2024年ACS应用材料与接口家族早期职业论坛

IF 8.2 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Xing Yi Ling
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This Forum highlights groundbreaking research and innovative ideas from the emerging authors in the scientific community. A broad range of topics are covered, among these, energy and biorelated research take center stage, with a significant number of papers dedicated to these fields. Given the diversity of the topics, it is challenging to single out individual contributions. Instead, I have approached this by analyzing the prevailing trends across the Forum. Energy research is undergoing a transformative phase, fueled by advancements in catalysts, photocatalysts, batteries materials, and fabrication techniques. These breakthroughs are driving innovations in energy storage, harvesting, and conversion technologies, offering sustainable and efficient solutions for the future. Multifunction catalysts and photocatalysts materials are unlocking new potential in applications such as zinc–air batteries, hydrogen production, and water splitting. (1−4) Progress in advanced photovoltaic materials, including perovskites and photonic nanomaterials, is accelerating renewable energy technologies. Thermoelectric materials enable the conversion of low-grade heat into usable energy, whereas lightweight, flexible materials, such as 2D structures and thin-film polymers, are paving the way for scalable solar films and stretchable thermoelectric generators. (5−7) In biomaterials, different types of nanoparticles are revolutionizing cancer therapy, imaging, and biosensor technologies. Stimuli-responsive materials are employed for targeted drug delivery and advanced medical applications. Meanwhile, bioinks and 3D-printed biomaterials are driving breakthroughs in tissue engineering and wound healing, combining biocompatibility with functional properties to support regenerative medicine. (8−12) I would like to highlight a few noteworthy articles in key themes such as energy, catalysis, and device technologies. In a perspective, Xin et al. discuss nonconventional electrochemical reactions in rechargeable lithium–sulfur (Li–S) batteries, addressing the challenge of unstable polysulfide intermediates. The authors review innovative strategies to enhance battery stability and performance, focusing on modifications to sulfur allotropes, electrolyte composition, and electrode design. (13) In a related study, Shi et al. investigate the nucleation mechanisms of lithium pits and their morphological evolution across large electrode areas. Their findings reveal that overpotential is inversely related to pit radius and exponentially related to nucleation rate, offering new insights for predicting and controlling surface area and roughness in lithium electrodes under various stripping conditions (Figure 2). (14) Figure 2. Selected graphics from <i>ACS Applied Materials &amp; Interfaces</i> Early Career Forum, showcasing energy-related research, including studies on lithium–sulfur batteries and lithium pit nucleation. In the rapidly growing area of electronics, two particularly exciting fields─optoelectronic synapses and heat harvesting─are showcased. Xu and co-workers present an organic optoelectronic synapse with multilevel memory, enabled by gate modulation. It mimics synaptic plasticity with both volatile and nonvolatile states, transitioning between short-term and long-term plasticity through gate voltage and light exposure. The device offers program/erase current ratios and stability, making it a promising candidate for neuromorphic systems in image processing and memory retention (Figure 3A). (15) In parallel, Cai et al. introduce a heat harvesting system that combines daytime radiative cooling with thermally regenerative electrochemical cycles (TREC). Using nanoporous polyethylene and MXene, the system passively generates a 35 °C temperature difference under sunlight, converting ambient heat into continuous electricity with a 50 mV cell voltage and over 20 mAh/g specific capacity, without external charging (Figure 3B). (16) Figure 3. Selected graphics from <i>ACS Applied Materials &amp; Interfaces</i> Early Career Forum. (A) Organic optoelectronic synapse with multilevel memory capabilities, demonstrating synaptic plasticity transitions between