利用木材化学标记在区域范围内追踪木材的起源:元素、锶和钕的同位素组成。

IF 8.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES
Science of the Total Environment Pub Date : 2024-12-20 Epub Date: 2024-11-29 DOI:10.1016/j.scitotenv.2024.177640
Anna Imbert Štulc, Anne Poszwa, Stéphane Ponton, Jean-Luc Dupouey, Julien Bouchez, Maximilien Beuret, Dimitri Rigoussen, Thierry Paul, Michel Lemoine, Sylvie Coubray, Olivier Girardclos, Christophe Gauthier, Jérémie Bardin, Thanh Thuy Nguyen Tu, Alexa Dufraisse
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引用次数: 0

摘要

树枝化学方法在确定木材的地理来源方面大有可为,是基于树环宽度的树枝起源研究的补充工具。根据木材的元素和同位素组成追踪木材的来源,对于区域范围内的产地研究特别有意义,因为树枝化学特征表明了地质和土壤学特征。虽然养分和微量元素的吸收反映了土壤生物可利用库的组成,但它也受到多种环境和树木相关因素的影响。我们评估了栎木产地研究中的树枝化学方法所面临的挑战:1)局部水平的地球化学变化;2)与栎木种类、树龄和社会地位相关的树枝化学变化。对法国塞纳河流域 12 个森林中的栎木进行了 13 种元素浓度和 2 种同位素(锶和钕)比率的综合分析。取样地点具有代表性的地质母质类型,选取了两种常见的温带栎树(柞树和栎树)的成年树。树木特征的影响明显弱于地点因素的影响,而且考虑到柞树和栎树的树枝化学成分差异极小,对确定地理来源没有影响。基于钙归一化元素浓度以及锶和钕同位素比值的线性判别分析正确划分了 93% 采样树木的原产地。锶同位素比值 87Sr/86Sr 是最强的产地指标,能够单独确定 55% 木材样本的产地。我们基于元素、锶和钕同位素组成的系统为木材追踪提供了可靠的指标,可应用于环境、生理学、历史和考古学方面的来源研究。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Tracing the origin of wood at the regional scale with dendrochemical markers: elemental and strontium and neodymium isotopic composition.

The dendrochemical approach holds significant promise for determining the geographical origin of wood as a complementary tool to dendroprovenancing based on tree-ring width. Tracing the origin of wood based on its elemental and isotopic composition is in particular interesting for provenance studies at the regional scale, as dendrochemical signatures are indicative of geological and pedological characteristics. Although, absorption of nutrients and trace elements reflects the composition of soil bioavailable pools, it is also modulated by multiple environmental and tree related factors. We assess the dendrochemical approach in oak wood provenance studies regarding the challenges posed by 1) geochemical variation at a local level, and 2) dendrochemical variation related to oak species, age and social status. A combination of 13 elemental concentrations and 2 isotope - Sr and Nd - ratios was analyzed in oak wood from 12 forests situated in the large Seine river catchment in France. The sampling targeted sites with representative types of geological parent material, where adult trees of two common temperate Quercus species (Quercus petraea and Quercus robur) were selected. The impact of tree characteristics was markedly weaker than that of the site factor and the minimal differences in dendrochemical composition between Quercus petraea and Quercus robur were considered without effect on determination of the geographical origin. Linear discriminant analysis based on Ca-normalized elemental concentrations and Sr and Nd isotope ratios correctly classified the origin of 93 % of the sampled trees. Strontium isotope ratio 87Sr/86Sr was the strongest provenance indicator capable of determining the origin of 55 % of wood samples on its own. Our system based on elemental and strontium and neodymium isotopic compositions provides robust indicators for wood tracing and might be applied to provenance studies in environment, physiology, history and archeology.

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来源期刊
Science of the Total Environment
Science of the Total Environment 环境科学-环境科学
CiteScore
17.60
自引率
10.20%
发文量
8726
审稿时长
2.4 months
期刊介绍: The Science of the Total Environment is an international journal dedicated to scientific research on the environment and its interaction with humanity. It covers a wide range of disciplines and seeks to publish innovative, hypothesis-driven, and impactful research that explores the entire environment, including the atmosphere, lithosphere, hydrosphere, biosphere, and anthroposphere. The journal's updated Aims & Scope emphasizes the importance of interdisciplinary environmental research with broad impact. Priority is given to studies that advance fundamental understanding and explore the interconnectedness of multiple environmental spheres. Field studies are preferred, while laboratory experiments must demonstrate significant methodological advancements or mechanistic insights with direct relevance to the environment.
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