甲烷氧化生成甲醛的甲烷营养催化

IF 42.8 1区化学 Q1 CHEMISTRY, PHYSICAL

Nature Catalysis Pub Date : 2024-12-20 DOI:10.1038/s41929-024-01252-y

引用次数: 0

摘要

众所周知，甲烷很难活化用于有用的化学反应。现在，我们开发出了一种由铁改性沸石和酶组成的串联催化剂系统，可在环境条件下使用过氧化氢作为氧化剂将甲烷部分氧化为甲醛。这种方法实现了高选择性和甲醛转化率。

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Methanotrophic catalysis for methane oxidation to formaldehyde

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Methanotrophic catalysis for methane oxidation to formaldehyde

Methane has been notoriously difficult to activate for useful chemistry. Now, a tandem catalyst system comprising an iron-modified zeolite and an enzyme is developed for the partial oxidation of methane to formaldehyde under ambient conditions using hydrogen peroxide as the oxidizing agent. This approach achieves high selectivity and conversion to formaldehyde.

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来源期刊

Nature Catalysis Chemical Engineering-Bioengineering

CiteScore

52.10

自引率

1.10%

发文量

140

期刊介绍： Nature Catalysis serves as a platform for researchers across chemistry and related fields, focusing on homogeneous catalysis, heterogeneous catalysis, and biocatalysts, encompassing both fundamental and applied studies. With a particular emphasis on advancing sustainable industries and processes, the journal provides comprehensive coverage of catalysis research, appealing to scientists, engineers, and researchers in academia and industry. Maintaining the high standards of the Nature brand, Nature Catalysis boasts a dedicated team of professional editors, rigorous peer-review processes, and swift publication times, ensuring editorial independence and quality. The journal publishes work spanning heterogeneous catalysis, homogeneous catalysis, and biocatalysis, covering areas such as catalytic synthesis, mechanisms, characterization, computational studies, nanoparticle catalysis, electrocatalysis, photocatalysis, environmental catalysis, asymmetric catalysis, and various forms of organocatalysis.