short-term and long-term memory states. (B) Low-grade heat harvesting system combining daytime radiative cooling with thermally regenerative electrochemical cycles, achieving continuous electricity generation. Finally, we extend our heartfelt thanks to all the authors, reviewers, and editors who made this third edition of the Early Career Forum a success. We look forward to continuing this tradition of recognizing early career researchers in future editions. Be sure to explore many other outstanding articles published across the ACS Applied Materials family journals. Access the full Forum at each of the family journals below: <i>ACS Applied Bio Materials</i>: Volume 7, Issue 12 <i>ACS Applied Electronic Materials</i>: Volume 6, Issue 12 <i>ACS Applied Energy Materials</i>: Volume 7, Issue 24 <i>ACS Applied Engineering Materials</i>: Volume 2, Issue 12 <i>ACS Applied Nano Materials</i>: Volume 7, Issue 23 <i>ACS Applied Optical Materials</i>: Volume 2, Issue 12 <i>ACS Applied Polymer Materials</i>: Volume 6, Issue 23 This article references 16 other publications. 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Instead, I have approached this by analyzing the prevailing trends across the Forum. Energy research is undergoing a transformative phase, fueled by advancements in catalysts, photocatalysts, batteries materials, and fabrication techniques. These breakthroughs are driving innovations in energy storage, harvesting, and conversion technologies, offering sustainable and efficient solutions for the future. Multifunction catalysts and photocatalysts materials are unlocking new potential in applications such as zinc–air batteries, hydrogen production, and water splitting. (1−4) Progress in advanced photovoltaic materials, including perovskites and photonic nanomaterials, is accelerating renewable energy technologies. Thermoelectric materials enable the conversion of low-grade heat into usable energy, whereas lightweight, flexible materials, such as 2D structures and thin-film polymers, are paving the way for scalable solar films and stretchable thermoelectric generators. (5−7) In biomaterials, different types of nanoparticles are revolutionizing cancer therapy, imaging, and biosensor technologies. Stimuli-responsive materials are employed for targeted drug delivery and advanced medical applications. Meanwhile, bioinks and 3D-printed biomaterials are driving breakthroughs in tissue engineering and wound healing, combining biocompatibility with functional properties to support regenerative medicine. (8−12) I would like to highlight a few noteworthy articles in key themes such as energy, catalysis, and device technologies. In a perspective, Xin et al. discuss nonconventional electrochemical reactions in rechargeable lithium–sulfur (Li–S) batteries, addressing the challenge of unstable polysulfide intermediates. The authors review innovative strategies to enhance battery stability and performance, focusing on modifications to sulfur allotropes, electrolyte composition, and electrode design. (13) In a related study, Shi et al. investigate the nucleation mechanisms of lithium pits and their morphological evolution across large electrode areas. Their findings reveal that overpotential is inversely related to pit radius and exponentially related to nucleation rate, offering new insights for predicting and controlling surface area and roughness in lithium electrodes under various stripping conditions (Figure 2). (14) Figure 2. Selected graphics from <i>ACS Applied Materials &amp; Interfaces</i> Early Career Forum, showcasing energy-related research, including studies on lithium–sulfur batteries and lithium pit nucleation. In the rapidly growing area of electronics, two particularly exciting fields─optoelectronic synapses and heat harvesting─are showcased. Xu and co-workers present an organic optoelectronic synapse with multilevel memory, enabled by gate modulation. It mimics synaptic plasticity with both volatile and nonvolatile states, transitioning between short-term and long-term plasticity through gate voltage and light exposure. The device offers program/erase current ratios and stability, making it a promising candidate for neuromorphic systems in image processing and memory retention (Figure 3A). (15) In parallel, Cai et al. introduce a heat harvesting system that combines daytime radiative cooling with thermally regenerative electrochemical cycles (TREC). Using nanoporous polyethylene and MXene, the system passively generates a 35 °C temperature difference under sunlight, converting ambient heat into continuous electricity with a 50 mV cell voltage and over 20 mAh/g specific capacity, without external charging (Figure 3B). (16) Figure 3. Selected graphics from <i>ACS Applied Materials &amp; Interfaces</i> Early Career Forum. 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引用次数: 0

