烟头的不同剩余部分在酚类化合物向水生环境转移中的作用及其生态风险。

IF 8.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES
Science of the Total Environment Pub Date : 2024-12-20 Epub Date: 2024-11-21 DOI:10.1016/j.scitotenv.2024.177584
Sina Dobaradaran, Amir Salemi, Gabriel E De-la-Torre, Ursula Telgheder, Torsten C Schmidt
{"title":"烟头的不同剩余部分在酚类化合物向水生环境转移中的作用及其生态风险。","authors":"Sina Dobaradaran, Amir Salemi, Gabriel E De-la-Torre, Ursula Telgheder, Torsten C Schmidt","doi":"10.1016/j.scitotenv.2024.177584","DOIUrl":null,"url":null,"abstract":"<p><p>Cigarette butts (CBs), the most prevalent waste material globally, have the potential to leach various toxic substances, including phenolic compounds (PhCs), into the environment and aquatic ecosystems. Nevertheless, there is a lack of knowledge concerning the long-term release of PhCs via the different parts of CBs which are littered into the environment. Hence, the present study was designed to investigate the ecological risk as well as the leachate concentrations of PhCs, including phenol, o-cresol, 2,4-dimethylphenol, pentachlorophenol and 2,3,4,6-tetrachlorophenol via different parts of CBs littered into water at several exposure times. Aged CBs collected from the environment, freshly smoked CBs, filter and paper, and remaining tobacco plus ash of freshly smoked CBs were studied to determine the leachate levels of PhCs. Pentachlorophenol and 2,3,4,6-tetrachlorophenol were not detected and quantified in the leachates of all CB types at all exposure times. The combination of filter and paper from freshly smoked CBs exhibited the highest mass-based leachate levels of phenol, o-cresol, and 2,4-dimethylphenol, whereas aged CBs showed the lowest levels. The mean leachate of phenol, o-cresol, and 2,4-dimethylphenol from all four examined CB types were in the ranges of 0.43-639.56, 0.77-58.61, and 0.25-16.58 μg L<sup>-1</sup> per CB, respectively. The ecological risk assessment showed that PhC leachates via all CB types had high risks for algae, Daphnia magna, and fish. The present study elucidated the release behavior of several PhCs and toxic CB-associated contaminants that have been overlooked in the literature.</p>","PeriodicalId":422,"journal":{"name":"Science of the Total Environment","volume":" ","pages":"177584"},"PeriodicalIF":8.2000,"publicationDate":"2024-12-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"The role of different remaining parts of cigarette butts in the transfer of phenolic compounds into the aquatic environment and their ecological risk.\",\"authors\":\"Sina Dobaradaran, Amir Salemi, Gabriel E De-la-Torre, Ursula Telgheder, Torsten C Schmidt\",\"doi\":\"10.1016/j.scitotenv.2024.177584\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>Cigarette butts (CBs), the most prevalent waste material globally, have the potential to leach various toxic substances, including phenolic compounds (PhCs), into the environment and aquatic ecosystems. Nevertheless, there is a lack of knowledge concerning the long-term release of PhCs via the different parts of CBs which are littered into the environment. Hence, the present study was designed to investigate the ecological risk as well as the leachate concentrations of PhCs, including phenol, o-cresol, 2,4-dimethylphenol, pentachlorophenol and 2,3,4,6-tetrachlorophenol via different parts of CBs littered into water at several exposure times. Aged CBs collected from the environment, freshly smoked CBs, filter and paper, and remaining tobacco plus ash of freshly smoked CBs were studied to determine the leachate levels of PhCs. Pentachlorophenol and 2,3,4,6-tetrachlorophenol were not detected and quantified in the leachates of all CB types at all exposure times. The combination of filter and paper from freshly smoked CBs exhibited the highest mass-based leachate levels of phenol, o-cresol, and 2,4-dimethylphenol, whereas aged CBs showed the lowest levels. The mean leachate of phenol, o-cresol, and 2,4-dimethylphenol from all four examined CB types were in the ranges of 0.43-639.56, 0.77-58.61, and 0.25-16.58 μg L<sup>-1</sup> per CB, respectively. The ecological risk assessment showed that PhC leachates via all CB types had high risks for algae, Daphnia magna, and fish. The present study elucidated the release behavior of several PhCs and toxic CB-associated contaminants that have been overlooked in the literature.</p>\",\"PeriodicalId\":422,\"journal\":{\"name\":\"Science of the Total Environment\",\"volume\":\" \",\"pages\":\"177584\"},\"PeriodicalIF\":8.2000,\"publicationDate\":\"2024-12-20\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Science of the Total Environment\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://doi.org/10.1016/j.scitotenv.2024.177584\",\"RegionNum\":1,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"2024/11/21 0:00:00\",\"PubModel\":\"Epub\",\"JCR\":\"Q1\",\"JCRName\":\"ENVIRONMENTAL SCIENCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Science of the Total Environment","FirstCategoryId":"93","ListUrlMain":"https://doi.org/10.1016/j.scitotenv.2024.177584","RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2024/11/21 0:00:00","PubModel":"Epub","JCR":"Q1","JCRName":"ENVIRONMENTAL SCIENCES","Score":null,"Total":0}
引用次数: 0

