低温条件下双门控范德瓦耳斯异质结构的片上太赫兹光谱学

IF 9.6 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Junseok Seo, Zhengguang Lu, Seunghyun Park, Jixiang Yang, Fangzhou Xia, Shenyong Ye, Yuxuan Yao, Tonghang Han, Lihan Shi, Kenji Watanabe, Takashi Taniguchi, Amir Yacoby, Long Ju
{"title":"低温条件下双门控范德瓦耳斯异质结构的片上太赫兹光谱学","authors":"Junseok Seo, Zhengguang Lu, Seunghyun Park, Jixiang Yang, Fangzhou Xia, Shenyong Ye, Yuxuan Yao, Tonghang Han, Lihan Shi, Kenji Watanabe, Takashi Taniguchi, Amir Yacoby, Long Ju","doi":"10.1021/acs.nanolett.4c04137","DOIUrl":null,"url":null,"abstract":"Van der Waals heterostructures have emerged as a versatile platform to study correlated and topological electron physics. Spectroscopy experiments in the THz regime are crucial since the energy of THz photons matches that of relevant excitations and charge dynamics. However, their micrometer size and complex (dual-)gated structures have challenged such measurements. Here, we demonstrate on-chip THz spectroscopy on a dual-gated bilayer graphene device at liquid helium temperature. To avoid unwanted THz absorption by metallic gates, we developed a scheme of operation by combining semiconducting gates and optically controlled gating. This allows us to measure the clean THz response of graphene without being affected by the gates. We observed the THz signatures of electric-field-induced bandgap opening at the charge neutrality. We measured Drude conductivities at varied charge densities and extracted key parameters including effective masses and scattering rates. This work paves the way for studying novel emergent phenomena in dual-gated two-dimensional materials.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":null,"pages":null},"PeriodicalIF":9.6000,"publicationDate":"2024-11-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"On-Chip Terahertz Spectroscopy for Dual-Gated van der Waals Heterostructures at Cryogenic Temperatures\",\"authors\":\"Junseok Seo, Zhengguang Lu, Seunghyun Park, Jixiang Yang, Fangzhou Xia, Shenyong Ye, Yuxuan Yao, Tonghang Han, Lihan Shi, Kenji Watanabe, Takashi Taniguchi, Amir Yacoby, Long Ju\",\"doi\":\"10.1021/acs.nanolett.4c04137\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Van der Waals heterostructures have emerged as a versatile platform to study correlated and topological electron physics. Spectroscopy experiments in the THz regime are crucial since the energy of THz photons matches that of relevant excitations and charge dynamics. However, their micrometer size and complex (dual-)gated structures have challenged such measurements. Here, we demonstrate on-chip THz spectroscopy on a dual-gated bilayer graphene device at liquid helium temperature. To avoid unwanted THz absorption by metallic gates, we developed a scheme of operation by combining semiconducting gates and optically controlled gating. This allows us to measure the clean THz response of graphene without being affected by the gates. We observed the THz signatures of electric-field-induced bandgap opening at the charge neutrality. We measured Drude conductivities at varied charge densities and extracted key parameters including effective masses and scattering rates. This work paves the way for studying novel emergent phenomena in dual-gated two-dimensional materials.\",\"PeriodicalId\":53,\"journal\":{\"name\":\"Nano Letters\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":9.6000,\"publicationDate\":\"2024-11-13\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nano Letters\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1021/acs.nanolett.4c04137\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Letters","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acs.nanolett.4c04137","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

范德华异质结构已成为研究相关和拓扑电子物理学的多功能平台。由于太赫兹光子的能量与相关激发和电荷动力学的能量相匹配,因此太赫兹机制下的光谱学实验至关重要。然而,太赫兹光子的微米尺寸和复杂的(双)门控结构给此类测量带来了挑战。在这里,我们展示了在液氦温度下在双栅双层石墨烯器件上进行片上太赫兹光谱分析的方法。为了避免金属栅极产生不必要的太赫兹吸收,我们开发了一种结合半导体栅极和光控栅极的操作方案。这使我们能够测量石墨烯的纯 THz 响应,而不受栅极的影响。我们观察到了电荷中性时电场诱导带隙打开的太赫兹特征。我们测量了不同电荷密度下的德鲁德电导率,并提取了包括有效质量和散射率在内的关键参数。这项工作为研究双栅二维材料中的新出现现象铺平了道路。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

On-Chip Terahertz Spectroscopy for Dual-Gated van der Waals Heterostructures at Cryogenic Temperatures

On-Chip Terahertz Spectroscopy for Dual-Gated van der Waals Heterostructures at Cryogenic Temperatures
Van der Waals heterostructures have emerged as a versatile platform to study correlated and topological electron physics. Spectroscopy experiments in the THz regime are crucial since the energy of THz photons matches that of relevant excitations and charge dynamics. However, their micrometer size and complex (dual-)gated structures have challenged such measurements. Here, we demonstrate on-chip THz spectroscopy on a dual-gated bilayer graphene device at liquid helium temperature. To avoid unwanted THz absorption by metallic gates, we developed a scheme of operation by combining semiconducting gates and optically controlled gating. This allows us to measure the clean THz response of graphene without being affected by the gates. We observed the THz signatures of electric-field-induced bandgap opening at the charge neutrality. We measured Drude conductivities at varied charge densities and extracted key parameters including effective masses and scattering rates. This work paves the way for studying novel emergent phenomena in dual-gated two-dimensional materials.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Nano Letters
Nano Letters 工程技术-材料科学:综合
CiteScore
16.80
自引率
2.80%
发文量
1182
审稿时长
1.4 months
期刊介绍: Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including: - Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale - Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies - Modeling and simulation of synthetic, assembly, and interaction processes - Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance - Applications of nanoscale materials in living and environmental systems Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信