材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY

ACS Applied Materials & Interfaces Pub Date : 2025-01-03 DOI:10.1021/acsami.4c18272

Bingbing Shi, Lijuan Qi, Jingxiong Jiang, Wentao Hu, Tai-Bao Wei, Wen-Juan Qu, Qi Lin

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引用次数: 0

摘要

明确定义的三维超分子聚合物的发展提出了重大挑战，特别是在实现晶体状态结构方面。本研究通过在固体状态下自组装蛤烯（CLP）和萘二亚胺衍生物（NDIOH）来构建结晶三维超分子聚合物来解决这一挑战。从一维线性超分子聚合物到二维超分子聚合物，再到结晶的三维超分子聚合物。制备的结晶三维超分子聚合物具有良好的光热转化效果。这项工作促进了对晶体状态下功能三维超分子聚合物的理解和设计。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

A Crystalline 3D Supramolecular Polymer Constructed by Clamparene-Based Controllable Self-Assembly and Its Application in Photothermal Conversion

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A Crystalline 3D Supramolecular Polymer Constructed by Clamparene-Based Controllable Self-Assembly and Its Application in Photothermal Conversion

The development of well-defined three-dimensional supramolecular polymers presents significant challenges, particularly in achieving crystalline state structures. This study addresses this challenge by presenting the construction of a crystalline three-dimensional supramolecular polymer through the self-assembly of clamparene (CLP) and a naphthalene diimide derivative (NDIOH) in the solid state. The hierarchical self-assembly progresses from one-dimensional linear supramolecular polymers to two-dimensional supramolecular polymers and ultimately to a crystalline three-dimensional supramolecular polymer. Moreover, the prepared crystalline three-dimensional supramolecular polymer demonstrates effective photothermal conversion. This work advances the understanding and design of functional three-dimensional supramolecular polymers in the crystalline state.

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来源期刊

ACS Applied Materials & Interfaces 工程技术-材料科学：综合

CiteScore

16.00

自引率

6.30%

发文量

4978

审稿时长

1.8 months

期刊介绍： ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.