基于 MXene 的材料在电化学检测酚类污染物方面的多功能性

IF 20.3 1区 化学 Q1 CHEMISTRY, INORGANIC & NUCLEAR
Reddicherla Umapathi , Chikkili Venkateswara Raju , Moein Safarkhani , Jebiti Haribabu , Hyun Uk Lee , Gokana Mohana Rani , Yun Suk Huh
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引用次数: 0

摘要

酚类污染物是最令人担忧的环境污染物之一,严重威胁人类健康和生态环境。为防止对水生环境和空气质量造成危害,需要对有害酚类污染物进行有效处理。因此,迫切需要一种有效且易于操作的传感平台来快速检测有害酚类污染物。电化学传感器被认为是有效的传感平台,最近取得的重大进展就是明证。具有特殊多功能性和结构的先进纳米材料是提高灵敏度、检测、准确性和选择性的理想电极材料。MXenes 是一种创新的二维(2D)层状材料,由过渡金属氮化物、碳化物和碳氮化物组成。在所有合成二维材料中,MXenes 的导电率最高。由于其独特的性能,它们已成为电化学(生物)传感应用中用途广泛的重要材料。基于二氧化二烯的复合材料具有良好的物理化学和电化学特性,在电化学检测各种有害污染物方面表现出卓越的传感性能。本研究系统、协同地回顾了 MXene 基复合材料在酚类污染物电化学检测方面的最新进展。重点研究了酚类化合物的毒性效应。全面介绍了用于酚类污染物电化学检测的基于 MXene 的复合材料的电极制造、传感机理、电分析性能和多功能性。最后,我们讨论了设计和开发高性能电化学传感器所面临的挑战和未来前景,预计这将为酚类污染物检测传感策略的新途径铺平道路。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Versatility of MXene based materials for the electrochemical detection of phenolic contaminants

Versatility of MXene based materials for the electrochemical detection of phenolic contaminants
Phenolic contaminants are among the most concerning environmental pollutants that seriously threaten human health and ecological environment. Effective treatment of hazardous phenolic pollutants is required to prevent harm to aquatic environments and air quality. Hence, there is an urgent need for an effective and easy-to-operate sensing platform for rapid detection of hazardous phenolic contaminants. Electrochemical sensors are considered effective sensing platforms, as evidenced by significant recent advancements. Advanced nanomaterials with exceptional multifunctionalities and structures are ideal electrode materials for enhancing sensitivity, detection, accuracy, and selectivity. MXenes are innovative two-dimensional (2D) layered materials comprising transition metal nitrides, carbides, and carbon–nitrides. MXenes demonstrated highest electrical conductivity among all synthetic 2D materials. Due to their unique properties, they have emerged as versatile and substantial materials for electrochemical (bio)sensing applications. MXene-based composites with good physicochemical and electrochemical properties have demonstrated excellent sensing behavior for the electrochemical detection of various hazardous contaminants. This study systematically and synergistically reviewed the recent progress in MXene-based composites for the electrochemical detection of phenolic contaminants. Focused on toxic effects of phenolic compounds. Comprehensive information was provided on the electrode fabrication, sensing mechanism, electroanalytical performance, and versatility of MXene based composite materials for electrochemical sensing of phenolic contaminants. Finally, we discussed the challenges and future perspectives for the design and development of high-performance electrochemical sensors, which are expected to pave the way for novel pathways in sensing strategies for the detection of phenolic contaminants.
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来源期刊
Coordination Chemistry Reviews
Coordination Chemistry Reviews 化学-无机化学与核化学
CiteScore
34.30
自引率
5.30%
发文量
457
审稿时长
54 days
期刊介绍: Coordination Chemistry Reviews offers rapid publication of review articles on current and significant topics in coordination chemistry, encompassing organometallic, supramolecular, theoretical, and bioinorganic chemistry. It also covers catalysis, materials chemistry, and metal-organic frameworks from a coordination chemistry perspective. Reviews summarize recent developments or discuss specific techniques, welcoming contributions from both established and emerging researchers. The journal releases special issues on timely subjects, including those featuring contributions from specific regions or conferences. Occasional full-length book articles are also featured. Additionally, special volumes cover annual reviews of main group chemistry, transition metal group chemistry, and organometallic chemistry. These comprehensive reviews are vital resources for those engaged in coordination chemistry, further establishing Coordination Chemistry Reviews as a hub for insightful surveys in inorganic and physical inorganic chemistry.
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