摘要

烟头(CBs)是全球最常见的废弃物,有可能向环境和水生生态系统沥滤各种有毒物质,包括酚类化合物(PhCs)。然而,目前还缺乏有关酚类化合物通过烟蒂的不同部分长期释放到环境中的知识。因此,本研究旨在调查在不同暴露时间下,通过丢弃到水中的 CBs 不同部分释放的 PhCs(包括苯酚、邻甲酚、2,4-二甲基苯酚、五氯苯酚和 2,3,4,6-四氯苯酚)的生态风险和沥滤液浓度。研究了从环境中收集的陈年烟草卷烟、新抽的烟草卷烟、过滤纸和纸,以及新抽的烟草卷烟的剩余烟丝和烟灰,以确定浸出液中的 PhCs 含量。在所有接触时间内,所有类型的大麻烟浸出液中均未检测到五氯苯酚和 2,3,4,6- 四氯苯酚,也未对其进行定量。新熏制 CB 的滤纸和纸张组合显示出最高的苯酚、邻甲酚和 2,4-二甲基苯酚浸出物质量水平,而老化 CB 的浸出物水平最低。所有四种受检 CB 的苯酚、邻甲酚和 2,4-二甲基苯酚平均浸出物含量范围分别为 0.43-639.56、0.77-58.61 和 0.25-16.58 μg L-1。生态风险评估结果表明,所有 CB 类型的 PhC 浸出物对藻类、大型水蚤和鱼类的风险都很高。本研究阐明了文献中忽略的几种 PhCs 和有毒 CB 相关污染物的释放行为。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
The role of different remaining parts of cigarette butts in the transfer of phenolic compounds into the aquatic environment and their ecological risk.

Cigarette butts (CBs), the most prevalent waste material globally, have the potential to leach various toxic substances, including phenolic compounds (PhCs), into the environment and aquatic ecosystems. Nevertheless, there is a lack of knowledge concerning the long-term release of PhCs via the different parts of CBs which are littered into the environment. Hence, the present study was designed to investigate the ecological risk as well as the leachate concentrations of PhCs, including phenol, o-cresol, 2,4-dimethylphenol, pentachlorophenol and 2,3,4,6-tetrachlorophenol via different parts of CBs littered into water at several exposure times. Aged CBs collected from the environment, freshly smoked CBs, filter and paper, and remaining tobacco plus ash of freshly smoked CBs were studied to determine the leachate levels of PhCs. Pentachlorophenol and 2,3,4,6-tetrachlorophenol were not detected and quantified in the leachates of all CB types at all exposure times. The combination of filter and paper from freshly smoked CBs exhibited the highest mass-based leachate levels of phenol, o-cresol, and 2,4-dimethylphenol, whereas aged CBs showed the lowest levels. The mean leachate of phenol, o-cresol, and 2,4-dimethylphenol from all four examined CB types were in the ranges of 0.43-639.56, 0.77-58.61, and 0.25-16.58 μg L-1 per CB, respectively. The ecological risk assessment showed that PhC leachates via all CB types had high risks for algae, Daphnia magna, and fish. The present study elucidated the release behavior of several PhCs and toxic CB-associated contaminants that have been overlooked in the literature.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Science of the Total Environment
Science of the Total Environment 环境科学-环境科学
CiteScore
17.60
自引率
10.20%
发文量
8726
审稿时长
2.4 months
期刊介绍: The Science of the Total Environment is an international journal dedicated to scientific research on the environment and its interaction with humanity. It covers a wide range of disciplines and seeks to publish innovative, hypothesis-driven, and impactful research that explores the entire environment, including the atmosphere, lithosphere, hydrosphere, biosphere, and anthroposphere. The journal's updated Aims & Scope emphasizes the importance of interdisciplinary environmental research with broad impact. Priority is given to studies that advance fundamental understanding and explore the interconnectedness of multiple environmental spheres. Field studies are preferred, while laboratory experiments must demonstrate significant methodological advancements or mechanistic insights with direct relevance to the environment.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信