通过多键协同作用构建的 PVA/壳聚糖基多功能水凝胶及其在柔性传感器中的应用

IF 10.7 1区 化学 Q1 CHEMISTRY, APPLIED
Tiantian Wang , Bingbing Xu , Tong Yu , Yan Yu , Jiayi Fu , Yuhang Wang , Xianwu Gao , Zhebin Xue , Ruoxin Li , Guangtao Chang
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引用次数: 0

摘要

水凝胶作为柔性可穿戴设备的理想材料,已经引起了人们的极大兴趣。然而,开发多功能水凝胶仍是一大挑战。在这项研究中,我们制备了一种基于聚乙烯醇(PVA)和壳聚糖(CS)的多功能水凝胶,其特点是强度高、导电性好、耐冷冻和保水。该水凝胶配方采用了对羧基苯硼酸(PBA)和 MXene,并结合了冻融循环和甘油(GL)浸泡技术。此外,我们还探索了这种水凝胶在运动检测和传感方面的应用。研究结果表明,该水凝胶具有优异的机械性能,强度高达 3.42 兆帕,模量和韧性分别是纯 PVA 水凝胶的 7 倍和 5 倍。此外,当 MXene 的分散度为 8 Vol% 时,其电导率为 163.15 mS/m,我们探索了其在应变传感(GF = 7.03)和运动检测方面的应用。该水凝胶具有良好的应变范围(600 %)和快速响应时间(42 毫秒),并在关节和呼吸处显示出规则而稳定的电信号,为该水凝胶在智能可穿戴柔性领域的应用提供了战略支持。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

PVA/chitosan-based multifunctional hydrogels constructed through multi-bonding synergies and their application in flexible sensors

PVA/chitosan-based multifunctional hydrogels constructed through multi-bonding synergies and their application in flexible sensors
Hydrogels have garnered significant interest as promising materials for flexible wearable devices. However, it remains a major challenge to develop multifunctional hydrogels. In this study, we prepared a multifunctional hydrogel based on the polyvinyl alcohol (PVA) and chitosan (CS), which is characterized by high strength, good electrical conductivity, and resistance to freezing and water retention. The hydrogel formulation utilizes p-carboxyphenylboronic acid (PBA) and MXene in combination with freeze-thaw cycling and glycerin (GL) immersion technology. Additionally, we explored the applications of this hydrogel in motion detection and sensing. Research results indicate that the hydrogel has excellent mechanical properties, achieving a strength of up to 3.42 MPa, with modulus and toughness improved by 7 times and 5 times, respectively, compared to pure PVA hydrogels. Moreover, when the MXene dispersion is at 8 vol%, the conductivity is 163.15 mS/m, and we explore their applications in strain sensing (GF = 7.03) and motion detection. The hydrogels exhibit a good strain range (600 %) and a fast response time (42 ms), as well as regular and stable electrical signals demonstrated at joints and breathing, providing strategic support for the application of this hydrogel in the field of smart wearable flexibility.
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来源期刊
Carbohydrate Polymers
Carbohydrate Polymers 化学-高分子科学
CiteScore
22.40
自引率
8.00%
发文量
1286
审稿时长
47 days
期刊介绍: Carbohydrate Polymers stands as a prominent journal in the glycoscience field, dedicated to exploring and harnessing the potential of polysaccharides with applications spanning bioenergy, bioplastics, biomaterials, biorefining, chemistry, drug delivery, food, health, nanotechnology, packaging, paper, pharmaceuticals, medicine, oil recovery, textiles, tissue engineering, wood, and various aspects of glycoscience. The journal emphasizes the central role of well-characterized carbohydrate polymers, highlighting their significance as the primary focus rather than a peripheral topic. Each paper must prominently feature at least one named carbohydrate polymer, evident in both citation and title, with a commitment to innovative research that advances scientific knowledge.
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