极性天电晶体晶格中位错的沃尔特拉弹性理论破译

IF 9.1 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Kohta Kasai*, Tao Xu, Susumu Minami and Takahiro Shimada*, 
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引用次数: 0

摘要

新出现的极性天融晶体(SkX)由于其非对称的电偶极子拓扑结构、类类粒子行为和独特的电反应,在技术应用方面引起了广泛关注。了解 SkX 缺陷(尤其是位错)对其独特的晶格动力学和响应至关重要;然而,这一点仍然难以捉摸。在这里,我们不仅证明了 SkX 位错表现出异常变形的核心结构,天元伸长率超过 50%,而且还发现在 SkX 中,Volterra 的位错弹性理论被打破了。我们的相场模拟显示,SkX 位错的这些明显特征源于天元的刚柔准粒子转变,这取决于电场和温度。在 SkX 中,存在固有的力学机制,可通过天元的迁移和变形来缓解错配。这项工作提供了对一类新的晶格力学和由准粒子 SkX 独特性质产生的相关功能的新见解。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Breakdown of Volterra’s Elasticity Theory of Dislocations in Polar Skyrmion Lattices

Breakdown of Volterra’s Elasticity Theory of Dislocations in Polar Skyrmion Lattices

Emerging polar skyrmion crystals (SkX) have raised much interest for technological applications owing to their nontrivial topologies of electric dipoles, quasiparticle-like behaviors, and unique electrical responses. Understanding SkX defects, especially dislocations, is crucial for their unique lattice dynamics and responses; however, it still remains elusive. Here, we have not only demonstrated that a SkX dislocation exhibits an anomalously deformed core structure with over 50% elongation of skyrmions but also discovered that Volterra’s elasticity theory of dislocation is broken down in SkX. Our phase-field simulation reveals that these distinct features of SkX dislocation arise from a rigid to soft quasiparticle transition of skyrmions depending on the electric field and temperature. In SkX, there exist inherent mechanics that mitigate the mismatch by both migration and deformation of skyrmions. This work provides novel insights into a new class of lattice mechanics and related functionality arising from the unique properties of quasi-particle SkX.

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来源期刊
Nano Letters
Nano Letters 工程技术-材料科学:综合
CiteScore
16.80
自引率
2.80%
发文量
1182
审稿时长
1.4 months
期刊介绍: Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including: - Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale - Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies - Modeling and simulation of synthetic, assembly, and interaction processes - Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance - Applications of nanoscale materials in living and environmental systems Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.
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