{"title":"基于Bi2Se3/AlInAsSb异质结的自供电超宽光电探测器的双极调制用于波长敏感成像和加密光通信","authors":"Yajie Han, Shujie Jiao, Xiangyu Zhang, Ping Rong, Yue Zhao, Dongwei Jiang, Wen He, Dongbo Wang, Shiyong Gao, Jinzhong Wang","doi":"10.1002/adma.202416935","DOIUrl":null,"url":null,"abstract":"<p>Broadband photodetectors (PDs) have garnered significant attention due to their ability to detect optical signals across a wide wavelength range, with applications spanning military reconnaissance, environmental monitoring, and medical imaging. However, existing broadband detectors face several practical challenges, including limited detection range, uneven photoresponse, and difficult to distinguish multispectral signals. To address these limitations, this study presents a self-powered ultra-wide PD based on the Bi<sub>2</sub>Se<sub>3</sub>/AlInAsSb heterojunction. The device can detect signals across a wide wavelength range from 250 nm to 1900 nm, exhibiting outstanding optoelectronic performance with a maximum responsivity of 0.5 A W<sup>−1</sup>, a detectivity of 4.2 × 10<sup>12</sup> Jones, a switching ratio of 1.1 × 10<sup>4</sup>, and an external quantum efficiency of 71.4%. Furthermore, the detector achieves a detectivity greater than 10<sup>10</sup> Jones across the entire broadband range, significantly improving photoresponse uniformity. Notably, due to the differential band alignment of the two materials across spectral ranges, this detector exhibits a photocurrent polarity reversal in the 650–680 nm range. Leveraging its broadband and bipolar characteristics, this PD successfully enables secure information encryption in communication systems. This study significantly advances broadband PD technology, enhancing its practical uses and introducing innovative solutions for secure communications, thus strengthening communication security and confidentiality.</p>","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":"37 7","pages":""},"PeriodicalIF":26.8000,"publicationDate":"2024-12-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Bipolar Modulation in a Self-Powered Ultra-Wide Photodetector Based on Bi2Se3/AlInAsSb Heterojunction for Wavelength-Sensitive Imaging and Encrypted Optical Communication\",\"authors\":\"Yajie Han, Shujie Jiao, Xiangyu Zhang, Ping Rong, Yue Zhao, Dongwei Jiang, Wen He, Dongbo Wang, Shiyong Gao, Jinzhong Wang\",\"doi\":\"10.1002/adma.202416935\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>Broadband photodetectors (PDs) have garnered significant attention due to their ability to detect optical signals across a wide wavelength range, with applications spanning military reconnaissance, environmental monitoring, and medical imaging. However, existing broadband detectors face several practical challenges, including limited detection range, uneven photoresponse, and difficult to distinguish multispectral signals. To address these limitations, this study presents a self-powered ultra-wide PD based on the Bi<sub>2</sub>Se<sub>3</sub>/AlInAsSb heterojunction. The device can detect signals across a wide wavelength range from 250 nm to 1900 nm, exhibiting outstanding optoelectronic performance with a maximum responsivity of 0.5 A W<sup>−1</sup>, a detectivity of 4.2 × 10<sup>12</sup> Jones, a switching ratio of 1.1 × 10<sup>4</sup>, and an external quantum efficiency of 71.4%. Furthermore, the detector achieves a detectivity greater than 10<sup>10</sup> Jones across the entire broadband range, significantly improving photoresponse uniformity. Notably, due to the differential band alignment of the two materials across spectral ranges, this detector exhibits a photocurrent polarity reversal in the 650–680 nm range. Leveraging its broadband and bipolar characteristics, this PD successfully enables secure information encryption in communication systems. This study significantly advances broadband PD technology, enhancing its practical uses and introducing innovative solutions for secure communications, thus strengthening communication security and confidentiality.</p>\",\"PeriodicalId\":114,\"journal\":{\"name\":\"Advanced Materials\",\"volume\":\"37 7\",\"pages\":\"\"},\"PeriodicalIF\":26.8000,\"publicationDate\":\"2024-12-25\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Advanced Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://onlinelibrary.wiley.com/doi/10.1002/adma.202416935\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Materials","FirstCategoryId":"88","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/adma.202416935","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Bipolar Modulation in a Self-Powered Ultra-Wide Photodetector Based on Bi2Se3/AlInAsSb Heterojunction for Wavelength-Sensitive Imaging and Encrypted Optical Communication
Broadband photodetectors (PDs) have garnered significant attention due to their ability to detect optical signals across a wide wavelength range, with applications spanning military reconnaissance, environmental monitoring, and medical imaging. However, existing broadband detectors face several practical challenges, including limited detection range, uneven photoresponse, and difficult to distinguish multispectral signals. To address these limitations, this study presents a self-powered ultra-wide PD based on the Bi2Se3/AlInAsSb heterojunction. The device can detect signals across a wide wavelength range from 250 nm to 1900 nm, exhibiting outstanding optoelectronic performance with a maximum responsivity of 0.5 A W−1, a detectivity of 4.2 × 1012 Jones, a switching ratio of 1.1 × 104, and an external quantum efficiency of 71.4%. Furthermore, the detector achieves a detectivity greater than 1010 Jones across the entire broadband range, significantly improving photoresponse uniformity. Notably, due to the differential band alignment of the two materials across spectral ranges, this detector exhibits a photocurrent polarity reversal in the 650–680 nm range. Leveraging its broadband and bipolar characteristics, this PD successfully enables secure information encryption in communication systems. This study significantly advances broadband PD technology, enhancing its practical uses and introducing innovative solutions for secure communications, thus strengthening communication security and confidentiality.
期刊介绍:
Advanced Materials, one of the world's most prestigious journals and the foundation of the Advanced portfolio, is the home of choice for best-in-class materials science for more than 30 years. Following this fast-growing and interdisciplinary field, we are considering and publishing the most important discoveries on any and all materials from materials scientists, chemists, physicists, engineers as well as health and life scientists and bringing you the latest results and trends in modern materials-related research every week.