{"title":"机器学习心理疲劳测量微米厚弹性表皮电子元件(MMMEEE)。","authors":"Haogeng Liu, Haichuan Li, Yexiong Wang, Yan Liu, Lizhi Xiao, Weidong Guo, Yaoguang Lin, Hongteng Wang, Tianqi Wang, Haiwang Yan, Shunkai Lai, Yaofei Chen, Zongxia Mou, Lei Chen, Yunhan Luo, Gui-Shi Liu, Xingcai Zhang","doi":"10.1021/acs.nanolett.4c02474","DOIUrl":null,"url":null,"abstract":"<p><p>Electrophysiological (EP) signals are key biomarkers for monitoring mental fatigue (MF) and general health, but state-of-the-art wearable EP-based MF monitoring systems are bulky and require user-specific, labeled data. Ultrathin epidermal electrodes with high performance are ideal for constructing imperceptive EP sensing systems; however, the lack of a simple and scalable fabrication delays their application in MF recognition. Here, we report a facile, scalable printing-welding-transferring strategy (PWT) for printing μm-thickness micropatterned silver nanowires (AgNWs)/sticky polydimethylsiloxane, welding the AgNWs via plasmonic effect, and transferring the electrode to skin as tattoos. The PWT provides electrodes with conformability, comfort, and stability for EP sensing. Leveraging the facile and scalable PWT, we develop plug-and-play wireless multimodal epidermal electronics integrated with an unsupervised transfer learning (UTL) scheme for MF recognition across various users. The UTL adaptively minimizes the intersubject difference and achieves high accuracy, without demand of expensive computation and labels from target users.</p>","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":" ","pages":"16221-16230"},"PeriodicalIF":9.1000,"publicationDate":"2024-12-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Machine-Learning Mental-Fatigue-Measuring μm-Thick Elastic Epidermal Electronics (MMMEEE).\",\"authors\":\"Haogeng Liu, Haichuan Li, Yexiong Wang, Yan Liu, Lizhi Xiao, Weidong Guo, Yaoguang Lin, Hongteng Wang, Tianqi Wang, Haiwang Yan, Shunkai Lai, Yaofei Chen, Zongxia Mou, Lei Chen, Yunhan Luo, Gui-Shi Liu, Xingcai Zhang\",\"doi\":\"10.1021/acs.nanolett.4c02474\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>Electrophysiological (EP) signals are key biomarkers for monitoring mental fatigue (MF) and general health, but state-of-the-art wearable EP-based MF monitoring systems are bulky and require user-specific, labeled data. Ultrathin epidermal electrodes with high performance are ideal for constructing imperceptive EP sensing systems; however, the lack of a simple and scalable fabrication delays their application in MF recognition. Here, we report a facile, scalable printing-welding-transferring strategy (PWT) for printing μm-thickness micropatterned silver nanowires (AgNWs)/sticky polydimethylsiloxane, welding the AgNWs via plasmonic effect, and transferring the electrode to skin as tattoos. The PWT provides electrodes with conformability, comfort, and stability for EP sensing. Leveraging the facile and scalable PWT, we develop plug-and-play wireless multimodal epidermal electronics integrated with an unsupervised transfer learning (UTL) scheme for MF recognition across various users. The UTL adaptively minimizes the intersubject difference and achieves high accuracy, without demand of expensive computation and labels from target users.</p>\",\"PeriodicalId\":53,\"journal\":{\"name\":\"Nano Letters\",\"volume\":\" \",\"pages\":\"16221-16230\"},\"PeriodicalIF\":9.1000,\"publicationDate\":\"2024-12-25\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nano Letters\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1021/acs.nanolett.4c02474\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"2024/11/27 0:00:00\",\"PubModel\":\"Epub\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Letters","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acs.nanolett.4c02474","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2024/11/27 0:00:00","PubModel":"Epub","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
摘要
电生理(EP)信号是监测精神疲劳(MF)和一般健康状况的关键生物标志物,但最先进的基于电生理信号的可穿戴式精神疲劳监测系统十分笨重,而且需要用户特定的标记数据。具有高性能的超薄表皮电极是构建无感知 EP 传感系统的理想选择;然而,由于缺乏简单且可扩展的制造方法,它们在中频识别中的应用受到了延误。在此,我们报告了一种简便、可扩展的印刷-焊接-转移策略(PWT),用于印刷微米厚的微图案银纳米线(AgNWs)/粘性聚二甲基硅氧烷,通过等离子效应焊接 AgNWs,并将电极作为纹身转移到皮肤上。PWT 为 EP 传感提供了具有保形性、舒适性和稳定性的电极。利用简便且可扩展的PWT,我们开发了即插即用的无线多模态表皮电子器件,并集成了无监督转移学习(UTL)方案,用于识别不同用户的中频。UTL能自适应地最小化受试者间的差异,并实现高准确度,而无需昂贵的计算和目标用户的标签。
Electrophysiological (EP) signals are key biomarkers for monitoring mental fatigue (MF) and general health, but state-of-the-art wearable EP-based MF monitoring systems are bulky and require user-specific, labeled data. Ultrathin epidermal electrodes with high performance are ideal for constructing imperceptive EP sensing systems; however, the lack of a simple and scalable fabrication delays their application in MF recognition. Here, we report a facile, scalable printing-welding-transferring strategy (PWT) for printing μm-thickness micropatterned silver nanowires (AgNWs)/sticky polydimethylsiloxane, welding the AgNWs via plasmonic effect, and transferring the electrode to skin as tattoos. The PWT provides electrodes with conformability, comfort, and stability for EP sensing. Leveraging the facile and scalable PWT, we develop plug-and-play wireless multimodal epidermal electronics integrated with an unsupervised transfer learning (UTL) scheme for MF recognition across various users. The UTL adaptively minimizes the intersubject difference and achieves high accuracy, without demand of expensive computation and labels from target users.
期刊介绍:
Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including:
- Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale
- Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies
- Modeling and simulation of synthetic, assembly, and interaction processes
- Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance
- Applications of nanoscale materials in living and environmental systems
Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.