摘要

本文是早期职业论坛2024特刊的一部分。我们很高兴地举办2024年ACS AMI家庭早期职业论坛,展示了来自全球早期职业科学家的135位杰出贡献(图1)。其中,共有25位贡献来自ACS应用材料公司。接口:ACS应用能源材料22个,ACS应用生物材料23个,ACS应用高分子材料18个,ACS应用纳米材料17个,ACS应用电子材料14个,ACS应用光学材料11个,ACS应用工程材料5个。图1所示。应用材料组合期刊早期职业论坛文章作者的地理分布。本论坛突出了科学界新兴作者的突破性研究和创新思想。涵盖了广泛的主题,其中,能源和生物相关的研究占据了中心舞台,有大量的论文致力于这些领域。鉴于主题的多样性,挑选出个人的贡献是具有挑战性的。相反,我通过分析整个论坛的流行趋势来解决这个问题。由于催化剂、光催化剂、电池材料和制造技术的进步,能源研究正在经历一个变革阶段。这些突破正在推动能源储存、收集和转换技术的创新,为未来提供可持续和高效的解决方案。多功能催化剂和光催化剂材料在锌空气电池、制氢和水分解等应用中释放出新的潜力。(1−4)包括钙钛矿和光子纳米材料在内的先进光伏材料的进展正在加速可再生能源技术的发展。热电材料能够将低等级的热量转化为可用的能量,而轻质、柔性的材料,如二维结构和薄膜聚合物,正在为可扩展的太阳能薄膜和可拉伸的热电发电机铺平道路。(5−7)在生物材料领域,不同类型的纳米颗粒正在彻底改变癌症治疗、成像和生物传感器技术。刺激反应材料用于靶向药物输送和先进的医疗应用。与此同时,生物墨水和3d打印生物材料正在推动组织工程和伤口愈合方面的突破,将生物相容性与功能特性结合起来,支持再生医学。(8−12)我想重点介绍几篇关于能源、催化和设备技术等关键主题的值得注意的文章。从一个角度来看,Xin等人讨论了可充电锂硫(Li-S)电池中的非常规电化学反应,解决了不稳定多硫化物中间体的挑战。作者回顾了提高电池稳定性和性能的创新策略,重点是对硫同素异素物,电解质成分和电极设计的修改。(13)在一项相关研究中,Shi等人研究了锂坑的成核机制及其在大电极区域的形态演变。他们的研究结果表明,过电位与坑半径呈负相关,与成核速率呈指数相关,这为预测和控制不同剥离条件下锂电极的表面积和粗糙度提供了新的见解(图2)。选自ACS应用材料&amp;界面早期职业论坛,展示能源相关研究,包括锂硫电池和锂坑成核的研究。在快速发展的电子学领域,两个特别令人兴奋的领域──光电突触和热收集──被展示出来。Xu和他的同事们提出了一个有机光电突触与多电平记忆,启用门调制。它以挥发性和非挥发性状态模拟突触可塑性,通过栅电压和光照在短期和长期可塑性之间转换。该器件提供程序/擦除电流比和稳定性,使其成为图像处理和记忆保留中神经形态系统的有希望的候选者(图3A)。(15)与此同时,Cai等人介绍了一种将日间辐射冷却与热再生电化学循环(TREC)相结合的热收集系统。该系统使用纳米多孔聚乙烯和MXene,在阳光下被动产生35°C的温差,将环境热量转化为连续的电能,电池电压为50 mV,比容量超过20 mAh/g,无需外部充电(图3B)。(16)图3。选自ACS应用材料&amp;接口早期职业论坛。(A)具有多层次记忆能力的有机光电突触,显示了突触在短期和长期记忆状态之间的可塑性转换。 (B)低品位集热系统,将日间辐射冷却与热再生电化学循环相结合,实现连续发电。最后,我们衷心感谢所有的作者、审稿人和编辑,他们使第三届早期职业论坛取得了成功。我们期待着在未来的版本中继续这一传统,以表彰早期职业研究人员。一定要探索ACS应用材料家族期刊上发表的许多其他优秀文章。访问以下每个家庭期刊的完整论坛:ACS应用生物材料:第7卷,第12期ACS应用电子材料:第6卷,第12期ACS应用能源材料:第7卷,第24期ACS应用工程材料:第2卷,第12期ACS应用纳米材料:第7卷,第23期ACS应用光学材料:第2卷,第12期ACS应用聚合物材料:第6卷,第23期本文引用了16个其他出版物。这篇文章尚未被其他出版物引用。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

ACS Applied Materials & Interfaces Family Early Career Forum 2024

ACS Applied Materials & Interfaces Family Early Career Forum 2024
This article is part of the Early Career Forum 2024 special issue. We are delighted to present the 2024 ACS AMI Family Early Career Forum, showcasing 135 exceptional contributions from early career scientists worldwide (Figure 1). Among these, there are a total of 25 contributions to ACS Applied Materials & Interfaces, 22 to ACS Applied Energy Materials, 23 to ACS Applied Bio Materials, 18 to ACS Applied Polymer Materials, 17 to ACS Applied Nano Materials, 14 to ACS Applied Electronic Materials, 11 to ACS Applied Optical Materials, and 5 to ACS Applied Engineering Materials. Figure 1. Geographical distribution of authors for the articles in the Applied Materials Portfolio Journals’ Early Career Forum. This Forum highlights groundbreaking research and innovative ideas from the emerging authors in the scientific community. A broad range of topics are covered, among these, energy and biorelated research take center stage, with a significant number of papers dedicated to these fields. Given the diversity of the topics, it is challenging to single out individual contributions. Instead, I have approached this by analyzing the prevailing trends across the Forum. Energy research is undergoing a transformative phase, fueled by advancements in catalysts, photocatalysts, batteries materials, and fabrication techniques. These breakthroughs are driving innovations in energy storage, harvesting, and conversion technologies, offering sustainable and efficient solutions for the future. Multifunction catalysts and photocatalysts materials are unlocking new potential in applications such as zinc–air batteries, hydrogen production, and water splitting. (1−4) Progress in advanced photovoltaic materials, including perovskites and photonic nanomaterials, is accelerating renewable energy technologies. Thermoelectric materials enable the conversion of low-grade heat into usable energy, whereas lightweight, flexible