利用可见光活性 M 型六氟化铅/g-C3N4 复合材料高效去除医院废水中的四环素

IF 2.3 4区 材料科学 Q2 MATERIALS SCIENCE, CERAMICS
Mudasir Mahmood, Shahid Iqbal, Muhammad Jamshaid, Ambreen Kalsoom, Amal M. Al-Mohaimeed, Rashid Iqbal, Firdous Bibi, Qasim Raza, Mohamed Soliman Elshikh
{"title":"利用可见光活性 M 型六氟化铅/g-C3N4 复合材料高效去除医院废水中的四环素","authors":"Mudasir Mahmood,&nbsp;Shahid Iqbal,&nbsp;Muhammad Jamshaid,&nbsp;Ambreen Kalsoom,&nbsp;Amal M. Al-Mohaimeed,&nbsp;Rashid Iqbal,&nbsp;Firdous Bibi,&nbsp;Qasim Raza,&nbsp;Mohamed Soliman Elshikh","doi":"10.1007/s10971-024-06590-8","DOIUrl":null,"url":null,"abstract":"<div><p>The hospital wastewater is major contributor to pharmaceutical contaminants, particularly antibiotic like tetracycline. Tetracycline is often found as a pollutant in water bodies, primarily due to its improper disposal and excretion through human and animal waste. This wastewater poses serious environmental and health risks. We synthesized a novel composite material M type lead hexaferrites/g-carbon nitride (PbFe<sub>12</sub>O<sub>19</sub>/g-C<sub>3</sub>N<sub>4</sub>) to address this alarming issue. The combine effect of lead hexaferrite with graphitic-C<sub>3</sub>N<sub>4</sub>, aiming to enhance the degradation of tetracycline (TC). The characterization of the synthesized composite was conducted using X-ray diffraction spectroscopy (XRD), Scanning electron microscope (SEM), Fourier transform infrared radiation spectroscopy (FTIR) and UV-Visible spectroscopy. The photocatalytic output of the samples was evaluated under sunlight irradiation. The results demonstrated superior removal efficiency of tetracycline up to 90% in only 60 min compared to individual components. This work highlights the potential of PbFe<sub>12</sub>O<sub>19</sub>/g-C<sub>3</sub>N<sub>4</sub> composites as effective photocatalysts for treating pharmaceutical contaminants especially tetracycline in wastewater.</p><h3>Graphical Abstract</h3><div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":664,"journal":{"name":"Journal of Sol-Gel Science and Technology","volume":"112 3","pages":"801 - 813"},"PeriodicalIF":2.3000,"publicationDate":"2024-10-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Efficient tetracycline removal from hospital wastewater using visible light active M-type lead hexaferrite/g-C3N4 composites\",\"authors\":\"Mudasir Mahmood,&nbsp;Shahid Iqbal,&nbsp;Muhammad Jamshaid,&nbsp;Ambreen Kalsoom,&nbsp;Amal M. Al-Mohaimeed,&nbsp;Rashid Iqbal,&nbsp;Firdous Bibi,&nbsp;Qasim Raza,&nbsp;Mohamed Soliman Elshikh\",\"doi\":\"10.1007/s10971-024-06590-8\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>The hospital wastewater is major contributor to pharmaceutical contaminants, particularly antibiotic like tetracycline. Tetracycline is often found as a pollutant in water bodies, primarily due to its improper disposal and excretion through human and animal waste. This wastewater poses serious environmental and health risks. We synthesized a novel composite material M type lead hexaferrites/g-carbon nitride (PbFe<sub>12</sub>O<sub>19</sub>/g-C<sub>3</sub>N<sub>4</sub>) to address this alarming issue. The combine effect of lead hexaferrite with graphitic-C<sub>3</sub>N<sub>4</sub>, aiming to enhance the degradation of tetracycline (TC). The characterization of the synthesized composite was conducted using X-ray diffraction spectroscopy (XRD), Scanning electron microscope (SEM), Fourier transform infrared radiation spectroscopy (FTIR) and UV-Visible spectroscopy. The photocatalytic output of the samples was evaluated under sunlight irradiation. The results demonstrated superior removal efficiency of tetracycline up to 90% in only 60 min compared to individual components. This work highlights the potential of PbFe<sub>12</sub>O<sub>19</sub>/g-C<sub>3</sub>N<sub>4</sub> composites as effective photocatalysts for treating pharmaceutical contaminants especially tetracycline in wastewater.</p><h3>Graphical Abstract</h3><div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>\",\"PeriodicalId\":664,\"journal\":{\"name\":\"Journal of Sol-Gel Science and Technology\",\"volume\":\"112 3\",\"pages\":\"801 - 813\"},\"PeriodicalIF\":2.3000,\"publicationDate\":\"2024-10-14\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Sol-Gel Science and Technology\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://link.springer.com/article/10.1007/s10971-024-06590-8\",\"RegionNum\":4,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"MATERIALS SCIENCE, CERAMICS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Sol-Gel Science and Technology","FirstCategoryId":"88","ListUrlMain":"https://link.springer.com/article/10.1007/s10971-024-06590-8","RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, CERAMICS","Score":null,"Total":0}
引用次数: 0

