{"title":"利用煤气化炉渣制备用于处理兰炭废水的吸附剂及其吸附机理。","authors":"Huan-Xi Wang, Jia-Rui Zhao, Yu-Tong He, Yun-Hua Xu","doi":"10.1080/09593330.2024.2420285","DOIUrl":null,"url":null,"abstract":"<p><p>Solid waste coal gasification slag has certain hardness, porosity, pore structure and specific surface area, etc. which can be utilized in environmental protection materials and other areas of high value. Yulin City, high-quality coal resources derived from the excellent quality of charcoal products, but its processing will produce a large number of high chemical oxygen demand (COD), high volatile phenol, high ammonia nitrogen 'three high' wastewater, the ecological environment is very harmful. The results of the modification of the refined coal gasification fine residue showed that the removal rates of the three were enhanced to 91%, 89% and 83%, respectively, after adsorption at a pH of 9.5, an injection ratio of 1:5 and 25 ℃ for 25 min. The reason is that the modification treatment significantly increased the specific surface area of the adsorbent from 103 m<sup>2</sup>/g to 606 m<sup>2</sup>/g, which effectively increased the adsorption active sites for the pollutant molecules. The adsorption process of COD from modified refining coal gasification slag for the treatment of charcoal wastewater was thermodynamically investigated. The thermodynamic study shows that the adsorption process of modified refining coal gasification slag on pollutants in the charcoal wastewater is an exothermic and spontaneous process.</p>","PeriodicalId":12009,"journal":{"name":"Environmental Technology","volume":" ","pages":"2092-2109"},"PeriodicalIF":2.2000,"publicationDate":"2025-05-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Preparation of adsorbent from coal gasification slag for the treatment of waste water from lanchar and its adsorption mechanism.\",\"authors\":\"Huan-Xi Wang, Jia-Rui Zhao, Yu-Tong He, Yun-Hua Xu\",\"doi\":\"10.1080/09593330.2024.2420285\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>Solid waste coal gasification slag has certain hardness, porosity, pore structure and specific surface area, etc. which can be utilized in environmental protection materials and other areas of high value. Yulin City, high-quality coal resources derived from the excellent quality of charcoal products, but its processing will produce a large number of high chemical oxygen demand (COD), high volatile phenol, high ammonia nitrogen 'three high' wastewater, the ecological environment is very harmful. The results of the modification of the refined coal gasification fine residue showed that the removal rates of the three were enhanced to 91%, 89% and 83%, respectively, after adsorption at a pH of 9.5, an injection ratio of 1:5 and 25 ℃ for 25 min. The reason is that the modification treatment significantly increased the specific surface area of the adsorbent from 103 m<sup>2</sup>/g to 606 m<sup>2</sup>/g, which effectively increased the adsorption active sites for the pollutant molecules. The adsorption process of COD from modified refining coal gasification slag for the treatment of charcoal wastewater was thermodynamically investigated. The thermodynamic study shows that the adsorption process of modified refining coal gasification slag on pollutants in the charcoal wastewater is an exothermic and spontaneous process.</p>\",\"PeriodicalId\":12009,\"journal\":{\"name\":\"Environmental Technology\",\"volume\":\" \",\"pages\":\"2092-2109\"},\"PeriodicalIF\":2.2000,\"publicationDate\":\"2025-05-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Environmental Technology\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://doi.org/10.1080/09593330.2024.2420285\",\"RegionNum\":4,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"2024/10/28 0:00:00\",\"PubModel\":\"Epub\",\"JCR\":\"Q3\",\"JCRName\":\"ENVIRONMENTAL SCIENCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Environmental Technology","FirstCategoryId":"93","ListUrlMain":"https://doi.org/10.1080/09593330.2024.2420285","RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2024/10/28 0:00:00","PubModel":"Epub","JCR":"Q3","JCRName":"ENVIRONMENTAL SCIENCES","Score":null,"Total":0}
Preparation of adsorbent from coal gasification slag for the treatment of waste water from lanchar and its adsorption mechanism.
Solid waste coal gasification slag has certain hardness, porosity, pore structure and specific surface area, etc. which can be utilized in environmental protection materials and other areas of high value. Yulin City, high-quality coal resources derived from the excellent quality of charcoal products, but its processing will produce a large number of high chemical oxygen demand (COD), high volatile phenol, high ammonia nitrogen 'three high' wastewater, the ecological environment is very harmful. The results of the modification of the refined coal gasification fine residue showed that the removal rates of the three were enhanced to 91%, 89% and 83%, respectively, after adsorption at a pH of 9.5, an injection ratio of 1:5 and 25 ℃ for 25 min. The reason is that the modification treatment significantly increased the specific surface area of the adsorbent from 103 m2/g to 606 m2/g, which effectively increased the adsorption active sites for the pollutant molecules. The adsorption process of COD from modified refining coal gasification slag for the treatment of charcoal wastewater was thermodynamically investigated. The thermodynamic study shows that the adsorption process of modified refining coal gasification slag on pollutants in the charcoal wastewater is an exothermic and spontaneous process.
期刊介绍:
Environmental Technology is a leading journal for the rapid publication of science and technology papers on a wide range of topics in applied environmental studies, from environmental engineering to environmental biotechnology, the circular economy, municipal and industrial wastewater management, drinking-water treatment, air- and water-pollution control, solid-waste management, industrial hygiene and associated technologies.
Environmental Technology is intended to provide rapid publication of new developments in environmental technology. The journal has an international readership with a broad scientific base. Contributions will be accepted from scientists and engineers in industry, government and universities. Accepted manuscripts are generally published within four months.
Please note that Environmental Technology does not publish any review papers unless for a specified special issue which is decided by the Editor. Please do submit your review papers to our sister journal Environmental Technology Reviews at http://www.tandfonline.com/toc/tetr20/current