金属有机框架电纺纳米纤维在纺织废水染料去除中的应用:综述

IF 7.4 2区 工程技术 Q1 ENGINEERING, CHEMICAL
Anastasia Silina, Ahmida El Achari, Fabien Salaün
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引用次数: 0

摘要

纺织业废水中的染料排放量逐年增加。染料在环境中持久存在或分解,通过自然界的水循环进入饮用水,对人类健康造成严重危害。研究人员已经研究并提出了各种废水处理技术来减少染料的排放,其中吸附技术似乎是最经济、最省时的技术。金属有机框架(MOFs)是一种吸附材料,因其具有高比表面积、孔径和体积可调性而被广泛应用。在染料去除方面,MOFs 仅用于批量实验,这阻碍了其在工业规模上的应用。在本综述中,我们将讨论如何全面了解 MOF 合成的最新策略,重点关注染料的有效吸附。通过实例介绍了 MOF 与染料之间最常见的相互作用,并试图了解表面电荷和尺寸相容性对吸附过程的贡献。此外,本研究还详细介绍了将 MOF 纳入电纺纳米纤维 (ENF) 载体的策略,并举例说明了 MOF/ENF 复合材料在吸附纺织污水中的染料方面的有效应用。研究强调,染料与 MOF 的相互作用是 MOF/ENF 吸附染料的主要原因。文章广泛讨论了 MOF/ENF 目前在工业纺织废水处理中应用的局限性,包括技术和环境问题。这些局限性需要在商业化之前加以解决,我们建议开展一些研究来解决这一问题。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Metal-organic framework electrospun nanofibers in application to dye removal from textile wastewaters: A review
Emissions of dyes with wastewater from textile industries are increasing every year. Dyes, persisting or decomposing in the environment, enter drinking water through nature's water cycle and can cause severe problems to human health. Researchers have investigated and proposed various wastewater treatment techniques to reduce dyes' emissions, including adsorption, which appears to be the most cost- and time-effective. Metal-organic frameworks (MOFs) are adsorption materials used for many applications for their high specific surface area, pore size, and volume tunability. In dye removal, MOFs are used exceptionally in batch experiments, which hinders their application on an industrial scale. In this review, a comprehensive understanding of the most recent strategies for MOF synthesis is discussed with a focus on effective adsorption of dyes. The most considered interactions between MOFs and dyes are presented with examples and an endeavor is made to understand the contribution of surface charge and size compatibility to adsorption process. Furthermore, the present survey presents the strategies for incorporation of MOF into electrospun nanofiber (ENF) carriers in detail and demonstrates examples of MOF/ENF composite’s effective application towards the adsorption of dye in textile effluents. It is highlighted that dye-MOF interactions are mostly responsible for the dye adsorption process on MOF/ENF. Current limitations of MOF/ENF application in industrial textile wastewater treatment are extensively discussed and include technical and environmental concerns. These limitations need to be resolved before commercialization, and we suggest a number of studies that can be conducted to address this issue.
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来源期刊
Journal of Environmental Chemical Engineering
Journal of Environmental Chemical Engineering Environmental Science-Pollution
CiteScore
11.40
自引率
6.50%
发文量
2017
审稿时长
27 days
期刊介绍: The Journal of Environmental Chemical Engineering (JECE) serves as a platform for the dissemination of original and innovative research focusing on the advancement of environmentally-friendly, sustainable technologies. JECE emphasizes the transition towards a carbon-neutral circular economy and a self-sufficient bio-based economy. Topics covered include soil, water, wastewater, and air decontamination; pollution monitoring, prevention, and control; advanced analytics, sensors, impact and risk assessment methodologies in environmental chemical engineering; resource recovery (water, nutrients, materials, energy); industrial ecology; valorization of waste streams; waste management (including e-waste); climate-water-energy-food nexus; novel materials for environmental, chemical, and energy applications; sustainability and environmental safety; water digitalization, water data science, and machine learning; process integration and intensification; recent developments in green chemistry for synthesis, catalysis, and energy; and original research on contaminants of emerging concern, persistent chemicals, and priority substances, including microplastics, nanoplastics, nanomaterials, micropollutants, antimicrobial resistance genes, and emerging pathogens (viruses, bacteria, parasites) of environmental significance.
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