Han Chen, Xue-Qing Zhan, Zhi-Ling Hong, Wang Ni, Chang-Chang Zhu, Yong-Ping Leng, Chun-Chi Chen, Rey-Ting Guo, Ning Ma, Fang-Chang Tsai
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引用次数: 0
摘要
水体中重金属离子含量超标对人类健康和生态系统的潜在危害日益引起世界各国的关注。因此,研究开发一种灵敏、直观的水质监测方法就显得尤为重要。本文构建了双网络设计的聚(丙烯酸-co- n -甲基丙烯酰胺)/聚(3,4-乙烯二氧噻吩):聚苯磺酸P(AA-co-N-MA)/PEDOT: PSS水凝胶,并用于Fe3+的检测。与以往报道相比,P(AA-co-N-MA)/PEDOT: PSS水凝胶对免疫铁离子(Fe3+)的检测更加灵敏和方便,可用于监测微量超标准(人体健康监测检测下限为0.52 ppm,对应0.06 S/m,水质监测阈值为0.16 S/m)。水凝胶中Fe3+含量与电导率之间的关系使其能够与其他电子器件集成,为人体Fe3+提供预警功能,对人体健康监测具有重要意义。
Hydrogel-Based Sensor for the Detection of Iron Ions and Excessive Alerting
The excessive content of heavy metal ions in water has attracted increasing worldwide attention due to the potential harm to human health and ecological systems. Therefore, it is particularly significant to research and develop a sensitive and straightforward water quality monitoring method. Here, a dual-network designed hydrogel poly(acrylic acid-co-N-methylolacrylamide)/poly(3,4-ethylenedioxythiophene): polystyrenesulfonate, P(AA-co-N-MA)/PEDOT: PSS, was constructed and used for Fe3+ detection. Compared with previous reports, the P(AA-co-N-MA)/PEDOT: PSS hydrogel has a much more sensitive and convenient detection of immune iron ions (Fe3+), is applied to monitor a trace of over-the-standard (the lower limit of detection is 0.52 ppm corresponding to 0.06 S/m for human health monitor, and the threshold for water quality monitoring is 0.16 S/m). The relationship between Fe3+ content and the conductivity of the hydrogel allows it to integrate with other electron devices to provide an early warning function for Fe3+ in the human body, which would be of great significance to human health monitoring.
期刊介绍:
Langmuir is an interdisciplinary journal publishing articles in the following subject categories:
Colloids: surfactants and self-assembly, dispersions, emulsions, foams
Interfaces: adsorption, reactions, films, forces
Biological Interfaces: biocolloids, biomolecular and biomimetic materials
Materials: nano- and mesostructured materials, polymers, gels, liquid crystals
Electrochemistry: interfacial charge transfer, charge transport, electrocatalysis, electrokinetic phenomena, bioelectrochemistry
Devices and Applications: sensors, fluidics, patterning, catalysis, photonic crystals
However, when high-impact, original work is submitted that does not fit within the above categories, decisions to accept or decline such papers will be based on one criteria: What Would Irving Do?
Langmuir ranks #2 in citations out of 136 journals in the category of Physical Chemistry with 113,157 total citations. The journal received an Impact Factor of 4.384*.
This journal is also indexed in the categories of Materials Science (ranked #1) and Multidisciplinary Chemistry (ranked #5).