高效可见光驱动的 S-Scheme 石墨烯桥 MoS2/Co3O4 纳米杂化物对有害染料的光催化性能和抗菌活性。

IF 8.1 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES
Linjer Chen , Chiu-Wen Chen , Cheng-Di Dong
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引用次数: 0

摘要

采用水热法制备了一种新型石墨烯桥接MoS2/Co3O4 (MCG)纳米杂化材料。具有强界面相互作用的有价值的、经济的S-scheme体系是光催化效率和高效利用的迫切要求。虽然在电荷载流子桥方面取得了很大的进展,但由于电导率较低,设施电荷载流子桥的电荷转移能力还远远不够。在可见光下进行光催化抑菌实验,结果表明,与MoS2和Co3O4裸样品相比,制备的具有强界面偶联的MCG纳米杂化物在可见光下对亚甲基蓝(MB)和大肠杆菌的光降解性能优异。此外,MCG-4纳米杂化物具有较好的光催化MB性能,抗菌活性分别为99.5%和100%,分别是原始MoS2样品的2.76倍和8.32倍。PL测量和EIS分析也表明MCG-4纳米杂化材料具有较高的光诱导载流子分离效率。本研究为高潜力s型光催化剂及其在环境修复领域的应用提供了新的研究方向。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Highly efficient visible-light-driven S-scheme graphene bridged MoS2/Co3O4 nanohybrid for the photocatalytic performance of hazardous dye and antibacterial activity

Highly efficient visible-light-driven S-scheme graphene bridged MoS2/Co3O4 nanohybrid for the photocatalytic performance of hazardous dye and antibacterial activity
A novel graphene-bridged MoS2/Co3O4 (MCG) nanohybrid was well fabricated by a hydrothermal route. The purpose of valuable and economical S-scheme systems with vigorous interface interactions is pressing to photocatalytic efficiency and efficient utilization. While mighty progress has been created with respect to charge carrier bridges, the charge transferring ability of the facility charge carrier bridges is far from capable owing to lower electrical conductivity. The photocatalytic antibacterial tests were performed with visible light activity, and the results exhibited that the as-prepared MCG nanohybrid with powerful interfacial coupling presented excellent photodegradation performance in comparison with bare MoS2 and Co3O4 samples for the removal of methylene blue (MB) and E-coli with visible light irradiation. In addition, a better photocatalytic MB capability and antibacterial activity of 99.5 % and 100 % are approached through MCG-4 nanohybrid, which is 2.76 and 8.32 folds higher than that of the pristine MoS2 sample. The PL measurements and EIS analysis also illustrated that MCG-4 nanohybrid possesses a great separation efficiency of photoinduced charge carriers. This work provides a new objective for high-potential S-scheme photocatalysts and their utilization in the field of environmental remediation.
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来源期刊
Chemosphere
Chemosphere 环境科学-环境科学
CiteScore
15.80
自引率
8.00%
发文量
4975
审稿时长
3.4 months
期刊介绍: Chemosphere, being an international multidisciplinary journal, is dedicated to publishing original communications and review articles on chemicals in the environment. The scope covers a wide range of topics, including the identification, quantification, behavior, fate, toxicology, treatment, and remediation of chemicals in the bio-, hydro-, litho-, and atmosphere, ensuring the broad dissemination of research in this field.
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