利用电喷雾质谱法测定人工碳水化合物受体复合物的结合常数和气相稳定性

IF 4.3 3区 材料科学 Q1 ENGINEERING, ELECTRICAL & ELECTRONIC
Alexander Weiß*, Manuel Dutschke, Carla Vogt and Jan Zuber*, 
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引用次数: 0

摘要

近年来,为确定人工碳水化合物受体与苷类化合物的复合物稳定性和选择性而进行的结合研究主要采用 1H NMR、等温滴定量热法(ITC)和其他光谱滴定技术。原生电喷雾离子化(ESI)质谱仅用于验证复合物的化学计量学,但也可以测定解离常数。在本文中,1,3,5-取代的 2,4,6-三乙基苯受体(CHR)与四种烷基-β-d-葡萄糖苷的结合情况各不相同,这些葡萄糖苷的烷基侧链长度分别为甲基(MGP)、己基(HGP)、辛基(OGP)和十二烷基(DGP)、受体与不同烷基侧链长度的烷基-β-d-葡萄糖苷(甲基(MGP)、己基(HGP)、辛基(OGP)和十二烷基(DGP)-β-d-葡萄糖苷)的复合物,在优化的喷雾条件下,采用两种离子模式的 ESI 傅立叶变换离子回旋共振质谱(ESI-FT-ICR-MS)进行了分析。该受体与不同糖类的复合物可按 1:1 和 2:1 的比例进行检测。计算得出的 1:1 复合物的解离常数显示出一种稳定性趋势,这取决于糖的烷基侧链长度:CHR:DGP;CHR:OGP;CHR:HGP;CHR:MGP。通过 CID-MS 测定的气相稳定性证实了这种结合亲和力的相对趋势。这些发现证实了 ESI-MS 作为一种研究非共价复合物稳定性的方法的有效性和适用性,从而为人工受体对碳水化合物的分子识别领域的研究提供了支持。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Determination of Binding Constants and Gas Phase Stabilities of Artificial Carbohydrate Receptor Complexes Using Electrospray Mass Spectrometry

In recent years, binding studies to determine complex stabilities and selectivities of artificial carbohydrate receptors with glycosides have been mainly performed using 1H NMR, isothermal titration calorimetry (ITC), and other spectroscopic titration techniques. Native electrospray ionization (ESI) mass spectrometry is used only to verify the complex stoichiometries, although determination of dissociation constants is also possible. Herein, the binding of a 1,3,5-substituted 2,4,6-triethylbenzene-based receptor (CHR) to four alkyl-β-d-glucosides with varying alkyl side chain lengths (methyl (MGP), hexyl (HGP), octyl (OGP), and dodecyl (DGP)-β-d-glucosides), which was analyzed by ESI Fourier transform ion cyclotron resonance mass spectrometry (ESI-FT-ICR-MS) under optimized spray conditions in both ion modes, is reported. The complexes of the receptor with different sugars could be detected in 1:1 and 2:1 stoichiometries. Dissociation constants calculated for the 1:1 complexes showed a stability trend depending on the length of the alkyl side chain of the sugar: CHR:DGP > CHR:OGP > CHR:HGP > CHR:MGP. Gas phase stabilities determined by CID-MS confirm this relative trend in binding affinities. These findings substantiate the validity and applicability of ESI-MS as a method for investigating noncovalent complex stabilities and thus support research in the field of molecular recognition of carbohydrates by artificial receptors.

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来源期刊
CiteScore
7.20
自引率
4.30%
发文量
567
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