{"title":"丽水国家石化工业综合体中导致氧化潜能的 PM2.5 和气态污染物主要来源的识别:PMF 模型的启示","authors":"Seoyeong Choe, Geun-Hye Yu, Myoungki Song, Sea-Ho Oh, Hajeong Jeon, Dong-Hoon Ko, Chaehyeong Park, Min-Suk Bae","doi":"10.1016/j.atmosenv.2024.120943","DOIUrl":null,"url":null,"abstract":"<div><div>This investigation seeks to characterize and pinpoint the sources of PM<sub>2.5</sub> and various gaseous pollutants within the Yeosu National Industrial Complex by employing the source apportionment model. PM<sub>2.5</sub> samples were gathered at 3-h intervals during various seasons using both quartz and Teflon filters, and subjected to chemical composition analysis. The mean PM<sub>2.5</sub> concentration was recorded at 22.8 μg/m³, with elevated levels observed during the winter. The source analysis delineated 5 p.m.<sub>2.5</sub> sources, featuring combinations of EC, Pb, Ni, Cu, and OC. Gaseous pollutants were categorized into CO, CO<sub>2</sub>, Chloroform, Isopropylbenzene & Chlorobenzene, Dichlorobenzene, and Vehicle emissions. Conditional Probability Functions analysis revealed various source inflow directions, predominantly influenced by the nearby industrial complex. The dithiothreitol assay-oxidative potential normalized to 9,10-phenanthrenequinone (QDTT-OP) of PM<sub>2.5</sub> demonstrated significant correlations with primary emission sources, particularly EC and Pb, due to incomplete combustion processes. Effectively managing these emissions is essential for mitigating health risks related to air pollution. This research offers crucial information for the formulation of strategies aimed at enhancing air quality and public health in industrialized regions.</div></div>","PeriodicalId":250,"journal":{"name":"Atmospheric Environment","volume":"342 ","pages":"Article 120943"},"PeriodicalIF":4.2000,"publicationDate":"2024-11-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Identification of major sources of PM2.5 and gaseous pollutants contributing to oxidative potential in the Yeosu national petrochemical industrial complex: Insights from the PMF model\",\"authors\":\"Seoyeong Choe, Geun-Hye Yu, Myoungki Song, Sea-Ho Oh, Hajeong Jeon, Dong-Hoon Ko, Chaehyeong Park, Min-Suk Bae\",\"doi\":\"10.1016/j.atmosenv.2024.120943\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>This investigation seeks to characterize and pinpoint the sources of PM<sub>2.5</sub> and various gaseous pollutants within the Yeosu National Industrial Complex by employing the source apportionment model. PM<sub>2.5</sub> samples were gathered at 3-h intervals during various seasons using both quartz and Teflon filters, and subjected to chemical composition analysis. The mean PM<sub>2.5</sub> concentration was recorded at 22.8 μg/m³, with elevated levels observed during the winter. The source analysis delineated 5 p.m.<sub>2.5</sub> sources, featuring combinations of EC, Pb, Ni, Cu, and OC. Gaseous pollutants were categorized into CO, CO<sub>2</sub>, Chloroform, Isopropylbenzene & Chlorobenzene, Dichlorobenzene, and Vehicle emissions. Conditional Probability Functions analysis revealed various source inflow directions, predominantly influenced by the nearby industrial complex. The dithiothreitol assay-oxidative potential normalized to 9,10-phenanthrenequinone (QDTT-OP) of PM<sub>2.5</sub> demonstrated significant correlations with primary emission sources, particularly EC and Pb, due to incomplete combustion processes. Effectively managing these emissions is essential for mitigating health risks related to air pollution. This research offers crucial information for the formulation of strategies aimed at enhancing air quality and public health in industrialized regions.</div></div>\",\"PeriodicalId\":250,\"journal\":{\"name\":\"Atmospheric Environment\",\"volume\":\"342 \",\"pages\":\"Article 120943\"},\"PeriodicalIF\":4.2000,\"publicationDate\":\"2024-11-20\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Atmospheric Environment\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S1352231024006186\",\"RegionNum\":2,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENVIRONMENTAL SCIENCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Atmospheric Environment","FirstCategoryId":"93","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1352231024006186","RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENVIRONMENTAL SCIENCES","Score":null,"Total":0}
Identification of major sources of PM2.5 and gaseous pollutants contributing to oxidative potential in the Yeosu national petrochemical industrial complex: Insights from the PMF model
This investigation seeks to characterize and pinpoint the sources of PM2.5 and various gaseous pollutants within the Yeosu National Industrial Complex by employing the source apportionment model. PM2.5 samples were gathered at 3-h intervals during various seasons using both quartz and Teflon filters, and subjected to chemical composition analysis. The mean PM2.5 concentration was recorded at 22.8 μg/m³, with elevated levels observed during the winter. The source analysis delineated 5 p.m.2.5 sources, featuring combinations of EC, Pb, Ni, Cu, and OC. Gaseous pollutants were categorized into CO, CO2, Chloroform, Isopropylbenzene & Chlorobenzene, Dichlorobenzene, and Vehicle emissions. Conditional Probability Functions analysis revealed various source inflow directions, predominantly influenced by the nearby industrial complex. The dithiothreitol assay-oxidative potential normalized to 9,10-phenanthrenequinone (QDTT-OP) of PM2.5 demonstrated significant correlations with primary emission sources, particularly EC and Pb, due to incomplete combustion processes. Effectively managing these emissions is essential for mitigating health risks related to air pollution. This research offers crucial information for the formulation of strategies aimed at enhancing air quality and public health in industrialized regions.
期刊介绍:
Atmospheric Environment has an open access mirror journal Atmospheric Environment: X, sharing the same aims and scope, editorial team, submission system and rigorous peer review.
Atmospheric Environment is the international journal for scientists in different disciplines related to atmospheric composition and its impacts. The journal publishes scientific articles with atmospheric relevance of emissions and depositions of gaseous and particulate compounds, chemical processes and physical effects in the atmosphere, as well as impacts of the changing atmospheric composition on human health, air quality, climate change, and ecosystems.