{"title":"地下储氢中生物积液效应的分析研究","authors":"Siqin Yu , Shaowen Mao , Mohamed Mehana","doi":"10.1016/j.ijhydene.2024.11.043","DOIUrl":null,"url":null,"abstract":"<div><div>Underground hydrogen storage (UHS) in porous formations is emerging as a promising solution to global decarbonization. While much knowledge from geologic carbon sequestration is transferable, a critical technical challenge unique to UHS is the active interaction between hydrogen and microbes. In this study, we develop an analytical framework to quantify the bioclogging effect in saline aquifers at the reservoir scale. Our objective is to understand how bioclogging will impact UHS operations and explore potential mitigation strategies. To achieve this, we extend the Buckley–Leverett solution to construct the solution, which is computationally efficient by preserving the analytical nature. Our findings reveal that near-well permeability impairment could be up to twice as severe as previously estimated, emphasizing the advantages of deeper formations with higher temperatures, where microbial activity is reduced. Furthermore, we observed an increase in hydrogen recovery and a progressive advancement of the gas plume front position across storage cycles. These insights not only contribute to designing operational conditions but also suggest effective mitigation strategies for maximizing hydrogen storage efficiency.</div></div>","PeriodicalId":337,"journal":{"name":"International Journal of Hydrogen Energy","volume":"94 ","pages":"Pages 862-870"},"PeriodicalIF":8.1000,"publicationDate":"2024-11-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Analytical study of bioclogging effects in underground hydrogen storage\",\"authors\":\"Siqin Yu , Shaowen Mao , Mohamed Mehana\",\"doi\":\"10.1016/j.ijhydene.2024.11.043\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Underground hydrogen storage (UHS) in porous formations is emerging as a promising solution to global decarbonization. While much knowledge from geologic carbon sequestration is transferable, a critical technical challenge unique to UHS is the active interaction between hydrogen and microbes. In this study, we develop an analytical framework to quantify the bioclogging effect in saline aquifers at the reservoir scale. Our objective is to understand how bioclogging will impact UHS operations and explore potential mitigation strategies. To achieve this, we extend the Buckley–Leverett solution to construct the solution, which is computationally efficient by preserving the analytical nature. Our findings reveal that near-well permeability impairment could be up to twice as severe as previously estimated, emphasizing the advantages of deeper formations with higher temperatures, where microbial activity is reduced. Furthermore, we observed an increase in hydrogen recovery and a progressive advancement of the gas plume front position across storage cycles. These insights not only contribute to designing operational conditions but also suggest effective mitigation strategies for maximizing hydrogen storage efficiency.</div></div>\",\"PeriodicalId\":337,\"journal\":{\"name\":\"International Journal of Hydrogen Energy\",\"volume\":\"94 \",\"pages\":\"Pages 862-870\"},\"PeriodicalIF\":8.1000,\"publicationDate\":\"2024-11-16\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"International Journal of Hydrogen Energy\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0360319924046974\",\"RegionNum\":2,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"International Journal of Hydrogen Energy","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0360319924046974","RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Analytical study of bioclogging effects in underground hydrogen storage
Underground hydrogen storage (UHS) in porous formations is emerging as a promising solution to global decarbonization. While much knowledge from geologic carbon sequestration is transferable, a critical technical challenge unique to UHS is the active interaction between hydrogen and microbes. In this study, we develop an analytical framework to quantify the bioclogging effect in saline aquifers at the reservoir scale. Our objective is to understand how bioclogging will impact UHS operations and explore potential mitigation strategies. To achieve this, we extend the Buckley–Leverett solution to construct the solution, which is computationally efficient by preserving the analytical nature. Our findings reveal that near-well permeability impairment could be up to twice as severe as previously estimated, emphasizing the advantages of deeper formations with higher temperatures, where microbial activity is reduced. Furthermore, we observed an increase in hydrogen recovery and a progressive advancement of the gas plume front position across storage cycles. These insights not only contribute to designing operational conditions but also suggest effective mitigation strategies for maximizing hydrogen storage efficiency.
期刊介绍:
The objective of the International Journal of Hydrogen Energy is to facilitate the exchange of new ideas, technological advancements, and research findings in the field of Hydrogen Energy among scientists and engineers worldwide. This journal showcases original research, both analytical and experimental, covering various aspects of Hydrogen Energy. These include production, storage, transmission, utilization, enabling technologies, environmental impact, economic considerations, and global perspectives on hydrogen and its carriers such as NH3, CH4, alcohols, etc.
The utilization aspect encompasses various methods such as thermochemical (combustion), photochemical, electrochemical (fuel cells), and nuclear conversion of hydrogen, hydrogen isotopes, and hydrogen carriers into thermal, mechanical, and electrical energies. The applications of these energies can be found in transportation (including aerospace), industrial, commercial, and residential sectors.