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引用次数: 0
摘要
电气可重构非线性元表面可对二次谐波发生(SHG)等非线性现象进行动态控制,从而开启信号处理、光开关和传感领域的新应用。以往的方法,如等离子体元表面中的电场诱导 SHG 和量子阱元表面中的斯塔克调谐非线性,分别由于金属的微弱 SHG 响应和量子阱的中红外限制而受到限制。为了满足在可见光和近红外范围内有效控制 SHG 的需求,我们提出了一种利用电光(EO)效应调制 SHG 的新方法。通过利用铌酸锂(LN)优异的 EO 和 SHG 特性,我们首次在元表面框架内将 EO 效应与 SHG 相结合。在 ±50 V 交流电压下,我们的铌酸锂元表面实现了 11.3% 的 SHG 振幅调制深度。这些成果为可重构光子应用开辟了新途径,包括可调谐非线性光源、量子光学和非线性信息处理。
Electrically reconfigurable nonlinear metasurfaces provide dynamic control over nonlinear phenomena such as second-harmonic generation (SHG), unlocking novel applications in signal processing, light switching, and sensing. Previous methods, like electric-field-induced SHG in plasmonic metasurfaces and Stark-tuned nonlinearities in quantum well metasurfaces, face limitations due to weak SHG responses from metals and mid-infrared constraints of quantum wells, respectively. Addressing the need for efficient SHG control in the visible and near-infrared ranges, we present a novel approach using the electro-optic (EO) effect to modulate SHG. By leveraging the exceptional EO and SHG properties of lithium niobate (LN), we integrate the EO effect with SHG within a metasurface framework for the first time. Our LN metasurface achieves an 11.3% modulation depth in SHG amplitude under a ±50 V alternating voltage. These results open new avenues for reconfigurable photonic applications. including tunable nonlinear light sources, quantum optics, and nonlinear information processing.
期刊介绍:
Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including:
- Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale
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- Modeling and simulation of synthetic, assembly, and interaction processes
- Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance
- Applications of nanoscale materials in living and environmental systems
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