materials, such as 2D structures and thin-film polymers, are paving the way for scalable solar films and stretchable thermoelectric generators. (5−7) In biomaterials, different types of nanoparticles are revolutionizing cancer therapy, imaging, and biosensor technologies. Stimuli-responsive materials are employed for targeted drug delivery and advanced medical applications. Meanwhile, bioinks and 3D-printed biomaterials are driving breakthroughs in tissue engineering and wound healing, combining biocompatibility with functional properties to support regenerative medicine. (8−12) I would like to highlight a few noteworthy articles in key themes such as energy, catalysis, and device technologies. In a perspective, Xin et al. discuss nonconventional electrochemical reactions in rechargeable lithium–sulfur (Li–S) batteries, addressing the challenge of unstable polysulfide intermediates. The authors review innovative strategies to enhance battery stability and performance, focusing on modifications to sulfur allotropes, electrolyte composition, and electrode design. (13) In a related study, Shi et al. investigate the nucleation mechanisms of lithium pits and their morphological evolution across large electrode areas. Their findings reveal that overpotential is inversely related to pit radius and exponentially related to nucleation rate, offering new insights for predicting and controlling surface area and roughness in lithium electrodes under various stripping conditions (Figure 2). (14) Figure 2. Selected graphics from ACS Applied Materials & Interfaces Early Career Forum, showcasing energy-related research, including studies on lithium–sulfur batteries and lithium pit nucleation. In the rapidly growing area of electronics, two particularly exciting fields─optoelectronic synapses and heat harvesting─are showcased. Xu and co-workers present an organic optoelectronic synapse with multilevel memory, enabled by gate modulation. It mimics synaptic plasticity with both volatile and nonvolatile states, transitioning between short-term and long-term plasticity through gate voltage and light exposure. The device offers program/erase current ratios and stability, making it a promising candidate for neuromorphic systems in image processing and memory retention (Figure 3A). (15) In parallel, Cai et al. introduce a heat harvesting system that combines daytime radiative cooling with thermally regenerative electrochemical cycles (TREC). Using nanoporous polyethylene and MXene, the system passively generates a 35 °C temperature difference under sunlight, converting ambient heat into continuous electricity with a 50 mV cell voltage and over 20 mAh/g specific capacity, without external charging (Figure 3B). (16) Figure 3. Selected graphics from ACS Applied Materials & Interfaces Early Career Forum. (A) Organic optoelectronic synapse with multilevel memory capabilities, demonstrating synaptic plasticity transitions between short-term and long-term memory states. (B) Low-grade heat harvesting system combining daytime radiative cooling with thermally regenerative electrochemical cycles, achieving continuous electricity generation. Finally, we extend our heartfelt thanks to all the authors, reviewers, and editors who made this third edition of the Early Career Forum a success. We look forward to continuing this tradition of recognizing early career researchers in future editions. Be sure to explore many other outstanding articles published across the ACS Applied Materials family journals. Access the full Forum at each of the family journals below: ACS Applied Bio Materials: Volume 7, Issue 12 ACS Applied Electronic Materials: Volume 6, Issue 12 ACS Applied Energy Materials: Volume 7, Issue 24 ACS Applied Engineering Materials: Volume 2, Issue 12 ACS Applied Nano Materials: Volume 7, Issue 23 ACS Applied Optical Materials: Volume 2, Issue 12 ACS Applied Polymer Materials: Volume 6, Issue 23 This article references 16 other publications. This article has not yet been cited by other publications.
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来源期刊
ACS Applied Materials & Interfaces
ACS Applied Materials & Interfaces 工程技术-材料科学:综合
CiteScore
16.00
自引率
6.30%
发文量
4978
审稿时长
1.8 months
期刊介绍: ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.
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