{"title":"以向日葵为灵感的智能蒸发器,具有全方位的太阳能跟踪,可高度增强能量捕获和可持续的淡水收集","authors":"Yuchun Shen, Rong Zhang, Guodong Hou, Yu Chen, Peng Yang, Xiaoshi Qian, Shaochun Tang","doi":"10.1016/j.cej.2024.157917","DOIUrl":null,"url":null,"abstract":"Efficient solar energy utilization and stability are critical for the developed field operation of interfacial solar vapor generation. Inspired by natural sunflowers, we developed an advanced biomimetic phototropic solar interfacial evaporator (BPSIE) capable of omnidirectional light tracking and efficient solar energy harvesting without any electronics. The stem of BPSIE is comprised of a stimuli-responsive hydrogel that detects incident light and moves in any direction in 3D space using embedded negative feedback control. The BPSIE maintains a high level of light-to-vapor energy conversion efficiency of 99.27 % and a water evaporation rate reaching 6.18 kg m<sup>-2</sup> h<sup>−1</sup> under 4 simulated solar irradiations due to its phototropism at incidence angles from 0° to 180°, enhancing energy harvest by 200 % compared to non-tropistic materials, which is confirmed by simulations of time-dependent volume shrinkage and temperature distribution. Different from other phototropic solar evaporators, our developed BPSIE is highly porous and mechanically strong and thus can hold itself in air. With only its stem immersed, the porous structure exhibits fast water transport from the water surface to evaporating disk. Additionally, the BPSIE is capable of fast self-healing if severely broken, providing additional stability and enabling sustainable field operation in the real world.","PeriodicalId":270,"journal":{"name":"Chemical Engineering Journal","volume":"9 1","pages":""},"PeriodicalIF":13.2000,"publicationDate":"2024-12-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Sunflower-inspired smart evaporator with omnidirectional solar tracking for highly enhanced energy-capturing and sustainable freshwater harvesting\",\"authors\":\"Yuchun Shen, Rong Zhang, Guodong Hou, Yu Chen, Peng Yang, Xiaoshi Qian, Shaochun Tang\",\"doi\":\"10.1016/j.cej.2024.157917\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Efficient solar energy utilization and stability are critical for the developed field operation of interfacial solar vapor generation. Inspired by natural sunflowers, we developed an advanced biomimetic phototropic solar interfacial evaporator (BPSIE) capable of omnidirectional light tracking and efficient solar energy harvesting without any electronics. The stem of BPSIE is comprised of a stimuli-responsive hydrogel that detects incident light and moves in any direction in 3D space using embedded negative feedback control. The BPSIE maintains a high level of light-to-vapor energy conversion efficiency of 99.27 % and a water evaporation rate reaching 6.18 kg m<sup>-2</sup> h<sup>−1</sup> under 4 simulated solar irradiations due to its phototropism at incidence angles from 0° to 180°, enhancing energy harvest by 200 % compared to non-tropistic materials, which is confirmed by simulations of time-dependent volume shrinkage and temperature distribution. Different from other phototropic solar evaporators, our developed BPSIE is highly porous and mechanically strong and thus can hold itself in air. With only its stem immersed, the porous structure exhibits fast water transport from the water surface to evaporating disk. Additionally, the BPSIE is capable of fast self-healing if severely broken, providing additional stability and enabling sustainable field operation in the real world.\",\"PeriodicalId\":270,\"journal\":{\"name\":\"Chemical Engineering Journal\",\"volume\":\"9 1\",\"pages\":\"\"},\"PeriodicalIF\":13.2000,\"publicationDate\":\"2024-12-06\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Chemical Engineering Journal\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://doi.org/10.1016/j.cej.2024.157917\",\"RegionNum\":1,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, CHEMICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Chemical Engineering Journal","FirstCategoryId":"5","ListUrlMain":"https://doi.org/10.1016/j.cej.2024.157917","RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
引用次数: 0
摘要
高效利用和稳定利用太阳能是界面太阳能蒸汽发电现场运行的关键。受天然向日葵的启发,我们开发了一种先进的仿生光致性太阳界面蒸发器(BPSIE),它能够在没有任何电子设备的情况下进行全方位的光跟踪和高效的太阳能收集。BPSIE的主体由一个刺激响应水凝胶组成,该水凝胶可以检测入射光,并使用嵌入式负反馈控制在3D空间中向任何方向移动。由于BPSIE在0°至180°的入射角范围内具有向光性,因此在4次模拟太阳照射下,BPSIE保持了99.27 %的光蒸汽能量转换效率和6.18 kg m-2 h - 1的水蒸发速率,与非向性材料相比,能量收获提高了200 %,这一点通过模拟随时间变化的体积收缩和温度分布得到了证实。与其他光敏性太阳能蒸发器不同,我们开发的BPSIE具有高度多孔性和机械强度,因此可以在空气中保持自身。多孔结构在只有阀杆浸入的情况下,表现出水从水面到蒸发盘的快速输送。此外,如果严重损坏,BPSIE能够快速自愈,提供额外的稳定性,并在现实世界中实现可持续的现场作业。
Sunflower-inspired smart evaporator with omnidirectional solar tracking for highly enhanced energy-capturing and sustainable freshwater harvesting
Efficient solar energy utilization and stability are critical for the developed field operation of interfacial solar vapor generation. Inspired by natural sunflowers, we developed an advanced biomimetic phototropic solar interfacial evaporator (BPSIE) capable of omnidirectional light tracking and efficient solar energy harvesting without any electronics. The stem of BPSIE is comprised of a stimuli-responsive hydrogel that detects incident light and moves in any direction in 3D space using embedded negative feedback control. The BPSIE maintains a high level of light-to-vapor energy conversion efficiency of 99.27 % and a water evaporation rate reaching 6.18 kg m-2 h−1 under 4 simulated solar irradiations due to its phototropism at incidence angles from 0° to 180°, enhancing energy harvest by 200 % compared to non-tropistic materials, which is confirmed by simulations of time-dependent volume shrinkage and temperature distribution. Different from other phototropic solar evaporators, our developed BPSIE is highly porous and mechanically strong and thus can hold itself in air. With only its stem immersed, the porous structure exhibits fast water transport from the water surface to evaporating disk. Additionally, the BPSIE is capable of fast self-healing if severely broken, providing additional stability and enabling sustainable field operation in the real world.
期刊介绍:
The Chemical Engineering Journal is an international research journal that invites contributions of original and novel fundamental research. It aims to provide an international platform for presenting original fundamental research, interpretative reviews, and discussions on new developments in chemical engineering. The journal welcomes papers that describe novel theory and its practical application, as well as those that demonstrate the transfer of techniques from other disciplines. It also welcomes reports on carefully conducted experimental work that is soundly interpreted. The main focus of the journal is on original and rigorous research results that have broad significance. The Catalysis section within the Chemical Engineering Journal focuses specifically on Experimental and Theoretical studies in the fields of heterogeneous catalysis, molecular catalysis, and biocatalysis. These studies have industrial impact on various sectors such as chemicals, energy, materials, foods, healthcare, and environmental protection.