气候变化和人类活动对河流主导的海岸带陆相有机碳积累变化的耦合影响

IF 3.3 2区 地球科学 Q1 OCEANOGRAPHY
Li Jiang, Limin Hu, Yazhi Bai, Jiazong Du, Naishuang Bi, Xiao Wu, Xueshi Sun, Zhigang Guo, Houjie Wang, Zuosheng Yang
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引用次数: 0

摘要

以河流为主的边缘海在全球碳循环中起着至关重要的作用。然而,有机碳(OC)的百年埋藏记录仍不清楚。本研究基于黄渤海(BS)沉积岩心,综合分析了沉积体OC、同位素组成(δ13C和Δ14C)、生物标志物(木质素和正构烷烃)和沉积演化。我们还汇编了几份来自其他河流主导的沿海边缘的已发表的OC埋葬记录。我们的研究结果表明,自20世纪50年代以来,BS中部陆源OC的积累呈现出同步下降的趋势,其证据是陆源/水生正构烷烃(TAR)的比值下降了50%,同时由于流域人类活动导致沉积物负荷显著减少。20世纪80年代以来,在冬季风暴频率增加的条件下,更强的水动力条件导致了更强烈的侵蚀和重悬浮,这可能是观测到的沉积物粗化以及伴随的降解木质素和老OC增加的原因,表明三角洲侵蚀引起的沉积物再分配可能影响更多木质异源OC组分的选择性运输和积累。木质素记录的时间剖面表明,在全球三角洲侵蚀加剧的情况下,河流主导的大型沿海边缘地区近期陆相OC埋藏具有空间异质性。与长江、珠江和密西西比河三角洲边缘以河流输入为主的OC埋藏相比,由于近期气候变化和沉积物负荷大幅下降的耦合作用,BS对陆相OC埋藏的水动力强迫影响更大。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Coupled Impact of Climate Change and Anthropogenic Activity on the Changes of Terrestrial Organic Carbon Accumulation in the River-Dominated Coastal Margin

River-dominated marginal seas play a crucial role in the global carbon cycle. However, the centennial burial record of organic carbon (OC) remains unclear. In this study, we conducted a comprehensive analysis of bulk OC, its isotopic composition (δ13C and Δ14C), biomarkers (lignin and n-alkanes), and sedimentological evolution based on sediment core from the Yellow River-dominated Bohai Sea (BS). We also compiled several published OC burial records from other river-dominated coastal margins. Our findings indicated that since the 1950s, the accumulation of terrestrial OC in central BS has shown a concurrent decline, as evidenced by a ∼50% decrease in terrigenous/aquatic ratio of n-alkanes (TAR), which accompanied by a significant reduction in sediment load due to the watershed human activities. More intense erosion and resuspension due to stronger hydrodynamic condition under the increasing frequency of winter storms could account for the observed sediment coarsening and concomitant increase of the degraded lignin and old-OC since the 1980s, suggesting that delta erosion-induced sediment redistribution could influence the selective transport and accumulation of the more woody allochthonous OC components. The temporal profiles of lignin records indicated a spatial heterogeneity of recent terrestrial OC burial among the large river-dominated coastal margins under the enhanced global delta erosion. Compared to the fluvial input-dominated OC burial in the Yangtze River, Pearl River and Mississippi River delta margins, a more hydrodynamic forcing impact on the terrestrial OC burial was discerned in the BS due to the coupled effect of recent climate change and substantial decline in sediment load.

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来源期刊
Journal of Geophysical Research-Oceans
Journal of Geophysical Research-Oceans Earth and Planetary Sciences-Oceanography
CiteScore
7.00
自引率
13.90%
发文量
429
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