用卟啉衍生物对海绵石墨烯进行超分子修饰可提高太阳能蒸汽发生器的光热转换效率

IF 8.2 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Elif Erçarıkcı, Demet Demirci Gültekin, Ezgi Topçu, Züleyha Kudaş, Murat Alanyalıoğlu and Kader Dağcı Kıranşan*, 
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引用次数: 0

摘要

太阳能似乎是从盐水和废水中获取清洁水的一个很有前景的解决方案。有了太阳能蒸汽发生器系统,就有可能以低成本、可持续和环保的方式有效地从废水中获取清洁水。在本研究中,研究人员利用卟啉衍生物超分子(PRF)对梯度石墨烯海绵材料(GGSM)进行改性,制备出 PRF/GGSM,作为太阳能蒸汽发生器的光热材料。具有石墨烯和卟啉衍生物超分子的 PRF/GGSM 是理想的太阳能热转换器,可轻松收集太阳光。这种材料具有微孔和梯度亲水结构,在 1 个太阳下的太阳热转换效率高达 92%,相当于 3.8 kg h-1 m-2 的水蒸发率。此外,这项研究还表明,PRF/GGSM 能有效地从海水、废水甚至浓酸碱溶液中生成清洁水。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Supramolecular Modification of Graphene Sponge with a Porphyrin Derivative Enhances the Photothermal Conversion Efficiency of a Solar Steam Generator

Solar energy seems to be a promising solution for obtaining clean water from saltwater and wastewater. With the solar steam generator system, it is possible to effectively acquire clean water from wastewater with a low-cost, sustainable, and environmentally friendly approach. In this study, PRF/GGSM, prepared by modification of gradient graphene sponge material (GGSM) with porphyrin derivative supramolecules (PRF), was investigated as a photothermal material for solar steam generation. PRF/GGSM possessing graphene and PRF served as ideal solar thermal converters that could easily gather sunlight. This material owing to its microporous and gradient hydrophilic structure has achieved a solar thermal conversion efficiency of up to 92% under 1 sun, corresponding to the water evaporation rate of 3.8 kg h–1 m–2. Moreover, this study exhibited that PRF/GGSM can efficiently generate clean water from seawater, wastewater, and even concentrated acid and alkali solutions.

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来源期刊
ACS Applied Materials & Interfaces
ACS Applied Materials & Interfaces 工程技术-材料科学:综合
CiteScore
16.00
自引率
6.30%
发文量
4978
审稿时长
1.8 months
期刊介绍: ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.
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