{"title":"基于NiSe的可调谐多孤子态超快光纤激光器及矢量双波长孤子的产生。","authors":"Long-Fei Ren, Zhi-Zeng Si, Jing Liu, Hao Sun, Chao-Qing Dai, Huai-Jun Sun, Yue-Yue Wang","doi":"10.1021/acsami.4c18533","DOIUrl":null,"url":null,"abstract":"<p><p>As a member of the chalcogenide family, NiSe exhibits a direct bandgap of 1.74 eV, making it a promising candidate for nonlinear optical devices. However, its potential in the near-infrared region of the telecommunication band has not been fully explored. In this study, a well-coupled saturable absorber (SA) device is fabricated for the first time using NiSe nanosheets, and it is applied to an ultrafast fiber laser, achieving an ultrashort pulse laser output with an optical conversion efficiency of 13.9%. The laser based on NiSe SA achieves tunable multisoliton mode locking, including conventional solitons, bound-state solitons, dual-wavelength solitons, and second to fourth harmonic solitons, over a wavelength range of 1528.5-1556 nm by adjusting the resonator's polarization state through the polarization controller and controlling the pump power. Numerical simulations and soliton dynamic analysis in the study of NiSe SA reveal the intricate details and behaviors of ultrafast soliton pulse locking. The results indicate that the well-coupled NiSe SA, characterized by a modulation depth of 36.73%, a saturation intensity of 0.287 MW/cm<sup>2</sup>, and excellent spectral broadband absorption properties, can enhance intracavity nonlinear effects and enable the realization of stable and tunable multisoliton mode-locked pulses. Additionally, soliton collisions with group velocity differences are investigated under stable dual-wavelength soliton output, especially vector dual-wavelength soliton. This demonstrates the excellent application potential of NiSe SA in fields such as ultrafast optical communications and information encryption.</p>","PeriodicalId":5,"journal":{"name":"ACS Applied Materials & Interfaces","volume":" ","pages":"3785-3795"},"PeriodicalIF":8.2000,"publicationDate":"2025-01-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Tunable Multisoliton State Ultrafast Fiber Laser Based on NiSe and Generation of Vector Dual-Wavelength Solitons.\",\"authors\":\"Long-Fei Ren, Zhi-Zeng Si, Jing Liu, Hao Sun, Chao-Qing Dai, Huai-Jun Sun, Yue-Yue Wang\",\"doi\":\"10.1021/acsami.4c18533\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>As a member of the chalcogenide family, NiSe exhibits a direct bandgap of 1.74 eV, making it a promising candidate for nonlinear optical devices. However, its potential in the near-infrared region of the telecommunication band has not been fully explored. In this study, a well-coupled saturable absorber (SA) device is fabricated for the first time using NiSe nanosheets, and it is applied to an ultrafast fiber laser, achieving an ultrashort pulse laser output with an optical conversion efficiency of 13.9%. The laser based on NiSe SA achieves tunable multisoliton mode locking, including conventional solitons, bound-state solitons, dual-wavelength solitons, and second to fourth harmonic solitons, over a wavelength range of 1528.5-1556 nm by adjusting the resonator's polarization state through the polarization controller and controlling the pump power. Numerical simulations and soliton dynamic analysis in the study of NiSe SA reveal the intricate details and behaviors of ultrafast soliton pulse locking. The results indicate that the well-coupled NiSe SA, characterized by a modulation depth of 36.73%, a saturation intensity of 0.287 MW/cm<sup>2</sup>, and excellent spectral broadband absorption properties, can enhance intracavity nonlinear effects and enable the realization of stable and tunable multisoliton mode-locked pulses. Additionally, soliton collisions with group velocity differences are investigated under stable dual-wavelength soliton output, especially vector dual-wavelength soliton. This demonstrates the excellent application potential of NiSe SA in fields such as ultrafast optical communications and information encryption.</p>\",\"PeriodicalId\":5,\"journal\":{\"name\":\"ACS Applied Materials & Interfaces\",\"volume\":\" \",\"pages\":\"3785-3795\"},\"PeriodicalIF\":8.2000,\"publicationDate\":\"2025-01-15\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Applied Materials & Interfaces\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1021/acsami.4c18533\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"2025/1/1 0:00:00\",\"PubModel\":\"Epub\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Materials & Interfaces","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acsami.4c18533","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2025/1/1 0:00:00","PubModel":"Epub","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Tunable Multisoliton State Ultrafast Fiber Laser Based on NiSe and Generation of Vector Dual-Wavelength Solitons.
As a member of the chalcogenide family, NiSe exhibits a direct bandgap of 1.74 eV, making it a promising candidate for nonlinear optical devices. However, its potential in the near-infrared region of the telecommunication band has not been fully explored. In this study, a well-coupled saturable absorber (SA) device is fabricated for the first time using NiSe nanosheets, and it is applied to an ultrafast fiber laser, achieving an ultrashort pulse laser output with an optical conversion efficiency of 13.9%. The laser based on NiSe SA achieves tunable multisoliton mode locking, including conventional solitons, bound-state solitons, dual-wavelength solitons, and second to fourth harmonic solitons, over a wavelength range of 1528.5-1556 nm by adjusting the resonator's polarization state through the polarization controller and controlling the pump power. Numerical simulations and soliton dynamic analysis in the study of NiSe SA reveal the intricate details and behaviors of ultrafast soliton pulse locking. The results indicate that the well-coupled NiSe SA, characterized by a modulation depth of 36.73%, a saturation intensity of 0.287 MW/cm2, and excellent spectral broadband absorption properties, can enhance intracavity nonlinear effects and enable the realization of stable and tunable multisoliton mode-locked pulses. Additionally, soliton collisions with group velocity differences are investigated under stable dual-wavelength soliton output, especially vector dual-wavelength soliton. This demonstrates the excellent application potential of NiSe SA in fields such as ultrafast optical communications and information encryption.
期刊介绍:
ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.