{"title":"北太平洋西部210Pb沉降通量的时间序列观测","authors":"Hajime Kawakami","doi":"10.1007/s10967-024-09801-2","DOIUrl":null,"url":null,"abstract":"<div><p>We observed the lead-210 (<sup>210</sup>Pb) sinking flux in subarctic and subtropical regions of the western North Pacific Ocean over time. The <sup>210</sup>Pb fluxes in the mesopelagic and bathypelagic zones were estimated from the disequilibrium between <sup>210</sup>Pb and radium-226 (<sup>226</sup>Ra) in the water column over the 4 seasons during several years. In the subarctic region, <sup>210</sup>Pb fluxes were larger (28–29 dpm m<sup>–2</sup> d<sup>–1</sup> at 500 m; 68–70 dpm m<sup>–2</sup> d<sup>–1</sup> at 4810 m) than those in the subtropical region (22–24 dpm m<sup>–2</sup> d<sup>–1</sup> at 500 m; 46–49 dpm m<sup>–2</sup> d<sup>–1</sup> at 4810 m). These results imply that the strength of the biological pump in the mesopelagic and bathypelagic zones is larger in the subarctic region than in the subtropical region of the western North Pacific. We also determined <sup>210</sup>Pb in sinking particles collected by moored sediment traps. In the subarctic (subtropical) region, the annual average of trapped <sup>210</sup>Pb flux at 500 and 4810 m were 3.0 (4.6) and 24.2 (18.6) dpm m<sup>–2</sup> d<sup>–1</sup>, respectively. Estimated from the <sup>210</sup>Pb flux in the water column and the <sup>210</sup>Pb flux in the sinking particles in the sediment trap experiment, the trapping efficiencies at 500 m (10–20%) were about a half of those at 4810 m (35–40%) in the sediment trap experiment.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"333 12","pages":"6507 - 6514"},"PeriodicalIF":1.5000,"publicationDate":"2024-10-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Time-series observation of 210Pb sinking fluxes in the western North Pacific\",\"authors\":\"Hajime Kawakami\",\"doi\":\"10.1007/s10967-024-09801-2\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>We observed the lead-210 (<sup>210</sup>Pb) sinking flux in subarctic and subtropical regions of the western North Pacific Ocean over time. The <sup>210</sup>Pb fluxes in the mesopelagic and bathypelagic zones were estimated from the disequilibrium between <sup>210</sup>Pb and radium-226 (<sup>226</sup>Ra) in the water column over the 4 seasons during several years. In the subarctic region, <sup>210</sup>Pb fluxes were larger (28–29 dpm m<sup>–2</sup> d<sup>–1</sup> at 500 m; 68–70 dpm m<sup>–2</sup> d<sup>–1</sup> at 4810 m) than those in the subtropical region (22–24 dpm m<sup>–2</sup> d<sup>–1</sup> at 500 m; 46–49 dpm m<sup>–2</sup> d<sup>–1</sup> at 4810 m). These results imply that the strength of the biological pump in the mesopelagic and bathypelagic zones is larger in the subarctic region than in the subtropical region of the western North Pacific. We also determined <sup>210</sup>Pb in sinking particles collected by moored sediment traps. In the subarctic (subtropical) region, the annual average of trapped <sup>210</sup>Pb flux at 500 and 4810 m were 3.0 (4.6) and 24.2 (18.6) dpm m<sup>–2</sup> d<sup>–1</sup>, respectively. Estimated from the <sup>210</sup>Pb flux in the water column and the <sup>210</sup>Pb flux in the sinking particles in the sediment trap experiment, the trapping efficiencies at 500 m (10–20%) were about a half of those at 4810 m (35–40%) in the sediment trap experiment.</p></div>\",\"PeriodicalId\":661,\"journal\":{\"name\":\"Journal of Radioanalytical and Nuclear Chemistry\",\"volume\":\"333 12\",\"pages\":\"6507 - 6514\"},\"PeriodicalIF\":1.5000,\"publicationDate\":\"2024-10-22\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Radioanalytical and Nuclear Chemistry\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://link.springer.com/article/10.1007/s10967-024-09801-2\",\"RegionNum\":3,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"CHEMISTRY, ANALYTICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Radioanalytical and Nuclear Chemistry","FirstCategoryId":"92","ListUrlMain":"https://link.springer.com/article/10.1007/s10967-024-09801-2","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, ANALYTICAL","Score":null,"Total":0}
引用次数: 0
摘要
研究了北太平洋西部亚北极和亚热带地区铅-210 (210Pb)沉降通量随时间的变化。通过多年来水柱中210Pb与镭-226 (226Ra)的不平衡,估算了中上层和深海4个季节的210Pb通量。在亚北极地区,210Pb通量较大(在500 m处为28-29 dpm m - 2 d-1;4810 m海拔高度为68 ~ 70 dpm m - 2 d-1), 500 m海拔高度为22 ~ 24 dpm m - 2 d-1;这些结果表明,亚北极地区中远洋和深海生物泵的强度大于北太平洋西部亚热带地区。我们还测定了系泊沉淀池收集的沉降颗粒中的210Pb。在亚北极(亚热带)地区,500和4810 m处捕获的210Pb通量的年平均值分别为3.0(4.6)和24.2 (18.6)dpm m - 2 d-1。根据捕集器试验中水柱中210Pb通量和沉降颗粒中210Pb通量估算,500 m处捕集效率(10-20%)约为4810 m处捕集效率(35-40%)的一半。
Time-series observation of 210Pb sinking fluxes in the western North Pacific
We observed the lead-210 (210Pb) sinking flux in subarctic and subtropical regions of the western North Pacific Ocean over time. The 210Pb fluxes in the mesopelagic and bathypelagic zones were estimated from the disequilibrium between 210Pb and radium-226 (226Ra) in the water column over the 4 seasons during several years. In the subarctic region, 210Pb fluxes were larger (28–29 dpm m–2 d–1 at 500 m; 68–70 dpm m–2 d–1 at 4810 m) than those in the subtropical region (22–24 dpm m–2 d–1 at 500 m; 46–49 dpm m–2 d–1 at 4810 m). These results imply that the strength of the biological pump in the mesopelagic and bathypelagic zones is larger in the subarctic region than in the subtropical region of the western North Pacific. We also determined 210Pb in sinking particles collected by moored sediment traps. In the subarctic (subtropical) region, the annual average of trapped 210Pb flux at 500 and 4810 m were 3.0 (4.6) and 24.2 (18.6) dpm m–2 d–1, respectively. Estimated from the 210Pb flux in the water column and the 210Pb flux in the sinking particles in the sediment trap experiment, the trapping efficiencies at 500 m (10–20%) were about a half of those at 4810 m (35–40%) in the sediment trap experiment.
期刊介绍:
An international periodical publishing original papers, letters, review papers and short communications on nuclear chemistry. The subjects covered include: Nuclear chemistry, Radiochemistry, Radiation chemistry, Radiobiological chemistry, Environmental radiochemistry, Production and control of radioisotopes and labelled compounds, Nuclear power plant chemistry, Nuclear fuel chemistry, Radioanalytical chemistry, Radiation detection and measurement, Nuclear instrumentation and automation, etc.