Michal Sanocki, Hayley C. Russell, Jasemine Handjaya, Jolene P. Reid
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Relative Generality and Risk: Quantitative Measures for Broad Catalyst Success
The performance of chiral catalysts is typically evaluated against empirical reaction outputs like yield and selectivity with traditional analyses limited to a single model system. Expansion of the reaction space permits catalysts to be assessed for generality, and this provides another useful metric for measuring the effectiveness of a catalyst. The catalyst generality algorithm will assign quantitative generality values to catalyst structures, but such broad assessments are applied with the assumption that the reactions under evaluation are more or less the same by disregarding any inherent challenges associated with a particular reaction class. To address this limitation, we introduce two metrics: relative generality and risk. These are designed to correct for variations in reaction difficulty and enable a more nuanced evaluation of the catalyst performance relative to the specific demands of each reaction. We show in a number of challenging examples that these metrics allow researchers to distinguish between catalysts genuinely exhibiting superior performance and those appearing favorable due to application toward less demanding reactions. This represents a significant advancement in quantifying catalyst success with demonstrated applications in retrospective analyses and early insights into emerging catalyst classes.
期刊介绍:
ACS Catalysis is an esteemed journal that publishes original research in the fields of heterogeneous catalysis, molecular catalysis, and biocatalysis. It offers broad coverage across diverse areas such as life sciences, organometallics and synthesis, photochemistry and electrochemistry, drug discovery and synthesis, materials science, environmental protection, polymer discovery and synthesis, and energy and fuels.
The scope of the journal is to showcase innovative work in various aspects of catalysis. This includes new reactions and novel synthetic approaches utilizing known catalysts, the discovery or modification of new catalysts, elucidation of catalytic mechanisms through cutting-edge investigations, practical enhancements of existing processes, as well as conceptual advances in the field. Contributions to ACS Catalysis can encompass both experimental and theoretical research focused on catalytic molecules, macromolecules, and materials that exhibit catalytic turnover.