{"title":"用于室温下 CO$_{2}$ 传感的 TiO$_{2}$ 装饰 MoS$_{2}$ 纳米复合材料","authors":"Rahul Gond;Prajjwal Shukla;Brajesh Rawat","doi":"10.1109/LSENS.2024.3480970","DOIUrl":null,"url":null,"abstract":"Continuous and real-time monitoring of carbon dioxide (CO\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\n) has become an urgent demand due to its significant impact on climate change, asphyxiation risks, agricultural productivity, and human health. Electrochemical sensors for CO\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\n monitoring face challenges, such as slow response time, high operating temperature, and lack of selectivity. To overcome these challenges, we propose a highly selective room-temperature (RT) CO\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\n detection sensor based on TiO\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\n-MoS\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\n nanocomposite (NC), which is manufactured using a screen printing methodology. The fabricated sensor achieved a response of approximately 2.11% and response/recovery times of nearly 102/37s at 1000 ppm. The sensitivity is observed to be approximately 0.0032%/ppm with an excellent response for the CO\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\n concentration range of 500–5000 ppm. Despite the typically low selectivity of unreactive CO\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\n gas, the fabricated sensor exhibits high selectivity, with a response of around 2.21× higher than that of the CO gas with the next highest response. The scalable fabrication methodology and RT operation make TiO\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\n-MoS\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\n sensor a highly viable candidate for production through a cost-effective and high performance CO\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\n sensing.","PeriodicalId":13014,"journal":{"name":"IEEE Sensors Letters","volume":"8 11","pages":"1-4"},"PeriodicalIF":2.2000,"publicationDate":"2024-10-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"TiO$_{2}$-Decorated MoS$_{2}$ Nanocomposite for CO$_{2}$ Sensing At Room Temperature\",\"authors\":\"Rahul Gond;Prajjwal Shukla;Brajesh Rawat\",\"doi\":\"10.1109/LSENS.2024.3480970\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Continuous and real-time monitoring of carbon dioxide (CO\\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\\n) has become an urgent demand due to its significant impact on climate change, asphyxiation risks, agricultural productivity, and human health. Electrochemical sensors for CO\\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\\n monitoring face challenges, such as slow response time, high operating temperature, and lack of selectivity. To overcome these challenges, we propose a highly selective room-temperature (RT) CO\\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\\n detection sensor based on TiO\\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\\n-MoS\\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\\n nanocomposite (NC), which is manufactured using a screen printing methodology. The fabricated sensor achieved a response of approximately 2.11% and response/recovery times of nearly 102/37s at 1000 ppm. The sensitivity is observed to be approximately 0.0032%/ppm with an excellent response for the CO\\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\\n concentration range of 500–5000 ppm. Despite the typically low selectivity of unreactive CO\\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\\n gas, the fabricated sensor exhibits high selectivity, with a response of around 2.21× higher than that of the CO gas with the next highest response. The scalable fabrication methodology and RT operation make TiO\\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\\n-MoS\\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\\n sensor a highly viable candidate for production through a cost-effective and high performance CO\\n<inline-formula><tex-math>$_{2}$</tex-math></inline-formula>\\n sensing.\",\"PeriodicalId\":13014,\"journal\":{\"name\":\"IEEE Sensors Letters\",\"volume\":\"8 11\",\"pages\":\"1-4\"},\"PeriodicalIF\":2.2000,\"publicationDate\":\"2024-10-15\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"IEEE Sensors Letters\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://ieeexplore.ieee.org/document/10717425/\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"ENGINEERING, ELECTRICAL & ELECTRONIC\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"IEEE Sensors Letters","FirstCategoryId":"1085","ListUrlMain":"https://ieeexplore.ieee.org/document/10717425/","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"ENGINEERING, ELECTRICAL & ELECTRONIC","Score":null,"Total":0}
TiO$_{2}$-Decorated MoS$_{2}$ Nanocomposite for CO$_{2}$ Sensing At Room Temperature
Continuous and real-time monitoring of carbon dioxide (CO
$_{2}$
) has become an urgent demand due to its significant impact on climate change, asphyxiation risks, agricultural productivity, and human health. Electrochemical sensors for CO
$_{2}$
monitoring face challenges, such as slow response time, high operating temperature, and lack of selectivity. To overcome these challenges, we propose a highly selective room-temperature (RT) CO
$_{2}$
detection sensor based on TiO
$_{2}$
-MoS
$_{2}$
nanocomposite (NC), which is manufactured using a screen printing methodology. The fabricated sensor achieved a response of approximately 2.11% and response/recovery times of nearly 102/37s at 1000 ppm. The sensitivity is observed to be approximately 0.0032%/ppm with an excellent response for the CO
$_{2}$
concentration range of 500–5000 ppm. Despite the typically low selectivity of unreactive CO
$_{2}$
gas, the fabricated sensor exhibits high selectivity, with a response of around 2.21× higher than that of the CO gas with the next highest response. The scalable fabrication methodology and RT operation make TiO
$_{2}$
-MoS
$_{2}$
sensor a highly viable candidate for production through a cost-effective and high performance CO
$_{2}$
sensing.