Matthew A Aubourg, Kenneth J T Livi, Gregory G Sawtell, Carlos C Sanchez-Gonzalez, Nicholas J Spada, Russell R Dickerson, Wen-An Chiou, Conchita Kamanzi, Gurumurthy Ramachandran, Ana M Rule, Christopher D Heaney
{"title":"利用电子显微镜确定美国马里兰州巴尔的摩市柯蒂斯湾露天煤炭码头附近居民区是否存在煤尘。","authors":"Matthew A Aubourg, Kenneth J T Livi, Gregory G Sawtell, Carlos C Sanchez-Gonzalez, Nicholas J Spada, Russell R Dickerson, Wen-An Chiou, Conchita Kamanzi, Gurumurthy Ramachandran, Ana M Rule, Christopher D Heaney","doi":"10.1016/j.scitotenv.2024.176842","DOIUrl":null,"url":null,"abstract":"<p><strong>Background: </strong>Despite decreasing US consumption, over 90 million metric tons of coal were exported by the US in 2023, requiring significant infrastructure for transport, handling, and storage of coal at export terminals. Residents in Curtis Bay, Baltimore, Maryland, USA live at the fenceline of an open-air coal terminal and have, for decades, reported rapid accumulation of black dust at their homes. Community-level exposure to coal dust originating from coal handling and storage terminals has remained largely unexplored.</p><p><strong>Objectives: </strong>To investigate community-identified concerns and use a community-driven approach to determine the presence/absence of coal dust on Curtis Bay surfaces.</p><p><strong>Methods: </strong>Passive settled dust samples were collected from two residential areas, 345 m and 1235 m from the coal terminal, using conductive carbon tape. Scanning electron microscopy and energy dispersive X-ray spectroscopy (SEM-EDX) of standard reference coal material and positive control material from the coal terminal in Curtis Bay were used to optimize the morphological and elemental classification criteria for coal dust. A manual SEM-EDX protocol was developed to identify coal particles in settled dust collected on conductive carbon tape in community settings.</p><p><strong>Results: </strong>SEM-EDX analysis confirmed presence of coal dust sampled at both residential locations. Estimated coal dust particle loading at the proximal and distal site were 13.2 and 3.4 coal particles/mm<sup>2</sup>, respectively. The coal dust particles identified met specific criteria, including size (>5 μm), morphology, and elemental composition (≥75 % carbon, ≤20 % oxygen).</p><p><strong>Discussion: </strong>These findings are consistent with longstanding community concerns and lived experiences regarding the presence of coal dust in Curtis Bay, which neighbors a major open-air coal terminal. This approach has potential for other communities neighboring coal terminals to assess similar concerns with residential coal dust exposure.</p>","PeriodicalId":422,"journal":{"name":"Science of the Total Environment","volume":" ","pages":"176842"},"PeriodicalIF":8.2000,"publicationDate":"2024-12-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Use of electron microscopy to determine presence of coal dust in a neighborhood bordering an open-air coal terminal in Curtis Bay, Baltimore, Maryland, USA.\",\"authors\":\"Matthew A Aubourg, Kenneth J T Livi, Gregory G Sawtell, Carlos C Sanchez-Gonzalez, Nicholas J Spada, Russell R Dickerson, Wen-An Chiou, Conchita Kamanzi, Gurumurthy Ramachandran, Ana M Rule, Christopher D Heaney\",\"doi\":\"10.1016/j.scitotenv.2024.176842\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><strong>Background: </strong>Despite decreasing US consumption, over 90 million metric tons of coal were exported by the US in 2023, requiring significant infrastructure for transport, handling, and storage of coal at export terminals. Residents in Curtis Bay, Baltimore, Maryland, USA live at the fenceline of an open-air coal terminal and have, for decades, reported rapid accumulation of black dust at their homes. Community-level exposure to coal dust originating from coal handling and storage terminals has remained largely unexplored.</p><p><strong>Objectives: </strong>To investigate community-identified concerns and use a community-driven approach to determine the presence/absence of coal dust on Curtis Bay surfaces.</p><p><strong>Methods: </strong>Passive settled dust samples were collected from two residential areas, 345 m and 1235 m from the coal terminal, using conductive carbon tape. Scanning electron microscopy and energy dispersive X-ray spectroscopy (SEM-EDX) of standard reference coal material and positive control material from the coal terminal in Curtis Bay were used to optimize the morphological and elemental classification criteria for coal dust. A manual SEM-EDX protocol was developed to identify coal particles in settled dust collected on conductive carbon tape in community settings.