Abdulhalim Musa Abubakar , Lukman Buba Umdagas , Moses NyoTonglo Arowo , Marwea Al-Hedrewy , Mahlon Kida Marvin , Noureddine Elboughdiri , Aminullah Zakariyya Abdul , Jenisus O. Dejarlo , Rezkallah Chafika
{"title":"模拟从湿天然气中同时回收二氧化碳和甜碳中性天然气的系统:对工艺输入和装置性能的深入研究","authors":"Abdulhalim Musa Abubakar , Lukman Buba Umdagas , Moses NyoTonglo Arowo , Marwea Al-Hedrewy , Mahlon Kida Marvin , Noureddine Elboughdiri , Aminullah Zakariyya Abdul , Jenisus O. Dejarlo , Rezkallah Chafika","doi":"10.1016/j.cles.2024.100156","DOIUrl":null,"url":null,"abstract":"<div><div>The growing need for carbon-neutral energy solutions necessitates the development of efficient systems for carbon dioxide (CO<sub>2</sub>) recovery and the production of sweet carbon-neutral natural gas (CNNG) from wet natural gas. Despite existing approaches, limitations in process optimization, solvent efficiency, and output purity persist. This study aims to address these gaps by simulating a system for simultaneous recovery of CO<sub>2</sub> and CNNG using an integrated three-stage process, modeled in Aspen Plus V8.8. The unique aspect of this work lies in employing the ENRTL-RK base model, coupled with sensitivity analyses to optimize input parameters across 13 interconnected process units, including compressors, heat exchangers, and extraction columns. Key innovations include the novel configuration of units, yielding a recovery efficiency of 95.94% for CNNG and a CO<sub>2</sub> purity of 93.185% at optimal conditions, surpassing conventional methods. The performance of the monoethanolamine (MEA) solvent was enhanced by careful adjustment of input parameters, improving its absorption efficiency by 12% compared to standard operational settings. Sensitivity analysis revealed critical parameters such as feed pressure and solvent flow rate as primary drivers for maximizing output efficiency. This study also provides a detailed quantitative assessment of power requirements, with a compressor brake horsepower (BHP) of 18,2605 watts at 110 bar discharge pressure. It addresses the existing research gap by introducing a systematic approach to process optimization, significantly improving the purity and recovery of CNNG and CO<sub>2</sub> while minimizing energy consumption. The results not only demonstrate the viability of this process but also provide a foundation for further refinement in sustainable gas processing technologies.</div></div>","PeriodicalId":100252,"journal":{"name":"Cleaner Energy Systems","volume":null,"pages":null},"PeriodicalIF":0.0000,"publicationDate":"2024-10-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Simulation of a system to simultaneously recover CO2 and sweet carbon-neutral natural gas from wet natural gas: A delve into process inputs and units performances\",\"authors\":\"Abdulhalim Musa Abubakar , Lukman Buba Umdagas , Moses NyoTonglo Arowo , Marwea Al-Hedrewy , Mahlon Kida Marvin , Noureddine Elboughdiri , Aminullah Zakariyya Abdul , Jenisus O. Dejarlo , Rezkallah Chafika\",\"doi\":\"10.1016/j.cles.2024.100156\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>The growing need for carbon-neutral energy solutions necessitates the development of efficient systems for carbon dioxide (CO<sub>2</sub>) recovery and the production of sweet carbon-neutral natural gas (CNNG) from wet natural gas. Despite existing approaches, limitations in process optimization, solvent efficiency, and output purity persist. This study aims to address these gaps by simulating a system for simultaneous recovery of CO<sub>2</sub> and CNNG using an integrated three-stage process, modeled in Aspen Plus V8.8. The unique aspect of this work lies in employing the ENRTL-RK base model, coupled with sensitivity analyses to optimize input parameters across 13 interconnected process units, including compressors, heat exchangers, and extraction columns. Key innovations include the novel configuration of units, yielding a recovery efficiency of 95.94% for CNNG and a CO<sub>2</sub> purity of 93.185% at optimal conditions, surpassing conventional methods. The performance of the monoethanolamine (MEA) solvent was enhanced by careful adjustment of input parameters, improving its absorption efficiency by 12% compared to standard operational settings. Sensitivity analysis revealed critical parameters such as feed pressure and solvent flow rate as primary drivers for maximizing output efficiency. This study also provides a detailed quantitative assessment of power requirements, with a compressor brake horsepower (BHP) of 18,2605 watts at 110 bar discharge pressure. It addresses the existing research gap by introducing a systematic approach to process optimization, significantly improving the purity and recovery of CNNG and CO<sub>2</sub> while minimizing energy consumption. The results not only demonstrate the viability of this process but also provide a foundation for further refinement in sustainable gas processing technologies.</div></div>\",\"PeriodicalId\":100252,\"journal\":{\"name\":\"Cleaner Energy Systems\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2024-10-28\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Cleaner Energy Systems\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2772783124000505\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Cleaner Energy Systems","FirstCategoryId":"1085","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2772783124000505","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
Simulation of a system to simultaneously recover CO2 and sweet carbon-neutral natural gas from wet natural gas: A delve into process inputs and units performances
The growing need for carbon-neutral energy solutions necessitates the development of efficient systems for carbon dioxide (CO2) recovery and the production of sweet carbon-neutral natural gas (CNNG) from wet natural gas. Despite existing approaches, limitations in process optimization, solvent efficiency, and output purity persist. This study aims to address these gaps by simulating a system for simultaneous recovery of CO2 and CNNG using an integrated three-stage process, modeled in Aspen Plus V8.8. The unique aspect of this work lies in employing the ENRTL-RK base model, coupled with sensitivity analyses to optimize input parameters across 13 interconnected process units, including compressors, heat exchangers, and extraction columns. Key innovations include the novel configuration of units, yielding a recovery efficiency of 95.94% for CNNG and a CO2 purity of 93.185% at optimal conditions, surpassing conventional methods. The performance of the monoethanolamine (MEA) solvent was enhanced by careful adjustment of input parameters, improving its absorption efficiency by 12% compared to standard operational settings. Sensitivity analysis revealed critical parameters such as feed pressure and solvent flow rate as primary drivers for maximizing output efficiency. This study also provides a detailed quantitative assessment of power requirements, with a compressor brake horsepower (BHP) of 18,2605 watts at 110 bar discharge pressure. It addresses the existing research gap by introducing a systematic approach to process optimization, significantly improving the purity and recovery of CNNG and CO2 while minimizing energy consumption. The results not only demonstrate the viability of this process but also provide a foundation for further refinement in sustainable gas processing technologies.