{"title":"基于单宁碳点的甲醛检测","authors":"Yaning Li, Chuanxi Chi, Yue Zhao, Guiquan Jiang, Junhua Wu, Jianxi Song","doi":"10.1016/j.ces.2024.120914","DOIUrl":null,"url":null,"abstract":"With the acceleration of industrialization, formaldehyde detection is becoming increasingly important. Numerous challenges persist about sensitivity and safety in the field of formaldehyde detection. This paper developed a formaldehyde detection material based on carbon dots, and effectively improved the sensitivity, safety and convenience of detection. Specifically, tannin acid (TA) was utilized as the carbon source and urea as the nitrogen source to prepare tannin/urea carbon dots (TA-CDs) with excellent performance. The fluorescence intensity of the carbon dot solution gradually decreased with increasing formaldehyde concentration. A significant linear relationship (R<sup>2</sup> = 0.99462) was observed in the range of 0.00015–0.035 mmol/L, with a practical formaldehyde detection limit of 0.296 μmol/L. This paper utilizes natural poly-phenol compound TA as the raw material, which boasts unique characteristics and low cost. TA-CDs prepared from it are abundant in surface defects and active sites, exhibiting significant advantages in formaldehyde detection and possessing immense application potential.","PeriodicalId":271,"journal":{"name":"Chemical Engineering Science","volume":"146 1","pages":""},"PeriodicalIF":4.1000,"publicationDate":"2024-11-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Formaldehyde detection based on tannin carbon dots\",\"authors\":\"Yaning Li, Chuanxi Chi, Yue Zhao, Guiquan Jiang, Junhua Wu, Jianxi Song\",\"doi\":\"10.1016/j.ces.2024.120914\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"With the acceleration of industrialization, formaldehyde detection is becoming increasingly important. Numerous challenges persist about sensitivity and safety in the field of formaldehyde detection. This paper developed a formaldehyde detection material based on carbon dots, and effectively improved the sensitivity, safety and convenience of detection. Specifically, tannin acid (TA) was utilized as the carbon source and urea as the nitrogen source to prepare tannin/urea carbon dots (TA-CDs) with excellent performance. The fluorescence intensity of the carbon dot solution gradually decreased with increasing formaldehyde concentration. A significant linear relationship (R<sup>2</sup> = 0.99462) was observed in the range of 0.00015–0.035 mmol/L, with a practical formaldehyde detection limit of 0.296 μmol/L. This paper utilizes natural poly-phenol compound TA as the raw material, which boasts unique characteristics and low cost. TA-CDs prepared from it are abundant in surface defects and active sites, exhibiting significant advantages in formaldehyde detection and possessing immense application potential.\",\"PeriodicalId\":271,\"journal\":{\"name\":\"Chemical Engineering Science\",\"volume\":\"146 1\",\"pages\":\"\"},\"PeriodicalIF\":4.1000,\"publicationDate\":\"2024-11-06\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Chemical Engineering Science\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://doi.org/10.1016/j.ces.2024.120914\",\"RegionNum\":2,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENGINEERING, CHEMICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Chemical Engineering Science","FirstCategoryId":"5","ListUrlMain":"https://doi.org/10.1016/j.ces.2024.120914","RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
Formaldehyde detection based on tannin carbon dots
With the acceleration of industrialization, formaldehyde detection is becoming increasingly important. Numerous challenges persist about sensitivity and safety in the field of formaldehyde detection. This paper developed a formaldehyde detection material based on carbon dots, and effectively improved the sensitivity, safety and convenience of detection. Specifically, tannin acid (TA) was utilized as the carbon source and urea as the nitrogen source to prepare tannin/urea carbon dots (TA-CDs) with excellent performance. The fluorescence intensity of the carbon dot solution gradually decreased with increasing formaldehyde concentration. A significant linear relationship (R2 = 0.99462) was observed in the range of 0.00015–0.035 mmol/L, with a practical formaldehyde detection limit of 0.296 μmol/L. This paper utilizes natural poly-phenol compound TA as the raw material, which boasts unique characteristics and low cost. TA-CDs prepared from it are abundant in surface defects and active sites, exhibiting significant advantages in formaldehyde detection and possessing immense application potential.
期刊介绍:
Chemical engineering enables the transformation of natural resources and energy into useful products for society. It draws on and applies natural sciences, mathematics and economics, and has developed fundamental engineering science that underpins the discipline.
Chemical Engineering Science (CES) has been publishing papers on the fundamentals of chemical engineering since 1951. CES is the platform where the most significant advances in the discipline have ever since been published. Chemical Engineering Science has accompanied and sustained chemical engineering through its development into the vibrant and broad scientific discipline it is today.