多谐振全太阳光谱完美超材料吸收器。

IF 4.4 3区 材料科学 Q2 CHEMISTRY, MULTIDISCIPLINARY
Nanomaterials Pub Date : 2024-12-06 DOI:10.3390/nano14231959
Zhe Shen, Junfan Ni
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引用次数: 0

摘要

目前,超材料的完美吸收特性在太阳能领域引起了广泛关注。超宽带吸收、入射角不敏感和偏振无关是设计吸收器的关键性能指标。在这项工作中,我们提出了一种基于多重共振吸收机制的超材料吸收器,包括传播表面等离子体共振(PSPR)、局部表面等离子体共振(LSPR)、电偶极子共振(EDR)和磁偶极子共振(MDR)。该吸收器由复合纳米圆柱和微腔组成,可实现对太阳能的全光谱吸收。在正常入射条件下,该吸收器在 272 纳米至 2742 纳米波长范围内获得了高吸收率(>95%)。在 280 纳米到 3000 纳米的波长范围内,吸收器在空气质量为 1.5 直射时的加权吸收率超过 98.5%。超宽带完美吸收可归因于这些共振的相互作用。通过分析结构参数对吸收效率的影响,该吸收器表现出优异的容错性。此外,所设计的吸收器对偏振和环境折射率变化不敏感,在入射角为 50° 时吸收率超过 80%。我们提出的吸收器在太阳能收集、光热转换和其他相关领域具有巨大的应用潜力。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Multi-Resonant Full-Solar-Spectrum Perfect Metamaterial Absorber.

Currently, perfect absorption properties of metamaterials have attracted widespread interest in the area of solar energy. Ultra-broadband absorption, incidence angle insensitivity, and polarization independence are key performance indicators in the design of the absorbers. In this work, we proposed a metamaterial absorber based on the absorption mechanism with multiple resonances, including propagation surface plasmon resonance (PSPR), localized surface plasmon resonance (LSPR), electric dipole resonance (EDR), and magnetic dipole resonance (MDR). The absorber, consisting of composite nanocylinders and a microcavity, can perform solar energy full-spectrum absorption. The proposed absorber obtained high absorption (>95%) from 272 nm to 2742 nm at normal incidence. The weighted absorption rate of the absorber at air mass 1.5 direct in the wavelength range of 280 nm to 3000 nm exceeds 98.5%. The ultra-broadband perfect absorption can be ascribed to the interaction of those resonances. The photothermal conversion efficiency of the absorber reaches 85.3% at 375 K. By analyzing the influence of the structural parameters on the absorption efficiency, the absorber exhibits excellent fault tolerance. In addition, the designed absorber is insensitive to polarization and variation in ambient refractive index and has an absorption rate of more than 80% at the incident angle of 50°. Our proposed absorber has great application potential in solar energy collection, photothermal conversion, and other related areas.

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来源期刊
Nanomaterials
Nanomaterials NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
8.50
自引率
9.40%
发文量
3841
审稿时长
14.22 days
期刊介绍: Nanomaterials (ISSN 2076-4991) is an international and interdisciplinary scholarly open access journal. It publishes reviews, regular research papers, communications, and short notes that are relevant to any field of study that involves nanomaterials, with respect to their science and application. Thus, theoretical and experimental articles will be accepted, along with articles that deal with the synthesis and use of nanomaterials. Articles that synthesize information from multiple fields, and which place discoveries within a broader context, will be preferred. There is no restriction on the length of the papers. Our aim is to encourage scientists to publish their experimental and theoretical research in as much detail as possible. Full experimental or methodical details, or both, must be provided for research articles. Computed data or files regarding the full details of the experimental procedure, if unable to be published in a normal way, can be deposited as supplementary material. Nanomaterials is dedicated to a high scientific standard. All manuscripts undergo a rigorous reviewing process and decisions are based on the recommendations of independent reviewers.
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