煤制芳烃工艺与干法/蒸汽混合重整相结合:技术经济分析和环境评估

IF 4.1 2区 工程技术 Q2 ENGINEERING, CHEMICAL
Junqiang Zhang , Peng Dong , Haifeng Lei , Ruonan Liu , Junwen Wang , Zhitong Zhao , Wei Zhang
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引用次数: 0

摘要

本研究提出了两种替代煤制芳烃工艺,即甲烷蒸汽转化辅助工艺(NG-CTA-S)和甲烷干法/蒸汽转化集成工艺(NG-CTA-DS),以减少与传统煤制芳烃(CTA)工艺相关的二氧化碳(CO2)排放。本研究对关键参数进行了详细的工艺模拟和优化,以确定碳排放量最低的芳烃生产路线。在进行环境评估的同时,还进行了全面的技术和经济分析,以比较拟议工艺和现有工艺。结果表明,NG-CTA-DS 工艺在技术经济性能和环境评估方面都表现优异。该工艺的碳元素利用率达到 85.95%,能效达到 78.80%,二氧化碳排放量减少了 3.65 千克/千克-芳烃,生产成本仅为 1.01887 亿美元。由此可见,与传统工艺相比,拟议的 NG-CTA-DS 工艺在提高技术、经济和环境性能方面潜力巨大,有望实现工业化。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Coal-to-aromatics process integrated with dry/steam-mixed reforming: Techno-economic analysis and environmental evaluation
Two alternative coal-to-aromatics processes, the methane steam reforming-assisted process (NG-CTA-S) and methane dry/steam reforming-integrated process (NG-CTA-DS), are proposed to mitigate carbon dioxide (CO2) emissions associated with conventional coal-to-aromatics (CTA) processes. This study conducted a detailed process simulation and optimization of key parameters to determine the aromatic production route with the lowest carbon emission. A comprehensive technical and economic analysis, along with an environmental assessment, was carried out to compare the proposed processes with existing ones. The results indicate that the NG-CTA-DS process has demonstrated superior techno-economic performance and environmental evaluation. It achieved an elemental carbon utilization of 85.95 %, an energy efficiency of 78.80 %, a reduced CO2 emission of 3.65 kg/kg-aromatics, and a production cost of only 1018.87 M$. Therefore, it is evident that the proposed NG-CTA-DS process holds significant potential to enhance the technical, economic, and environmental performance compared to the conventional process, making it a promising candidate for industrialization.
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来源期刊
Chemical Engineering Science
Chemical Engineering Science 工程技术-工程:化工
CiteScore
7.50
自引率
8.50%
发文量
1025
审稿时长
50 days
期刊介绍: Chemical engineering enables the transformation of natural resources and energy into useful products for society. It draws on and applies natural sciences, mathematics and economics, and has developed fundamental engineering science that underpins the discipline. Chemical Engineering Science (CES) has been publishing papers on the fundamentals of chemical engineering since 1951. CES is the platform where the most significant advances in the discipline have ever since been published. Chemical Engineering Science has accompanied and sustained chemical engineering through its development into the vibrant and broad scientific discipline it is today.
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