Minseob Lim, Jun Young Kim, Hyunji Kang, Tae Woong Yun, Hong-Baek Cho, Yong-Ho Choa
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引用次数: 0
摘要
本研究介绍了一种新型氢气传感器,它可在室温下高效工作,并具有高灵敏度和高选择性。这种传感器是利用激光诱导石墨烯(Pt/LIG)结构上的铂制作而成的。合成过程包括制造具有大表面积的高结晶石墨烯,它是纳米级铂催化剂的最佳载体。合成后的铂纳米粒子分散在 LIG 电极表面,并设想在环境条件下实现氢气传感性能,而无需加热或传感器装置。分析表明,铂纳米粒子的独特之处在于其小于 5 纳米的窄尺寸分布及其在 LIG 基底上的均匀沉积,LIG 基底本身具有 187.4 平方米/克的巨大比表面积。这种配置使传感器能够实现 200 ppb 的极低氢检测限。此外,该传感器还具有卓越的性能特性,包括高灵敏度、出色的线性度和超过 50 次循环的卓越稳定性。LIG 的高比表面积与铂纳米粒子的催化活性之间的协同作用有助于在室温下检测氢气。这项研究极大地促进了气体传感技术领域的发展,尤其是在需要在环境条件下准确可靠地检测氢气的应用领域。
Room temperature-based hydrogen gas sensing over Laser-Induced Graphene electrode supported Pt nanoparticles for low LOD
This study introduces a novel hydrogen sensor that operates efficiently at room temperature with high sensitivity and selectivity. This sensor was created by utilizing a platinum on laser-induced graphene (Pt/LIG) structure. The synthesis process involves the creation of highly crystalline graphene with a large surface area, which serves as an optimal support for nanosized pt catalysts. Post-synthesized Pt nanoparticles were dispersed on the surface of the LIG electrode and envisaged for the hydrogen gas sensing property under ambient conditions without a heating or sensor device. Analysis showed that the Pt nanoparticles are uniquely characterized by their narrow size distribution of less than 5 nm and their homogeneous deposition on the LIG substrate, which itself exhibits a substantial specific surface area of 187.4 m²/g. This configuration enables the sensor to achieve a very low limit for detection of hydrogen to 200 ppb. Moreover, the sensor demonstrates exceptional performance attributes, including high sensitivity, excellent linearity, and remarkable cycle stability over 50 cycles. The synergy between the high surface area of the LIG and the catalytic activity of the Pt nanoparticles facilitates the detection of hydrogen at room temperature. This study contributes significantly to the field of gas sensing technology, particularly in applications requiring accurate and reliable hydrogen detection at ambient conditions.
期刊介绍:
Sensors and Actuators Reports is a peer-reviewed open access journal launched out from the Sensors and Actuators journal family. Sensors and Actuators Reports is dedicated to publishing new and original works in the field of all type of sensors and actuators, including bio-, chemical-, physical-, and nano- sensors and actuators, which demonstrates significant progress beyond the current state of the art. The journal regularly publishes original research papers, reviews, and short communications.
For research papers and short communications, the journal aims to publish the new and original work supported by experimental results and as such purely theoretical works are not accepted.