在光电化学系统中有效利用光生电荷载体：从原子级到配置的工程策略

IF 51.4 1区化学 Q1 CHEMISTRY, MULTIDISCIPLINARY

Chemical Reviews Pub Date : 2024-11-21 DOI:10.1021/acs.chemrev.4c00382

Kai Song, Houjiang Liu, Biao Chen, Chuangchuang Gong, Jiawei Ding, Tengfei Wang, Enzuo Liu, Liying Ma, Naiqin Zhao, Fang He

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引用次数: 0

摘要

光电化学（PEC）系统对于太阳能转换、解决关键的能源和环境问题至关重要。然而，光生电荷载流子的利用效率较低，极大地限制了整体能量转换。因此，人们越来越关注开发提高光电极性能的策略。这篇综述系统地探讨了从原子和纳米层面到配置工程等方面的光致发光系统改造的最新进展。我们深入探讨了 PEC 结构、内在特性、光生成电荷载流子动力学及其利用之间的关系。此外，我们还提出了开发更高效 PEC 系统的未来方向和前景，为该领域的潜在创新提供了宝贵的见解。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

Toward Efficient Utilization of Photogenerated Charge Carriers in Photoelectrochemical Systems: Engineering Strategies from the Atomic Level to Configuration

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Toward Efficient Utilization of Photogenerated Charge Carriers in Photoelectrochemical Systems: Engineering Strategies from the Atomic Level to Configuration

Photoelectrochemical (PEC) systems are essential for solar energy conversion, addressing critical energy and environmental issues. However, the low efficiency in utilizing photogenerated charge carriers significantly limits overall energy conversion. Consequently, there is a growing focus on developing strategies to enhance photoelectrode performance. This review systematically explores recent advancements in PEC system modifications, spanning from atomic and nanoscopic levels to configuration engineering. We delve into the relationships between PEC structures, intrinsic properties, kinetics of photogenerated charge carriers, and their utilization. Additionally, we propose future directions and perspectives for developing more efficient PEC systems, offering valuable insights into potential innovations in the field.

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来源期刊

Chemical Reviews 化学-化学综合

CiteScore

106.00

自引率

1.10%

发文量

278

审稿时长

4.3 months

期刊介绍： Chemical Reviews is a highly regarded and highest-ranked journal covering the general topic of chemistry. Its mission is to provide comprehensive, authoritative, critical, and readable reviews of important recent research in organic, inorganic, physical, analytical, theoretical, and biological chemistry. Since 1985, Chemical Reviews has also published periodic thematic issues that focus on a single theme or direction of emerging research.