基于氢氧化钙板碳化的冷却塔直接捕集系统的技术经济研究

IF 9.7 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL
Mohammad Hosseinpour, Bijan Hejazi, Yolanda A. Criado
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引用次数: 0

摘要

直接空气捕获技术(DAC)是缓解全球变暖的一项重要的负排放技术。DAC工艺的主要挑战之一是与大型空气接触器中的气流系统相关的高能量和经济成本。最近,人们对使用水合石灰从大气中捕获低浓度的二氧化碳(~ 450 ppm)越来越感兴趣,特别是在空气相对湿度较高的情况下。冷却塔通常用于各种工业装置来冷却工艺用水,为水合石灰基DAC系统提供了理想的环境,因为它们将大量的环境空气暴露在水中。本研究评估了将垂直方向平行的Ca(OH)2平板整合到工业机械通风冷却塔上部的可行性,以同时执行水冷却和从通过的空气中捕获CO2的双重任务。非稳态缩芯模型(SCM)的结果表明,425座截面积20×20 m2的冷却塔可容纳5米长的Ca(OH)2垂直板,其孔隙率为0.55,厚度为2 cm,相邻板间距为2 cm,如果碳化板每年更换4次(周期为3个月),则可实现100万吨的年二氧化碳捕集率。通过使用一个放大的集中煅烧装置来再生回收的吸附剂,所提议的DAC过程的估计最终成本约为每吨二氧化碳捕获93.5至269美元,这使得所提议的系统在最先进的DAC技术中具有成本竞争力。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Techno-economic study of a direct air capture system based on the carbonation of Ca(OH)2 plates integrated into cooling towers

Techno-economic study of a direct air capture system based on the carbonation of Ca(OH)2 plates integrated into cooling towers
Direct Air Capture (DAC) is a crucial Negative Emissions Technology (NET) for mitigating global warming. One of the main challenges in DAC processes is the high energy and economic costs associated with airflow systems in large-scale air contactors. Recently, there has been a growing interest in using hydrate lime to capture low concentrations of CO2 (∼450 ppm) from the atmosphere, particularly at higher air relative humidity. Cooling towers, commonly used in various industrial units to cool process water, provide an ideal environment for hydrated lime-based DAC systems as they expose large flows of ambient air to water. This study assessed the feasibility of integrating vertically oriented parallel flat plates of Ca(OH)2 into the upper section of an industrial mechanical draft cooling tower to simultaneously perform the dual tasks of water cooling and CO2 capture from the passing air. Results of an unsteady-state Shrinking Core Model (SCM) showed that 425 cooling towers of 20×20 m2 cross-sectional area accommodating 5-meter long Ca(OH)2 vertical plates of porosity 0.55, thickness 2 cm, and distance between adjacent plates of 2 cm can achieve an annual CO2 capture rate of 1 million tons if the carbonated plates are replaced 4 times a year (3-month cycle duration). By utilizing a scaled-up centralized calcination unit for the regeneration of the recycled sorbent, the estimated final cost of the proposed DAC process is around $93.5 to $269 per ton of CO2 captured which makes the proposed system a cost-competitive alternative among the state-of-the-art DAC technologies.
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来源期刊
Journal of Cleaner Production
Journal of Cleaner Production 环境科学-工程:环境
CiteScore
20.40
自引率
9.00%
发文量
4720
审稿时长
111 days
期刊介绍: The Journal of Cleaner Production is an international, transdisciplinary journal that addresses and discusses theoretical and practical Cleaner Production, Environmental, and Sustainability issues. It aims to help societies become more sustainable by focusing on the concept of 'Cleaner Production', which aims at preventing waste production and increasing efficiencies in energy, water, resources, and human capital use. The journal serves as a platform for corporations, governments, education institutions, regions, and societies to engage in discussions and research related to Cleaner Production, environmental, and sustainability practices.
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