利用滑动电弧提高甲烷等离子重整的能耗

IF 9.9 1区 工程技术 Q1 ENERGY & FUELS
Haochuan He, Changhua Wang, He Ma, Hancheng Zhu, Xintong Zhang
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引用次数: 0

摘要

随着对可持续能源需求的增加,天然气制氢引起了人们的极大关注。利用清洁电力对天然气进行等离子体重整,有望为制氢提供一条低碳途径。然而,等离子体重整的高能量消耗仍然是一个主要的挑战。这项工作利用脉冲滑动电弧来维持脉冲间隔内的等离子体放电。电信号分析表明,在脉冲间隔时间内,电弧仅以峰值电压的1%就能继续滑动,等离子体的自维持时间长达50 μs。增强互补金属氧化物半导体(ICMOS)传感器捕获的图像和流体模拟结果表明,等离子体电弧在自持阶段保持甲烷解离活性。制氢的最小比能耗为127 kJ/mol,仅为当前主流等离子体甲烷重整能耗的20%。滑行电弧等离子体技术为绿色低能耗制氢提供了一种高效的无催化剂方法。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Improving energy consumption in plasma reforming of methane through gliding arc
As the demand for sustainable energy increases, hydrogen production from natural gas has garnered significant attention. Plasma reforming of natural gas using clean electricity promises low-carbon pathway for hydrogen production. However, the high energy consumption of plasma reforming remains a major challenge. This work utilizes pulsed gliding arc to maintain plasma discharge during pulse intervals. Electrical signal analysis indicates that the arcs can continue gliding with only 1 % of the peak voltage during pulse intervals, with the plasma self-sustaining for up to 50 μs. Images captured by intensified complementary metal–oxide–semiconductor (ICMOS) sensors and fluid simulation results demonstrate that the plasma arc retains methane dissociation activity during the self-sustaining phase. The minimum specific energy consumption for hydrogen production is 127 kJ/mol, which is only 20 % of the energy consumption of current mainstream methane reforming by plasma processes. The gliding arc plasma technique offers an efficient catalyst-free approach for green and low-energy hydrogen production.
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来源期刊
Energy Conversion and Management
Energy Conversion and Management 工程技术-力学
CiteScore
19.00
自引率
11.50%
发文量
1304
审稿时长
17 days
期刊介绍: The journal Energy Conversion and Management provides a forum for publishing original contributions and comprehensive technical review articles of interdisciplinary and original research on all important energy topics. The topics considered include energy generation, utilization, conversion, storage, transmission, conservation, management and sustainability. These topics typically involve various types of energy such as mechanical, thermal, nuclear, chemical, electromagnetic, magnetic and electric. These energy types cover all known energy resources, including renewable resources (e.g., solar, bio, hydro, wind, geothermal and ocean energy), fossil fuels and nuclear resources.
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