卟啉-石墨烯结构催化氢气转化微型综述。

IF 5.3 3区工程技术 Q2 ENERGY & FUELS

Energy & Fuels Pub Date : 2024-09-25 eCollection Date: 2024-10-17 DOI:10.1021/acs.energyfuels.4c03322

Emmanouil Nikoloudakis, Athanassios G Coutsolelos, Emmanuel Stratakis

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引用次数: 0

摘要

卟啉基衍生物作为光敏剂和催化剂，在光催化、电催化和光电催化制氢系统中得到了广泛研究。最近，由于氧化石墨烯、还原氧化石墨烯和石墨烯量子点等二维材料具有先进的电子特性、良好的稳定性和低成本制造，它们与这些材料的结合在氢气进化方面引起了极大的关注。这篇微型综述总结了卟啉-石墨烯组合在催化氢气生成中应用的最新进展。文中讨论了当前在这一应用中面临的挑战，并提出了未来的展望。

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Mini-Review on Catalytic Hydrogen Evolution from Porphyrin-Graphene Structures.

Porphyrin-based derivatives have been extensively investigated in photocatalytic, electrocatalytic, and photoelectrocatalytic H₂ production systems as both photosensitizers and catalysts. Recently, their combination with two-dimensional materials, such as graphene oxide, reduced graphene oxide, and graphene quantum dots, has attracted significant attention for hydrogen evolution due to the advanced electronic properties, good stability, and low-cost fabrication of these materials. This mini-review summarizes the recent developments concerning the application of porphyrin-graphene ensembles in catalytic H₂ generation. Current challenges concerning this application are discussed, and future perspectives are also proposed.

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来源期刊

Energy & Fuels 工程技术-工程：化工

CiteScore

9.20

自引率

13.20%

发文量

1101

审稿时长

2.1 months

期刊介绍： Energy & Fuels publishes reports of research in the technical area defined by the intersection of the disciplines of chemistry and chemical engineering and the application domain of non-nuclear energy and fuels. This includes research directed at the formation of, exploration for, and production of fossil fuels and biomass; the properties and structure or molecular composition of both raw fuels and refined products; the chemistry involved in the processing and utilization of fuels; fuel cells and their applications; and the analytical and instrumental techniques used in investigations of the foregoing areas.