摘要

医院废水是药物污染物的主要来源,尤其是四环素等抗生素。四环素经常作为污染物出现在水体中,这主要是由于其通过人类和动物排泄物的不当处置和排泄造成的。这种废水对环境和健康构成严重威胁。为了解决这一令人担忧的问题,我们合成了一种新型复合材料 M 型六价铁铅/氮化碳(PbFe12O19/g-C3N4)。六价铁铅与石墨化-C3N4的结合效应旨在增强四环素(TC)的降解。利用 X 射线衍射光谱(XRD)、扫描电子显微镜(SEM)、傅立叶变换红外光谱(FTIR)和紫外-可见光谱对合成的复合材料进行了表征。在阳光照射下,对样品的光催化输出进行了评估。结果表明,与单个成分相比,仅在 60 分钟内四环素的去除率就高达 90%。这项工作凸显了 PbFe12O19/g-C3N4 复合材料作为有效光催化剂处理制药污染物(尤其是废水中的四环素)的潜力。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Efficient tetracycline removal from hospital wastewater using visible light active M-type lead hexaferrite/g-C3N4 composites

Efficient tetracycline removal from hospital wastewater using visible light active M-type lead hexaferrite/g-C3N4 composites

The hospital wastewater is major contributor to pharmaceutical contaminants, particularly antibiotic like tetracycline. Tetracycline is often found as a pollutant in water bodies, primarily due to its improper disposal and excretion through human and animal waste. This wastewater poses serious environmental and health risks. We synthesized a novel composite material M type lead hexaferrites/g-carbon nitride (PbFe12O19/g-C3N4) to address this alarming issue. The combine effect of lead hexaferrite with graphitic-C3N4, aiming to enhance the degradation of tetracycline (TC). The characterization of the synthesized composite was conducted using X-ray diffraction spectroscopy (XRD), Scanning electron microscope (SEM), Fourier transform infrared radiation spectroscopy (FTIR) and UV-Visible spectroscopy. The photocatalytic output of the samples was evaluated under sunlight irradiation. The results demonstrated superior removal efficiency of tetracycline up to 90% in only 60 min compared to individual components. This work highlights the potential of PbFe12O19/g-C3N4 composites as effective photocatalysts for treating pharmaceutical contaminants especially tetracycline in wastewater.

Graphical Abstract

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Journal of Sol-Gel Science and Technology
Journal of Sol-Gel Science and Technology 工程技术-材料科学:硅酸盐
CiteScore
4.70
自引率
4.00%
发文量
280
审稿时长
2.1 months
期刊介绍: The primary objective of the Journal of Sol-Gel Science and Technology (JSST), the official journal of the International Sol-Gel Society, is to provide an international forum for the dissemination of scientific, technological, and general knowledge about materials processed by chemical nanotechnologies known as the "sol-gel" process. The materials of interest include gels, gel-derived glasses, ceramics in form of nano- and micro-powders, bulk, fibres, thin films and coatings as well as more recent materials such as hybrid organic-inorganic materials and composites. Such materials exhibit a wide range of optical, electronic, magnetic, chemical, environmental, and biomedical properties and functionalities. Methods for producing sol-gel-derived materials and the industrial uses of these materials are also of great interest.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信