Maharshi R. Dave, Fernando Vega and Nader Mahinpey*,
{"title":"采用多喷嘴装置改善胺吸收过程中CO2捕获的喷雾柱性能","authors":"Maharshi R. Dave, Fernando Vega and Nader Mahinpey*, ","doi":"10.1021/acs.iecr.4c0261510.1021/acs.iecr.4c02615","DOIUrl":null,"url":null,"abstract":"<p >The only commercially viable technology available today for CO<sub>2</sub> capture on an industrial scale is the amine absorption process. However, the capture cost is still significantly high and needs to be reduced to encourage more industries and businesses to implement the technology. One aspect of the process with a major scope of improvement is the absorber column. This research investigated the use of a spray column for gas–liquid contacting operation as compared to the currently used packed bed absorber, which is associated with high capital and maintenance cost. An experimental investigation was carried out using 30 wt % monoethanol amine as the solvent to obtain a CO<sub>2</sub> concentration and temperature profile along the spray column length and measure the overall absorption efficiency. The multinozzle arrangement used in this study showed the best performance as compared to the single-nozzle spray column with an increase in absorption efficiency by up to 10% under similar operating conditions.</p>","PeriodicalId":39,"journal":{"name":"Industrial & Engineering Chemistry Research","volume":"63 49","pages":"21519–21538 21519–21538"},"PeriodicalIF":3.9000,"publicationDate":"2024-11-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Improvement of the Spray Column Performance for CO2 Capture in an Amine Absorption Process Using Multiple Nozzle Arrangement\",\"authors\":\"Maharshi R. Dave, Fernando Vega and Nader Mahinpey*, \",\"doi\":\"10.1021/acs.iecr.4c0261510.1021/acs.iecr.4c02615\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >The only commercially viable technology available today for CO<sub>2</sub> capture on an industrial scale is the amine absorption process. However, the capture cost is still significantly high and needs to be reduced to encourage more industries and businesses to implement the technology. One aspect of the process with a major scope of improvement is the absorber column. This research investigated the use of a spray column for gas–liquid contacting operation as compared to the currently used packed bed absorber, which is associated with high capital and maintenance cost. An experimental investigation was carried out using 30 wt % monoethanol amine as the solvent to obtain a CO<sub>2</sub> concentration and temperature profile along the spray column length and measure the overall absorption efficiency. The multinozzle arrangement used in this study showed the best performance as compared to the single-nozzle spray column with an increase in absorption efficiency by up to 10% under similar operating conditions.</p>\",\"PeriodicalId\":39,\"journal\":{\"name\":\"Industrial & Engineering Chemistry Research\",\"volume\":\"63 49\",\"pages\":\"21519–21538 21519–21538\"},\"PeriodicalIF\":3.9000,\"publicationDate\":\"2024-11-27\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Industrial & Engineering Chemistry Research\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acs.iecr.4c02615\",\"RegionNum\":3,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENGINEERING, CHEMICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Industrial & Engineering Chemistry Research","FirstCategoryId":"5","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acs.iecr.4c02615","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
Improvement of the Spray Column Performance for CO2 Capture in an Amine Absorption Process Using Multiple Nozzle Arrangement
The only commercially viable technology available today for CO2 capture on an industrial scale is the amine absorption process. However, the capture cost is still significantly high and needs to be reduced to encourage more industries and businesses to implement the technology. One aspect of the process with a major scope of improvement is the absorber column. This research investigated the use of a spray column for gas–liquid contacting operation as compared to the currently used packed bed absorber, which is associated with high capital and maintenance cost. An experimental investigation was carried out using 30 wt % monoethanol amine as the solvent to obtain a CO2 concentration and temperature profile along the spray column length and measure the overall absorption efficiency. The multinozzle arrangement used in this study showed the best performance as compared to the single-nozzle spray column with an increase in absorption efficiency by up to 10% under similar operating conditions.
期刊介绍:
ndustrial & Engineering Chemistry, with variations in title and format, has been published since 1909 by the American Chemical Society. Industrial & Engineering Chemistry Research is a weekly publication that reports industrial and academic research in the broad fields of applied chemistry and chemical engineering with special focus on fundamentals, processes, and products.