将 MXene 基材料作为吸附剂、光催化剂、膜和传感器，用于检测和去除新出现的污染物和气态污染物：全面综述

IF 5.3 2区化学 Q2 CHEMISTRY, MULTIDISCIPLINARY

Arabian Journal of Chemistry Pub Date : 2024-11-06 DOI:10.1016/j.arabjc.2024.106052

Mohammad Hadi Dehghani , Nadeem Hussain Solangi , Nabisab Mujawar Mubarak , Natarajan Rajamohan , Subrajit Bosu , Amina Othmani , Md. Ahmaruzzaman , Soumya Ranjan Mishra , Baishali Bhattacharjee , Vishal Gadore , Talib Hussain Banglani , Nawab Waris , Ali hyder , Ayaz Ali Memon , Khalid Hussain Thebo , Payal Joshi , Grzegorz Boczkaj , Rama Rao Karri

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引用次数: 0

摘要

作为应对各种环境挑战的潜在解决方案，二维材料备受关注。石墨烯、二硫化钼、MXenes 和氮化硼已成为这些材料中最受欢迎的候选材料。本文全面回顾和讨论了 MXenes 在环境工程中的新兴应用。作为未来的吸附材料，MXenes 已展现出巨大的潜力。事实证明，它们能通过吸附现象高效去除新出现的污染物（重金属和有机污染物）。已证实 MXenes 能有效去除铅 (Pb2+)、铬 (Cr6+)、铜 (Cu2+)、铀 (U6+) 和汞 (Hg2+)，其吸附容量在 100 至 250 mg g-1 之间。此外，MXenes 还能有效去除多种放射性核素，包括铀、铕、锶、钡和钍。事实证明，通过吸附新出现的有机污染物，MXenes 在水处理方面具有很高的效率，甚至可以吸附亚甲基蓝、酸性蓝、刚果红、甲基橙和罗丹明 B（RhB）等各种有机染料。此外，MXenes 在吸附氯唑西林 (CLX)、氨苄西林 (AMP)、阿莫西林 (AMX)、环丙沙星 (CPX)、阿米替林 (AMT)、维拉帕米 (VRP)、卡马西平 (CBM)、17 α-炔雌醇、布洛芬 (IBP) 和双氯芬酸 (DCF) 等多种药物方面也表现出很高的处理性能。总的来说，MXenes 具有多种优势，如良好的导电性、热性能、高表面积和分子间相互作用的选择性。不过，在应用时需要对其环境影响和生命周期评估进行全面评估。

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MXene-based materials as adsorbents, photocatalysts, membranes and sensors for detection and removal of emerging and gaseous pollutants: A comprehensive review

2D materials have garnered significant attention as potential solutions to various environmental challenges. Graphene, molybdenum disulfide, MXenes, and boron nitride have emerged as the most popular candidates among these materials. This article presents a comprehensive review and discussion on the emerging applications of MXenes in environmental engineering. MXenes have demonstrated immense potential as future materials for adsorption purposes. They have proven to be highly effective in removing emerging pollutants (heavy metals and organic pollutants) through the adsorption phenomenon. The effectiveness of MXenes in removing lead (Pb²⁺), chromium (Cr⁶⁺), copper (Cu²⁺), uranium (U⁶⁺), and mercury (Hg²⁺) has been confirmed, with a sorption capacity ranging from 100 to 250 mg g⁻¹. Furthermore, MXenes have effectively removed several radionuclides, including uranium, europium, strontium, barium, and thorium. MXenes have proven to be highly efficient in treating water through adsorption in emerging organic pollutants, even for various organic dyes such as methylene blue, acid blue, congo red, methyl orange, and rhodamine B (RhB). Additionally, MXenes exhibit high treatment performance in adsorbing several pharmaceuticals like cloxacillin (CLX), ampicillin (AMP), amoxicillin (AMX), ciprofloxacin (CPX), amitriptyline (AMT), verapamil (VRP), carbamazepine (CBM), 17 α-ethinyl estradiol, ibuprofen (IBP), and diclofenac (DCF). Overall, MXenes offer several advantages, such as good conductivity, thermal performance, high surface area, and selectivity of intermolecular interactions. However, their application requires thoroughly evaluating their environmental impact and life cycle assessment.

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来源期刊

Arabian Journal of Chemistry CHEMISTRY, MULTIDISCIPLINARY-

CiteScore

10.80

自引率

3.30%

发文量

763

审稿时长

63 days

期刊介绍： The Arabian Journal of Chemistry is an English language, peer-reviewed scholarly publication in the area of chemistry. The Arabian Journal of Chemistry publishes original papers, reviews and short reports on, but not limited to: inorganic, physical, organic, analytical and biochemistry. The Arabian Journal of Chemistry is issued by the Arab Union of Chemists and is published by King Saud University together with the Saudi Chemical Society in collaboration with Elsevier and is edited by an international group of eminent researchers.