</p><p><strong>Results: </strong>SEM-EDX analysis confirmed presence of coal dust sampled at both residential locations. Estimated coal dust particle loading at the proximal and distal site were 13.2 and 3.4 coal particles/mm<sup>2</sup>, respectively. The coal dust particles identified met specific criteria, including size (>5 μm), morphology, and elemental composition (≥75 % carbon, ≤20 % oxygen).</p><p><strong>Discussion: </strong>These findings are consistent with longstanding community concerns and lived experiences regarding the presence of coal dust in Curtis Bay, which neighbors a major open-air coal terminal. This approach has potential for other communities neighboring coal terminals to assess similar concerns with residential coal dust exposure.</p>\",\"PeriodicalId\":422,\"journal\":{\"name\":\"Science of the Total Environment\",\"volume\":\" \",\"pages\":\"176842\"},\"PeriodicalIF\":8.2000,\"publicationDate\":\"2024-12-20\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Science of the Total Environment\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://doi.org/10.1016/j.scitotenv.2024.176842\",\"RegionNum\":1,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"2024/10/11 0:00:00\",\"PubModel\":\"Epub\",\"JCR\":\"Q1\",\"JCRName\":\"ENVIRONMENTAL SCIENCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Science of the Total Environment","FirstCategoryId":"93","ListUrlMain":"https://doi.org/10.1016/j.scitotenv.2024.176842","RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2024/10/11 0:00:00","PubModel":"Epub","JCR":"Q1","JCRName":"ENVIRONMENTAL SCIENCES","Score":null,"Total":0}
Use of electron microscopy to determine presence of coal dust in a neighborhood bordering an open-air coal terminal in Curtis Bay, Baltimore, Maryland, USA.
Background: Despite decreasing US consumption, over 90 million metric tons of coal were exported by the US in 2023, requiring significant infrastructure for transport, handling, and storage of coal at export terminals. Residents in Curtis Bay, Baltimore, Maryland, USA live at the fenceline of an open-air coal terminal and have, for decades, reported rapid accumulation of black dust at their homes. Community-level exposure to coal dust originating from coal handling and storage terminals has remained largely unexplored.
Objectives: To investigate community-identified concerns and use a community-driven approach to determine the presence/absence of coal dust on Curtis Bay surfaces.
Methods: Passive settled dust samples were collected from two residential areas, 345 m and 1235 m from the coal terminal, using conductive carbon tape. Scanning electron microscopy and energy dispersive X-ray spectroscopy (SEM-EDX) of standard reference coal material and positive control material from the coal terminal in Curtis Bay were used to optimize the morphological and elemental classification criteria for coal dust. A manual SEM-EDX protocol was developed to identify coal particles in settled dust collected on conductive carbon tape in community settings.
Results: SEM-EDX analysis confirmed presence of coal dust sampled at both residential locations. Estimated coal dust particle loading at the proximal and distal site were 13.2 and 3.4 coal particles/mm2, respectively. The coal dust particles identified met specific criteria, including size (>5 μm), morphology, and elemental composition (≥75 % carbon, ≤20 % oxygen).
Discussion: These findings are consistent with longstanding community concerns and lived experiences regarding the presence of coal dust in Curtis Bay, which neighbors a major open-air coal terminal. This approach has potential for other communities neighboring coal terminals to assess similar concerns with residential coal dust exposure.
期刊介绍:
The Science of the Total Environment is an international journal dedicated to scientific research on the environment and its interaction with humanity. It covers a wide range of disciplines and seeks to publish innovative, hypothesis-driven, and impactful research that explores the entire environment, including the atmosphere, lithosphere, hydrosphere, biosphere, and anthroposphere.
The journal's updated Aims & Scope emphasizes the importance of interdisciplinary environmental research with broad impact. Priority is given to studies that advance fundamental understanding and explore the interconnectedness of multiple environmental spheres. Field studies are preferred, while laboratory experiments must demonstrate significant methodological advancements or mechanistic insights with direct relevance to the environment.