{"title":"利用热解和前驱体渗透技术加强通过 3D 打印制造的碳化硅陶瓷结构的完整性","authors":"Manojit Das*, Arijit Jana, Karthik R, Rishabh Swarnkar, Astha Dixit, Sushanta Kumar Panda, Shobhit Kumar, Renjith Devasia* and Chandra Sekhar Tiwary*, ","doi":"10.1021/acsaenm.4c0047510.1021/acsaenm.4c00475","DOIUrl":null,"url":null,"abstract":"<p >3D printing, particularly direct ink writing (DIW), offers a different approach to crafting intricate ceramic structures. Here, 3D printing technology (direct ink writing (DIW)) based on extrusion has been utilized to fabricate SiC ceramic structures. The particle size, binder composition, and printing conditions were optimized to fabricate high-strength green structures. The mechanical properties of the 3D-printed SiC green structure were infiltrated with the liquid precursor, which filled the porous part of the structure. The composite is fired at a higher temperature, which results in the formation of SiC from the liquid precursor, demonstrating improved surface morphology, strength, density, and thermal properties of the printed structures. The 3D-printed SiC composite structures show an increase in mechanical strength up to 600% stronger as compared to the pristine SiC structures. Furthermore, the infiltrated, sintered composite demonstrates superior thermal properties, notably improved heat dissipation, in contrast to noninfiltrated samples, rendering it well-suited for high-temperature applications. This method presents a promising avenue for manufacturing advanced SiC components with superior properties.</p>","PeriodicalId":55639,"journal":{"name":"ACS Applied Engineering Materials","volume":"2 11","pages":"2549–2558 2549–2558"},"PeriodicalIF":0.0000,"publicationDate":"2024-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Strengthening SiC Ceramic Structural Integrity Made via 3D Printing with Pyrolysis and Precursor Infiltration\",\"authors\":\"Manojit Das*, Arijit Jana, Karthik R, Rishabh Swarnkar, Astha Dixit, Sushanta Kumar Panda, Shobhit Kumar, Renjith Devasia* and Chandra Sekhar Tiwary*, \",\"doi\":\"10.1021/acsaenm.4c0047510.1021/acsaenm.4c00475\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >3D printing, particularly direct ink writing (DIW), offers a different approach to crafting intricate ceramic structures. Here, 3D printing technology (direct ink writing (DIW)) based on extrusion has been utilized to fabricate SiC ceramic structures. The particle size, binder composition, and printing conditions were optimized to fabricate high-strength green structures. The mechanical properties of the 3D-printed SiC green structure were infiltrated with the liquid precursor, which filled the porous part of the structure. The composite is fired at a higher temperature, which results in the formation of SiC from the liquid precursor, demonstrating improved surface morphology, strength, density, and thermal properties of the printed structures. The 3D-printed SiC composite structures show an increase in mechanical strength up to 600% stronger as compared to the pristine SiC structures. Furthermore, the infiltrated, sintered composite demonstrates superior thermal properties, notably improved heat dissipation, in contrast to noninfiltrated samples, rendering it well-suited for high-temperature applications. This method presents a promising avenue for manufacturing advanced SiC components with superior properties.</p>\",\"PeriodicalId\":55639,\"journal\":{\"name\":\"ACS Applied Engineering Materials\",\"volume\":\"2 11\",\"pages\":\"2549–2558 2549–2558\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2024-11-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Applied Engineering Materials\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acsaenm.4c00475\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Engineering Materials","FirstCategoryId":"1085","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsaenm.4c00475","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
Strengthening SiC Ceramic Structural Integrity Made via 3D Printing with Pyrolysis and Precursor Infiltration
3D printing, particularly direct ink writing (DIW), offers a different approach to crafting intricate ceramic structures. Here, 3D printing technology (direct ink writing (DIW)) based on extrusion has been utilized to fabricate SiC ceramic structures. The particle size, binder composition, and printing conditions were optimized to fabricate high-strength green structures. The mechanical properties of the 3D-printed SiC green structure were infiltrated with the liquid precursor, which filled the porous part of the structure. The composite is fired at a higher temperature, which results in the formation of SiC from the liquid precursor, demonstrating improved surface morphology, strength, density, and thermal properties of the printed structures. The 3D-printed SiC composite structures show an increase in mechanical strength up to 600% stronger as compared to the pristine SiC structures. Furthermore, the infiltrated, sintered composite demonstrates superior thermal properties, notably improved heat dissipation, in contrast to noninfiltrated samples, rendering it well-suited for high-temperature applications. This method presents a promising avenue for manufacturing advanced SiC components with superior properties.
期刊介绍:
ACS Applied Engineering Materials is an international and interdisciplinary forum devoted to original research covering all aspects of engineered materials complementing the ACS Applied Materials portfolio. Papers that describe theory simulation modeling or machine learning assisted design of materials and that provide new insights into engineering applications are welcomed. The journal also considers experimental research that includes novel methods of preparing characterizing and evaluating new materials designed for timely applications. With its focus on innovative applications ACS Applied Engineering Materials also complements and expands the scope of existing ACS publications that focus on materials science discovery including Biomacromolecules Chemistry of Materials Crystal Growth & Design Industrial & Engineering Chemistry Research Inorganic Chemistry Langmuir and Macromolecules.The scope of ACS Applied Engineering Materials includes high quality research of an applied nature that integrates knowledge in materials science engineering physics mechanics and chemistry.