从茶叶中绿色合成新型二氧化钛:去除亚甲基蓝,用于光催化应用

IF 2.8 3区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY
Medina Mehenaoui, Nadia Chekir, Djilali Tassalit, Melissa Brachemi, Nada Bensadok, Seif El Islam Lebouachera
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引用次数: 0

摘要

染料在自然界的普遍存在对水质和污染有重大影响。近年来,水污染受到了广泛关注,因为这一资源对人类的长期发展至关重要,而且由于工业化、污染和气候变化的影响,它的稀缺性也受到了广泛关注。在废水处理和利用光催化去除污染物方面已经进行了大量的研究,光催化使用了各种纳米颗粒。绿色合成是一种使用植物提取物的简单、无毒、经济、环保的方法,用于生产二氧化钛等纳米颗粒。本研究以绿茶提取物为原料,采用绿色工艺在400、500和600℃的温度下合成二氧化钛纳米颗粒(TiO₂NPs),以测试其在太阳照射下光催化去除水中亚甲基蓝染料的效率。与在400°C(51%)和600°C(54%)下合成的tio2 NPs相比,在500°C下合成的tio2 NPs随着时间的推移表现出良好的染料降解(76%)。在500℃下,用XRD、SEM-EDS、UV-Vis光谱、ATR-IR光谱和XRF对tio2纳米粒子进行了全面表征。结果证实了纳米颗粒的形成。二氧化钛为纳米级,XRD分析表明,二氧化钛的平均晶粒尺寸约为15.2。因此,本研究提出了一种具有高潜力的绿色溶液,这些纳米颗粒可以降解污染物MB。这些纳米颗粒可以通过光催化改进并用于降解其他污染物,以及有助于水净化。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Novel green synthesis of TiO2 from tea leaves: removal of methylene blue for photocatalytic application

Novel green synthesis of TiO2 from tea leaves: removal of methylene blue for photocatalytic application

The prevalence of dyes in nature has a significant impact on water quality and pollution. Water pollution has received much attention in recent years because of the importance of this resource to humankind’s long-term development, its scarcity as a result of industrialization, pollution, and the effects of climate change. Much research has been conducted on wastewater treatment and the removal of pollutants using photocatalysis, which employs various nanoparticles. Green synthesis, which uses plant extracts, is a simple, nontoxic, cost-effective, and environmentally friendly method for producing nanoparticles like titanium dioxide. This study uses green tea leaf extract to synthesize titanium dioxide nanoparticles (TiO₂ NPs) at temperatures of 400, 500, and 600°C using a green process, with the view of testing their efficiency for the photocatalytic removal of methylene blue dye from water under solar irradiation. TiO₂ NPs synthesized at 500°C showed good dye degradation over time (76%) compared to those synthesized at 400°C (51%) and 600°C (54%). At 500°C, the TiO₂ NPs are thoroughly characterized using XRD, SEM–EDS, UV–Vis spectroscopy, ATR-IR spectroscopy, and XRF. The results confirm the formation of nanoparticles. Titanium dioxide is of nanometric order, with an average crystallite size of approximately 15.2, according to XRD analysis. As a result, this study presents a green solution with a high potential for these nanoparticles to degrade the pollutant MB. These nanoparticles can be improved and used to degrade other pollutants through photocatalysis, as well as to contribute to water purificationQuery.

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来源期刊
The European Physical Journal Plus
The European Physical Journal Plus PHYSICS, MULTIDISCIPLINARY-
CiteScore
5.40
自引率
8.80%
发文量
1150
审稿时长
4-8 weeks
期刊介绍: The aims of this peer-reviewed online journal are to distribute and archive all relevant material required to document, assess, validate and reconstruct in detail the body of knowledge in the physical and related sciences. The scope of EPJ Plus encompasses a broad landscape of fields and disciplines in the physical and related sciences - such as covered by the topical EPJ journals and with the explicit addition of geophysics, astrophysics, general relativity and cosmology, mathematical and quantum physics, classical and fluid mechanics, accelerator and medical physics, as well as physics techniques applied to any other topics, including energy, environment and cultural heritage.
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