Bo Long, Qian Zhang, Lintong Zhang, Qi Liu, Qiongqiong Xing, Fangfang Qu, Liying Deng, Peng Yan, Liwei Wang, Meng An, Dapeng Ye, Zhanhui Yuan
{"title":"基于 CNT@PSS-AuNPs/rGO 层状薄膜的传感器用于便携式环丙沙星检测","authors":"Bo Long, Qian Zhang, Lintong Zhang, Qi Liu, Qiongqiong Xing, Fangfang Qu, Liying Deng, Peng Yan, Liwei Wang, Meng An, Dapeng Ye, Zhanhui Yuan","doi":"10.1007/s42114-024-01156-2","DOIUrl":null,"url":null,"abstract":"<div><p>Trace amounts of antibiotics in water can accumulate in the human body through the food chain, posing significant health risks. Therefore, there is an urgent need to develop simple and effective methods for detecting antibiotics in water. In this study, we prepared electrochemical aptamer sensors based on carbon nanotubes@polystyrene sulfonate-gold nanoparticles/reduced graphene oxide (CNT@PSS-AuNPs/rGO) layered thin films for real-time, on-site detection of ciprofloxacin (CIP) in aquaculture environments, utilizing a portable sensing detection device. The CNT@PSS-AuNPs/rGO layered film offers an excellent specific surface area, providing ample binding sites for the aptamer. The functionalized CNT@PSS-AuNPs enhance the dispersibility and conductivity of the substrate material and increase the surface area of the electrode when loaded with rGO. Under optimal experimental conditions, the developed sensor exhibits a dynamic range from 4 ng/mL to 1.0 × 10<sup>3</sup> ng/mL and a limit of detection of 4 ng/mL (S/N = 3), demonstrating satisfactory sensitivity. The sensor also shows good stability, with a relative standard deviation of less than 1% after 100 repeated measurements. Moreover, when combined with a portable detection platform, CIP levels in aqueous environments can be analyzed intelligently, rapidly, and timely. Our study aims to promote simple and effective detection strategies, potentially extending their practical applications.</p></div>","PeriodicalId":7220,"journal":{"name":"Advanced Composites and Hybrid Materials","volume":"8 1","pages":""},"PeriodicalIF":23.2000,"publicationDate":"2024-12-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Sensors based on CNT@PSS-AuNPs/rGO layered films for portable detection of ciprofloxacin\",\"authors\":\"Bo Long, Qian Zhang, Lintong Zhang, Qi Liu, Qiongqiong Xing, Fangfang Qu, Liying Deng, Peng Yan, Liwei Wang, Meng An, Dapeng Ye, Zhanhui Yuan\",\"doi\":\"10.1007/s42114-024-01156-2\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Trace amounts of antibiotics in water can accumulate in the human body through the food chain, posing significant health risks. Therefore, there is an urgent need to develop simple and effective methods for detecting antibiotics in water. In this study, we prepared electrochemical aptamer sensors based on carbon nanotubes@polystyrene sulfonate-gold nanoparticles/reduced graphene oxide (CNT@PSS-AuNPs/rGO) layered thin films for real-time, on-site detection of ciprofloxacin (CIP) in aquaculture environments, utilizing a portable sensing detection device. The CNT@PSS-AuNPs/rGO layered film offers an excellent specific surface area, providing ample binding sites for the aptamer. The functionalized CNT@PSS-AuNPs enhance the dispersibility and conductivity of the substrate material and increase the surface area of the electrode when loaded with rGO. Under optimal experimental conditions, the developed sensor exhibits a dynamic range from 4 ng/mL to 1.0 × 10<sup>3</sup> ng/mL and a limit of detection of 4 ng/mL (S/N = 3), demonstrating satisfactory sensitivity. The sensor also shows good stability, with a relative standard deviation of less than 1% after 100 repeated measurements. Moreover, when combined with a portable detection platform, CIP levels in aqueous environments can be analyzed intelligently, rapidly, and timely. 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Sensors based on CNT@PSS-AuNPs/rGO layered films for portable detection of ciprofloxacin
Trace amounts of antibiotics in water can accumulate in the human body through the food chain, posing significant health risks. Therefore, there is an urgent need to develop simple and effective methods for detecting antibiotics in water. In this study, we prepared electrochemical aptamer sensors based on carbon nanotubes@polystyrene sulfonate-gold nanoparticles/reduced graphene oxide (CNT@PSS-AuNPs/rGO) layered thin films for real-time, on-site detection of ciprofloxacin (CIP) in aquaculture environments, utilizing a portable sensing detection device. The CNT@PSS-AuNPs/rGO layered film offers an excellent specific surface area, providing ample binding sites for the aptamer. The functionalized CNT@PSS-AuNPs enhance the dispersibility and conductivity of the substrate material and increase the surface area of the electrode when loaded with rGO. Under optimal experimental conditions, the developed sensor exhibits a dynamic range from 4 ng/mL to 1.0 × 103 ng/mL and a limit of detection of 4 ng/mL (S/N = 3), demonstrating satisfactory sensitivity. The sensor also shows good stability, with a relative standard deviation of less than 1% after 100 repeated measurements. Moreover, when combined with a portable detection platform, CIP levels in aqueous environments can be analyzed intelligently, rapidly, and timely. Our study aims to promote simple and effective detection strategies, potentially extending their practical applications.
期刊介绍：
Advanced Composites and Hybrid Materials is a leading international journal that promotes interdisciplinary collaboration among materials scientists, engineers, chemists, biologists, and physicists working on composites, including nanocomposites. Our aim is to facilitate rapid scientific communication in this field.
The journal publishes high-quality research on various aspects of composite materials, including materials design, surface and interface science/engineering, manufacturing, structure control, property design, device fabrication, and other applications. We also welcome simulation and modeling studies that are relevant to composites. Additionally, papers focusing on the relationship between fillers and the matrix are of particular interest.
Our scope includes polymer, metal, and ceramic matrices, with a special emphasis on reviews and meta-analyses related to materials selection. We cover a wide range of topics, including transport properties, strategies for controlling interfaces and composition distribution, bottom-up assembly of nanocomposites, highly porous and high-density composites, electronic structure design, materials synergisms, and thermoelectric materials.
Advanced Composites and Hybrid Materials follows a rigorous single-blind peer-review process to ensure the quality and integrity of the published work.
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