{"title":"综述:降低宽禁带钙钛矿太阳能电池开路电压损失的策略","authors":"Lu-Yao Chen , Qi Sun , Yue-Min Xie , Man-Keung Fung","doi":"10.1039/d4cc05131a","DOIUrl":null,"url":null,"abstract":"<div><div>Perovskite-based tandem solar cells (PTSCs) have made remarkable achievements in recent years, and the highest certified power conversion efficiency (PCE) of 33.9% has been achieved in perovskite/silicon tandem solar cells (PSTSCs), indicating their great commercialization potential. Nevertheless, the performance of PTSCs continues to be hindered by the compromised performance of wide-bandgap perovskite solar cells (WPSCs), particularly the high <em>V</em><sub>OC</sub> deficit of WPSCs. Therefore, numerous strategies have been developed to minimize the <em>V</em><sub>OC</sub> loss of WPSCs. Herein, we sort to comprehensively review about the reported studies on reducing the <em>V</em><sub>OC</sub> deficit of WPSCs, focusing on interface modification, charge transport material (CTM) exploration, and additive engineering, with the aim of providing guidelines for increasing the <em>V</em><sub>OC</sub> of WPSCs. Finally, we will provide a conclusive outlook on WPSCs, sharing our perspectives to inspire further advancements in both WPSCs and PTSCs.</div></div>","PeriodicalId":67,"journal":{"name":"Chemical Communications","volume":"61 6","pages":"Pages 1063-1086"},"PeriodicalIF":4.2000,"publicationDate":"2024-12-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"A review: strategies for reducing the open-circuit voltage loss of wide-bandgap perovskite solar cells\",\"authors\":\"Lu-Yao Chen , Qi Sun , Yue-Min Xie , Man-Keung Fung\",\"doi\":\"10.1039/d4cc05131a\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Perovskite-based tandem solar cells (PTSCs) have made remarkable achievements in recent years, and the highest certified power conversion efficiency (PCE) of 33.9% has been achieved in perovskite/silicon tandem solar cells (PSTSCs), indicating their great commercialization potential. Nevertheless, the performance of PTSCs continues to be hindered by the compromised performance of wide-bandgap perovskite solar cells (WPSCs), particularly the high <em>V</em><sub>OC</sub> deficit of WPSCs. Therefore, numerous strategies have been developed to minimize the <em>V</em><sub>OC</sub> loss of WPSCs. Herein, we sort to comprehensively review about the reported studies on reducing the <em>V</em><sub>OC</sub> deficit of WPSCs, focusing on interface modification, charge transport material (CTM) exploration, and additive engineering, with the aim of providing guidelines for increasing the <em>V</em><sub>OC</sub> of WPSCs. Finally, we will provide a conclusive outlook on WPSCs, sharing our perspectives to inspire further advancements in both WPSCs and PTSCs.</div></div>\",\"PeriodicalId\":67,\"journal\":{\"name\":\"Chemical Communications\",\"volume\":\"61 6\",\"pages\":\"Pages 1063-1086\"},\"PeriodicalIF\":4.2000,\"publicationDate\":\"2024-12-13\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Chemical Communications\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://www.sciencedirect.com/org/science/article/pii/S1359734524027149\",\"RegionNum\":2,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Chemical Communications","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/org/science/article/pii/S1359734524027149","RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
A review: strategies for reducing the open-circuit voltage loss of wide-bandgap perovskite solar cells
Perovskite-based tandem solar cells (PTSCs) have made remarkable achievements in recent years, and the highest certified power conversion efficiency (PCE) of 33.9% has been achieved in perovskite/silicon tandem solar cells (PSTSCs), indicating their great commercialization potential. Nevertheless, the performance of PTSCs continues to be hindered by the compromised performance of wide-bandgap perovskite solar cells (WPSCs), particularly the high VOC deficit of WPSCs. Therefore, numerous strategies have been developed to minimize the VOC loss of WPSCs. Herein, we sort to comprehensively review about the reported studies on reducing the VOC deficit of WPSCs, focusing on interface modification, charge transport material (CTM) exploration, and additive engineering, with the aim of providing guidelines for increasing the VOC of WPSCs. Finally, we will provide a conclusive outlook on WPSCs, sharing our perspectives to inspire further advancements in both WPSCs and PTSCs.
期刊介绍:
ChemComm (Chemical Communications) is renowned as the fastest publisher of articles providing information on new avenues of research, drawn from all the world''s major areas of chemical research.